Self-consistent solution for the magnetic exchange interaction mediated by a superconductor

We theoretically determine the magnetic exchange interaction between two ferromagnets coupled by a superconductor using a tight-binding lattice model. The main purpose of this study is to determine how the self-consistently determined superconducting state influences the exchange interaction and the preferred ground-state of the system, including the role of impurity scattering. We find that the superconducting state eliminates RKKY-like oscillations for a sufficiently large superconducting gap, making the anti-parallel orientation the ground state of the system. Interestingly, the superconducting gap is larger in the parallel configuration than in the anti-parallel configuration, giving a larger superconducting condensation energy, even when the preferred ground state is anti-parallel. We also show that increasing the impurity concentration in the superconductor causes the exchange interaction to decrease, likely due to an increasing localization of the mediating quasiparticles in the superconductor.

Solvent-tuned magnetic exchange interactions in Dy2 systems ligated by a μ-phenolato heptadentate Schiff base

Solvent-tuning changes the magnetic exchange interaction and results in different magnetic relaxation dynamics in Dy2 systems ligated by a μ-phenolato heptadentate Schiff base.