scholarly journals ac Susceptometry of 2D van der Waals Magnets Enabled by the Coherent Control of Quantum Sensors

PRX Quantum ◽  
2021 ◽  
Vol 2 (3) ◽  
Author(s):  
Xin-Yue Zhang ◽  
Yu-Xuan Wang ◽  
Thomas A. Tartaglia ◽  
Thomas Ding ◽  
Mason J. Gray ◽  
...  
Nanoscale ◽  
2018 ◽  
Vol 10 (30) ◽  
pp. 14432-14440 ◽  
Author(s):  
Ruiqiang Guo ◽  
Young-Dahl Jho ◽  
Austin J. Minnich

Coherent manipulation of thermal phonon transport in vdW superlattices can expand the property space beyond that occupied by natural materials.


Nanoscale ◽  
2021 ◽  
Author(s):  
Tae Gwan Park ◽  
Hong Ryeol Na ◽  
Seung-Hyun Chun ◽  
Won Bae Cho ◽  
Sunghun Lee ◽  
...  

Interlayer vibrations with discrete quantized modes in two-dimensional (2D) materials can be excited by ultrafast light due to the inherent low dimensionality and van der Waals force as a restoring...


2018 ◽  
Vol 14 (2) ◽  
pp. 120-125 ◽  
Author(s):  
Joel I-Jan Wang ◽  
Daniel Rodan-Legrain ◽  
Landry Bretheau ◽  
Daniel L. Campbell ◽  
Bharath Kannan ◽  
...  

2022 ◽  
Vol 13 (1) ◽  
Author(s):  
Emre Ergeçen ◽  
Batyr Ilyas ◽  
Dan Mao ◽  
Hoi Chun Po ◽  
Mehmet Burak Yilmaz ◽  
...  

AbstractIn van der Waals (vdW) materials, strong coupling between different degrees of freedom can hybridize elementary excitations into bound states with mixed character1–3. Correctly identifying the nature and composition of these bound states is key to understanding their ground state properties and excitation spectra4,5. Here, we use ultrafast spectroscopy to reveal bound states of d-orbitals and phonons in 2D vdW antiferromagnet NiPS3. These bound states manifest themselves through equally spaced phonon replicas in frequency domain. These states are optically dark above the Néel temperature and become accessible with magnetic order. By launching this phonon and spectrally tracking its amplitude, we establish the electronic origin of bound states as localized d–d excitations. Our data directly yield electron-phonon coupling strength which exceeds the highest known value in 2D systems6. These results demonstrate NiPS3 as a platform to study strong interactions between spins, orbitals and lattice, and open pathways to coherent control of 2D magnets.


2021 ◽  
Vol 4 (1) ◽  
Author(s):  
Igor V. Bondarev ◽  
Oleg L. Berman ◽  
Roman Ya. Kezerashvili ◽  
Yurii E. Lozovik

AbstractThroughout the years, strongly correlated coherent states of excitons have been the subject of intense theoretical and experimental studies. This topic has recently boomed due to new emerging quantum materials such as van der Waals (vdW) bound atomically thin layers of transition metal dichalcogenides (TMDs). We analyze the collective properties of charged interlayer excitons observed recently in bilayer TMD heterostructures. We predict strongly correlated phases—crystal and Wigner crystal—that can be selectively realized with TMD bilayers of properly chosen electron-hole effective masses by just varying their interlayer separation distance. Our results can be used for nonlinear coherent control, charge transport and spinoptronics application development with quantum vdW heterostuctures.


1997 ◽  
Vol 91 (4) ◽  
pp. 689-696 ◽  
Author(s):  
HAI-BO QIAN ◽  
WOUTER HERREBOUT ◽  
BRIAN HOWARD

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