Measurement of the neutron energy spectrum of Back-n #ES1 at CSNS

The China spallation neutron source (CSNS) was built and started running since 2018. It produces neutrons by impinging 1.6 GeV protons onto a tungsten target with 25 Hz repetition frequency. A beam line exploiting the back-streaming neutrons (Back-n) was built mainly for nuclear data measurement and started commissioning simultaneously with CSNS in 2018. There are two experimental endstations along the Back-n beam line: endstation 1 (#ES1) with a neutron flight path of about 55 m and endstation 2 (#ES2) with about 76 m. The neutron energy spectra of both #ES1 and #ES2 were measured since it is important for feasibility study and analysis. In this paper, the measurement of the neutron energy spectrum of Back-n #ES1 is reported. It is measured by a multi-layer fission chamber using the 235U samples as the neutron converters. The neutron energy spectrum from 0.1 eV to 30 MeV is obtained. The integral neutron flux (from 0.1 eV to 30 MeV) normalized to the proton beam power of 100 kW is 1.55×107 neutrons/cm2/s.

AMS Measurement of 237Np at CIAE

237Np (≃2.14 × 106 yr half-life) is potentially applicable in studies on nuclear safeguards and radioactive waste migration. The atomic ratio of 237Np/U in nature is 10−12 or even lower, depending strongly on the integral neutron flux received by the material. As an ultra-sensitive technique, accelerator mass spectrometry (AMS) is the best for measuring ultratrace 237Np. By extracting negative molecular ions NpO– from the oxide sample using 238UO– and 208Pb16O2– pilot beams for the simulation of 237Np ion transport, identifying the interference isotopes by high-resolution dedicated injector, electrostatic analyzer, and time of flight (TOF) detector, a method for AMS measurement of 237Np was set up on the HI-13 accelerator at the China Institute of Atomic Energy (CIAE). A sensitivity of <10–11 has been achieved for the isotopic ratio 237Np/238U.