Strong light emission from defective hexagonal boron nitride monolayer coupled to near-touching random plasmonic nanounits

2021 ◽  
Author(s):  
Zeinab Eftekhari ◽  
Amir Ghobadi ◽  
Mahmut Soydan ◽  
Deniz Yildirim ◽  
neval cinel ◽  
...  
2019 ◽  
Vol 2 (1) ◽  
Author(s):  
Snežana Lazić ◽  
André Espinha ◽  
Sergio Pinilla Yanguas ◽  
Carlos Gibaja ◽  
Félix Zamora ◽  
...  

Abstract Luminescent defects in hexagonal boron nitride (h-BN) have recently emerged as a promising platform for non-classical light emission. On-chip solutions, however, require techniques for controllable in-situ manipulation of quantum light. Here, we demonstrate the dynamic spectral and temporal tuning of the optical emission from h-BN via moving acousto-mechanical modulation induced by stimulated phonons. When perturbed by the propagating acoustic phonon, the optically probed radiative h-BN defects are periodically strained and their sharp emission lines are modulated by the deformation potential coupling. This results in an acoustically driven spectral tuning within a 2.5-meV bandwidth. Our findings, supported by first-principles theoretical calculations, reveal exceptionally high elasto-optic coupling in h-BN of ~50 meV/%. Temporal control of the emitted photons is achieved by combining the acoustically mediated fine-spectral tuning with spectral detection filtering. This study opens the door to the use of sound for scalable integration of h-BN emitters in nanophotonic and quantum information technologies.


2014 ◽  
Vol 20 (4) ◽  
pp. 1053-1059 ◽  
Author(s):  
Nicholas L. McDougall ◽  
Rebecca J. Nicholls ◽  
Jim G. Partridge ◽  
Dougal G. McCulloch

AbstractHexagonal boron nitride (hBN) is a promising material for a range of applications including deep-ultraviolet light emission. Despite extensive experimental studies, some fundamental aspects of hBN remain unknown, such as the type of stacking faults likely to be present and their influence on electronic properties. In this paper, different stacking configurations of hBN are investigated using CASTEP, a pseudopotential density functional theory code. AB-b stacking faults, in which B atoms are positioned directly on top of one another while N atoms are located above the center of BN hexagons, are shown to be likely in conventional AB stacked hBN. Bandstructure calculations predict a single direct bandgap structure that may be responsible for the discrepancies in bandgap type observed experimentally. Calculations of the near edge structure showed that different stackings of hBN are distinguishable using measurements of core-loss edges in X-ray absorption and electron energy loss spectroscopy. AB stacking was found to best reproduce features in the experimental B and N K-edges. The calculations also show that splitting of the 1s to π* peak in the B K-edge, recently observed experimentally, may be accounted for by the presence of AB-b stacking faults.


2020 ◽  
Vol 124 (37) ◽  
pp. 7340-7345
Author(s):  
Beilei Sun ◽  
Xin Xu ◽  
Guodong Zhou ◽  
Li Tao ◽  
Wang Xinran ◽  
...  

2016 ◽  
Vol 41 (21) ◽  
pp. 4991 ◽  
Author(s):  
Bofeng Zhu ◽  
Guobin Ren ◽  
Yixiao Gao ◽  
Haisu Li ◽  
Beilei Wu ◽  
...  

Nanophotonics ◽  
2019 ◽  
Vol 8 (11) ◽  
pp. 2041-2048 ◽  
Author(s):  
Alexander Bommer ◽  
Christoph Becher

AbstractIn recent years, mono-layers and multi-layers of hexagonal boron nitride (hBN) have been demonstrated as host materials for localized atomic defects that can be used as emitters for ultra-bright, non-classical light. The origin of the emission, however, is still subject to debate. Based on measurements of photon statistics, lifetime and polarization on selected emitters, we find that these atomic defects do not act as pure single photon emitters. Our results strongly and consistently indicate that each zero phonon line of individual emitters comprises two independent electronic transitions. These results give new insights into the nature of the observed emission and hint at a double defect nature of emitters in multi-layer hBN.


2021 ◽  
Vol 11 (1) ◽  
Author(s):  
Akbar Basha Dhu-al-jalali-wal-ikram Shaik ◽  
Penchalaiah Palla

AbstractSingle photon quantum emitters are important building blocks of optical quantum technologies. Hexagonal boron nitride (hBN), an atomically thin wide band gap two dimensional material, hosts robust, optically active luminescent point defects, which are known to reduce phonon lifetimes, promises as a stable single-photon source at room temperature. In this Review, we present the recent advances in hBN quantum light emission, comparisons with other 2D material based quantum sources and analyze the performance of hBN quantum emitters. We also discuss state-of-the-art stable single photon emitter’s fabrication in UV, visible and near IR regions, their activation, characterization techniques, photostability towards a wide range of operating temperatures and harsh environments, Density-functional theory predictions of possible hBN defect structures for single photon emission in UV to IR regions and applications of single photon sources in quantum communication and quantum photonic circuits with associated potential obstacles.


2D Materials ◽  
2016 ◽  
Vol 4 (1) ◽  
pp. 011004 ◽  
Author(s):  
T Q P Vuong ◽  
G Cassabois ◽  
P Valvin ◽  
V Jacques ◽  
A Van Der Lee ◽  
...  

Nano Letters ◽  
2021 ◽  
Author(s):  
Anna Kuzmina ◽  
Markus Parzefall ◽  
Patrick Back ◽  
Takashi Taniguchi ◽  
Kenji Watanabe ◽  
...  

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