Femtosecond time-resolved charged particle imaging studies of the ultraviolet photodissociation of the NO dimer

2003 ◽  
Vol 119 (22) ◽  
pp. 11728-11739 ◽  
Author(s):  
Masaaki Tsubouchi ◽  
Cornelis A. de Lange ◽  
Toshinori Suzuki
2018 ◽  
Vol 8 (8) ◽  
pp. 1227 ◽  
Author(s):  
Vincent Loriot ◽  
Luis Bañares ◽  
Rebeca de Nalda

We present a tutorial to realize a multidimensional fitting procedure capable of extracting all the relevant information contained in a sequence of charged particle images acquired as a function of time in femtosecond pump–probe experiments. The images are reproduced using a 3D fitting method, which provides the velocity (or center-of-mass kinetic energy) and angular distributions contained in the images and their time evolution. A detailed example of the method is shown through the analysis of the time-resolved predissociation dynamics of CH3I on the B-band origin (Gitzinger et al., J. Chem. Phys.2010, 133, 234313). We show that the multidimensional approach is essential for the analysis of complex images that contain several overlapping contributions where reduced dimensionality analyses cannot provide a reliable description of the features present in the image sequence. This methodology can be generalized to many types of multidimensional data analysis.


Author(s):  
Vincent Loriot ◽  
Luis Bañares ◽  
Rebeca de Nalda

We present a tutorial to realize a multidimensional fitting procedure capable of extracting all the relevant information contained in a sequence of charged particle images acquired as a function of time in femtosecond pump-probe experiments. The images are reproduced using a 3D fitting method, which provides the velocity (or center-of-mass kinetic energy) and angular distributions contained in the images and their time evolution. A detailed example of the method is shown through the analysis of the time-resolved predissociation dynamics of CH3I on the B-band origin [Gitzinger et al., J. Chem. Phys. 133, 234313 (2010)]. We show that the multidimensional approach is essential for the analysis of complex images that contain several overlapping contributions where reduced dimensionality analyses cannot provide a reliable description of the features present in the image sequence. This methodology can be generalized to many types of multidimensional data analysis.


2008 ◽  
Vol 50 (2-6) ◽  
pp. 606-610 ◽  
Author(s):  
S. Nishinomiya ◽  
K. Katagiri ◽  
T. Niinou ◽  
J. Kaneko ◽  
H. Fukuda ◽  
...  

2008 ◽  
Author(s):  
Ludovic Rapp ◽  
Christophe Cibert ◽  
Anne Patricia Alloncle ◽  
Philippe Delaporte ◽  
Sebastien Nenon ◽  
...  

2009 ◽  
Author(s):  
X. L. Zhang ◽  
R. S. Fletcher ◽  
S. L. Rolston ◽  
James R. Danielson ◽  
Thomas Sunn Pedersen

Author(s):  
Ingo Fischer ◽  
Stephen T Pratt

Photoelectron spectroscopy has long been a powerful method in the toolbox of experimental physical chemistry and molecular physics. Recent improvements in coincidence methods, charged-particle imaging, and electron energy resolution have...


2002 ◽  
Vol 29 (11) ◽  
pp. 2529-2540 ◽  
Author(s):  
Martin P. Tornai ◽  
Bradley E. Patt ◽  
Jan S. Iwanczyk ◽  
Carolyn R. Tull ◽  
Lawrence R. MacDonald ◽  
...  

2009 ◽  
Vol 56 (5) ◽  
pp. 2628-2635 ◽  
Author(s):  
Liying Chen ◽  
Lisa S. Gobar ◽  
Negar G. Knowles ◽  
Donald W. Wilson ◽  
Harrison H. Barrett

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