scholarly journals Non-Markovianity: initial correlations and nonlinear optical measurements

Author(s):  
Arend G. Dijkstra ◽  
Yoshitaka Tanimura

By extending the response function approach developed in nonlinear optics, we analytically derive an expression for the non-Markovianity in the time evolution of a system in contact with a quantum mechanical bath, and find a close connection with the directly observable nonlinear optical response. The result indicates that memory in the bath-induced fluctuations rather than in the dissipation causes non-Markovianity. Initial correlations between states of the system and the bath are shown to be essential for a correct understanding of the non-Markovianity. These correlations are included in our treatment through a preparation function.

APL Photonics ◽  
2018 ◽  
Vol 3 (1) ◽  
pp. 016102 ◽  
Author(s):  
Hanying Deng ◽  
David Zs. Manrique ◽  
Xianfeng Chen ◽  
Nicolae C. Panoiu ◽  
Fangwei Ye

2001 ◽  
Vol 709 ◽  
Author(s):  
Kenji Kiyohara ◽  
Koji Ohta ◽  
Yo Shimizu

ABSTRACTWe investigated the third-order nonlinear optical response of a Gay-Berne system at the isotropic, nematic, and smectic phases by molecular dynamics simulation. The components of the optical response were calculated for the three different axes with respect to the director of the system, separately. In the nematic phase, in particular, we observed that the response function does not vanish at long times. This means that the orientation of the director of the system is permanently changed by an instant irradiation of polarized light, as a result of third-order nonlinear optical response. In the smectic phase, however, all the components of the response function decay quickly. Our results give a theoretical background at molecular level on the interpretation of the reported experimental observations of peculiar dynamics of liquid crystalline systems at irradiation of laser lights.


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