coordination solids
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2020 ◽  
Vol 11 (1) ◽  
Author(s):  
Laura Voigt ◽  
Mariusz Kubus ◽  
Kasper S. Pedersen

Abstract Tessellation of self-assembling molecular building blocks is a promising strategy to design metal-organic materials exhibiting geometrical frustration and ensuing frustrated physical properties. Appearing in two-dimensional quasiperiodic phases, tilings consisting of five-vertex nodes are regarded as approximants for quasicrystals. Unfortunately, these structural motifs are exceedingly rare due to the complications of acquiring five-fold coordination confined to the plane. Lanthanide ions display the sufficient coordinative plasticity, and large ionic radii, to allow their incorporation into irregular molecule-based arrays. We herein present the use of ytterbium(II) as a five-vertex node in a two-dimensional coordination solid, YbI2(4,4′-bipyridine)2.5. The semi-regular Archimedean tessellation structure verges on quasicrystallinity and paves the way for lanthanide-based metal-organic materials with interesting photonic and magnetic properties.


2020 ◽  
Vol 289 ◽  
pp. 121479
Author(s):  
Renata Carolina Alves ◽  
Guilherme Nunes Lucena ◽  
Renan Lira de Farias ◽  
Patrícia Bento da Silva ◽  
Isabel Cristiane da Silva ◽  
...  

Polyhedron ◽  
2018 ◽  
Vol 151 ◽  
pp. 381-393 ◽  
Author(s):  
Debajit Dutta ◽  
Sanjib Chetry ◽  
Anshuman Gogoi ◽  
Bula Choudhury ◽  
Ankur K. Guha ◽  
...  

ChemMedChem ◽  
2017 ◽  
Vol 12 (21) ◽  
pp. 1739-1742 ◽  
Author(s):  
Dana J. Levine ◽  
Miguel I. Gonzalez ◽  
Christina M. Legendre ◽  
Tomče Runčevski ◽  
Julia Oktawiec ◽  
...  

2014 ◽  
Vol 126 (5) ◽  
pp. 1433-1442 ◽  
Author(s):  
VINEET KUMAR ◽  
ARITRA KUNDU ◽  
MONIKA SINGH ◽  
KANDALAM V RAMANUJACHARY ◽  
ARUNACHALAM RAMANAN

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