Three Pulse Photon Echo Peak Shift Study of the B800 Band of the LH2 Complex ofRps.acidophilaat Room Temperature:  A Coupled Master Equation and Nonlinear Optical Response Function Approach

2001 ◽  
Vol 105 (9) ◽  
pp. 1887-1894 ◽  
Author(s):  
Ritesh Agarwal ◽  
Mino Yang ◽  
Qing-Hua Xu ◽  
Graham R. Fleming
ACS Photonics ◽  
2021 ◽  
Vol 8 (2) ◽  
pp. 550-556
Author(s):  
Javier Hernandez-Rueda ◽  
Marc L. Noordam ◽  
Irina Komen ◽  
L. Kuipers

Author(s):  
Arend G. Dijkstra ◽  
Yoshitaka Tanimura

By extending the response function approach developed in nonlinear optics, we analytically derive an expression for the non-Markovianity in the time evolution of a system in contact with a quantum mechanical bath, and find a close connection with the directly observable nonlinear optical response. The result indicates that memory in the bath-induced fluctuations rather than in the dissipation causes non-Markovianity. Initial correlations between states of the system and the bath are shown to be essential for a correct understanding of the non-Markovianity. These correlations are included in our treatment through a preparation function.


2012 ◽  
Vol 500 ◽  
pp. 62-65
Author(s):  
Yee Sin Ang ◽  
Chao Zhang

We demonstrate that bilayer graphene exhibits strong nonlinear optical response in the terahertz frequency regime. The electric field strength required to generate single-frequency and triple-frequency nonlinear optical responses comparable to the linear optical response is only moderate and can be easily achieved in laboratory. This strong nonlinear optical response persists even in room temperature. This suggests that bilayer graphene can potentially be utilized in nonlinear terahertz photonics.


2001 ◽  
Vol 709 ◽  
Author(s):  
Kenji Kiyohara ◽  
Koji Ohta ◽  
Yo Shimizu

ABSTRACTWe investigated the third-order nonlinear optical response of a Gay-Berne system at the isotropic, nematic, and smectic phases by molecular dynamics simulation. The components of the optical response were calculated for the three different axes with respect to the director of the system, separately. In the nematic phase, in particular, we observed that the response function does not vanish at long times. This means that the orientation of the director of the system is permanently changed by an instant irradiation of polarized light, as a result of third-order nonlinear optical response. In the smectic phase, however, all the components of the response function decay quickly. Our results give a theoretical background at molecular level on the interpretation of the reported experimental observations of peculiar dynamics of liquid crystalline systems at irradiation of laser lights.


2002 ◽  
Vol 106 (33) ◽  
pp. 7573-7578 ◽  
Author(s):  
Ritesh Agarwal ◽  
Abbas H. Rizvi ◽  
Bradley S. Prall ◽  
John D. Olsen ◽  
C. Neil Hunter ◽  
...  

2021 ◽  
Vol 64 (9) ◽  
Author(s):  
MengYu Zong ◽  
YuQian Zu ◽  
Jia Guo ◽  
Zhen Zhang ◽  
JingJing Liu ◽  
...  

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