Optical Detection of Magnetic Resonance (ODMR) Studies of the Electronic Structure of Complex Defects in GaP

1987 ◽  
Vol 104 ◽  
Author(s):  
W. M. Chen ◽  
M. Godlewski ◽  
B. Monemar ◽  
H. P. Gislason

ABSTRACTOptical detection of magnetic resonance (ODMR) is applied to studies of neutral (“isoelectronic”) complex defects in GaP, via monitoring recombination of the excited bound exciton (BE) state associated with these defects. With examples of isoelectronic complex defects in GaP associated with C, Cu, Li and the PGa -antisite, it is shown how the ODMR data reveal the magnetic properties of both electrons and holes bound at such defects. The procedures to conclude on defect symmetry, structure and identity are also elucidated.

1989 ◽  
Vol 163 ◽  
Author(s):  
W.M. Chen ◽  
A. Henry ◽  
E. Janzén ◽  
B. Monemar ◽  
M.L.W. Thewalt

AbstractWe report an investigation on the electronic structure of two bound exciton (BE) systems from a complex defect in S-doped Si, by optical detection of magnetic resonance (ODMR). A spin-triplet (S=1) is identified to be the lowest electronic state of the BE's, which gives rise to deep photoluminescence (PL) emissions when recombining. A weak anisotropy of the magnetic interaction of the BE’s (not possible to resolve in Zeeman data) is revealed, which leads directly to the determination of the symmetry for the excited state of the defect. A S-related complex model is suggested as the identity of the defect. A critical test of two possible metastable configurations of the constituents of a single defect is undertaken.


2021 ◽  
Vol 7 (7) ◽  
pp. 96
Author(s):  
Lucia Gigli ◽  
Silvia Di Grande ◽  
Enrico Ravera ◽  
Giacomo Parigi ◽  
Claudio Luchinat

Nuclear Magnetic Resonance is particularly sensitive to the electronic structure of matter and is thus a powerful tool to characterize in-depth the magnetic properties of a system. NMR is indeed increasingly recognized as an ideal tool to add precious structural information for the development of Single Ion Magnets, small complexes that are recently gaining much popularity due to their quantum computing and spintronics applications. In this review, we recall the theoretical principles of paramagnetic NMR, with particular attention to lanthanoids, and we give an overview of the recent advances in this field.


2021 ◽  
Vol 23 (10) ◽  
pp. 6171-6181
Author(s):  
Yaoqi Gao ◽  
Baozeng Zhou ◽  
Xiaocha Wang

It is found that the biaxial strain, electric field and interlayer distance can effectively modulate the electronic structure and magnetic properties of two-dimensional van der Waals heterostructures.


1995 ◽  
Vol 384 ◽  
Author(s):  
Zhi-Qiang Li ◽  
Yuichi Hashi ◽  
Jing-Zhi Yu ◽  
Kaoru Ohno ◽  
Yoshiyuki Kawazoe

ABSTRACTThe electronic structure and magnetic properties of rhodium clusters with sizes of 1 - 43 atoms embedded in the nickel host are studied by the first-principles spin-polarized calculations within the local density functional formalism. Single Rh atom in Ni matrix is found to have magnetic moment of 0.45μB. Rh13 and Rhl 9 clusters in Ni matrix have lower magnetic moments compared with the free ones. The most interesting finding is tha.t Rh43 cluster, which is bulk-like nonmagnetic in vacuum, becomes ferromagnetic when embedded in the nickel host.


2005 ◽  
Vol 367 (1-4) ◽  
pp. 61-71 ◽  
Author(s):  
Y. Yang ◽  
C. Jing ◽  
J.G. Yang ◽  
S.X. Cao ◽  
J.C. Zhang

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