Mechanism of ultrafast spin-polarization switching in nanostructures

2019 ◽  
Vol 99 (11) ◽  
Author(s):  
V. N. Mantsevich ◽  
I. V. Rozhansky ◽  
N. S. Maslova ◽  
P. I. Arseyev ◽  
N. S. Averkiev ◽  
...  
2018 ◽  
Vol 10 (36) ◽  
pp. 30614-30622 ◽  
Author(s):  
Shiheng Liang ◽  
Zhongwei Yu ◽  
Xavier Devaux ◽  
Anthony Ferri ◽  
Weichuan Huang ◽  
...  

2001 ◽  
Vol 105 (15) ◽  
pp. 3741-3744 ◽  
Author(s):  
Tetsuo Okutsu ◽  
Masaki Ooyama ◽  
Katsuhiko Tani ◽  
Hiroshi Hiratsuka ◽  
Akio Kawai ◽  
...  

1980 ◽  
Vol 45 (6) ◽  
pp. 1669-1676 ◽  
Author(s):  
Pavel Kubáček

The first step of electrochemical oxidation of 2-phenyl- and 2-(4-tolyl)-1,3,4,7-tetramethylisoindoles in anhydrous acetonitrile produces relatively stable cationradicals which have been studied by means of EPR spectroscopy using the method of internal electrochemical generation of radicals under reduced temperature. The same electrochemical behaviour of the both studied derivatives and identical EPR spectra of their cationradicals can be explained within the Huckel MO method. The largest contribution to the magnitude of splitting constant of nitrogen nucleus is due to π-σ-spin polarization of C-N bonds caused by high spin abundance of pz-AO of carbon atoms. Half-life of decomposition of the studied cationradicals is 4 min at -30°C.


Author(s):  
M. M. Glazov

The transfer of nonequilibrium spin polarization between the electron and nuclear subsystems is studied in detail. Usually, a thermal orientation of nuclei in magnetic field is negligible due to their small magnetic moments, but if electron spins are optically oriented, efficient nuclear spin polarization can occur. The microscopic approach to the dynamical nuclear polarization effect based on the kinetic equation method, along with a phenomenological but very powerful description of dynamical nuclear polarization in terms of the nuclear spin temperature concept is given. In this way, one can account for the interaction between neighbouring nuclei without solving a complex many-body problem. The hyperfine interaction also induces the feedback of polarized nuclei on the electron spin system giving rise to a number of nonlinear effects: bistability of nuclear spin polarization and anomalous Hanle effect, dragging and locking of optical resonances in quantum dots. Theory is illustrated by experimental data on dynamical nuclear polarization.


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