Exploiting two-dimensional hybrid perovskites incorporating secondary amines for high-performance array photodetection

2020 ◽  
Vol 8 (37) ◽  
pp. 12848-12853
Author(s):  
Tao Yang ◽  
Yaobin Li ◽  
Shiguo Han ◽  
Yi Liu ◽  
Zhiyun Xu ◽  
...  

We present a new 2D hybrid perovskite by alloying secondary dimethylammonium cation as the “perovskiter” into the PbI3 framework, which shows the strong in-plane photoresponses.

Author(s):  
Yu Ma ◽  
Jiaqi Wang ◽  
Yi Liu ◽  
Shiguo Han ◽  
Yaobin Li ◽  
...  

Self-powered photodetection with an extremely low detection limit of 82 nW cm−2 is achieved in a 2D hybrid perovskite ferroelectric. This result sheds light on future advances of ferroelectrics toward smart optoelectronic device applications.


2020 ◽  
Vol 8 (4) ◽  
pp. 1875-1886 ◽  
Author(s):  
Ambra Pisanu ◽  
Mauro Coduri ◽  
Marta Morana ◽  
Yasemin O. Ciftci ◽  
Aurora Rizzo ◽  
...  

The role of halide substitution in a lead-free 2D hybrid perovskite is studied on the BZA2SnX4 (BZA = benzylammonium; X = Cl, Br, I) system, by reporting the two novel compositions BZA2SnBr4 and BZA2SnCl4.


2019 ◽  
Vol 7 (14) ◽  
pp. 4004-4012 ◽  
Author(s):  
Fan Zhang ◽  
Huaye Zhang ◽  
Lijie Zhu ◽  
Liang Qin ◽  
Yue Wang ◽  
...  

High-performance bottom-gate 2D-layered (PEA)2SnI4 field-effect transistors have been fabricated using PVA/CL-PVP as gate dielectric layers.


2018 ◽  
Vol 6 (15) ◽  
pp. 3945-3950 ◽  
Author(s):  
Lijie Zhu ◽  
Huaye Zhang ◽  
Qipeng Lu ◽  
Yue Wang ◽  
Zhenbo Deng ◽  
...  

The (PEA)2PbX4(PEA = C8H9NH3, X = Cl, Br, I) nanosheets: P3HT composite films were prepared as channel layers for high performance field-effect transistors.


2019 ◽  
Vol 75 (3) ◽  
pp. 354-358 ◽  
Author(s):  
Ling Cheng ◽  
Yingjie Cao

Recently, with the prevalence of `perovskite fever', organic–inorganic hybrid perovskites (OHPs) have attracted intense attention due to their remarkable structural variability and highly tunable properties. In particular, the optical and electrical properties of organic–inorganic hybrid lead halides are typical of the OHP family. Besides, although three-dimensional hybrid perovskites, such as [CH3NH3]PbX 3 (X = Cl, Br or I), have been reported, the development of new organic–inorganic hybrid semiconductors is still an area in urgent need of exploration. Here, an organic–inorganic hybrid lead halide perovskite is reported, namely poly[(2-azaniumylethyl)trimethylphosphanium [tetra-μ-bromido-plumbate(II)]], {(C5H16NP)[PbBr4]} n , in which an organic cation is embedded in inorganic two-dimensional (2D) mesh layers to produce a sandwich structure. This unique sandwich 2D hybrid perovskite material shows an indirect band gap of ∼2.700 eV. The properties of this compound as a semiconductor are demonstrated by a series of optical characterizations and indicate potential applications for optical devices.


Author(s):  
beibei wang ◽  
Huaixi Chen ◽  
Wuqian Guo ◽  
Yi Liu ◽  
Shiguo Han ◽  
...  

Two-dimensional (2D) Ruddlesden-Popper hybrid perovskites (RPHPs) have shown enormous potentials for photoelectric applications, owing to their advantages of structural diversity and unique physical properties. Despite extensive studies, the cage-incorporation of...


2017 ◽  
Author(s):  
Varun Bheemireddy

The two-dimensional(2D) materials are highly promising candidates to realise elegant and e cient transistor. In the present letter, we conjecture a novel co-planar metal-insulator-semiconductor(MIS) device(capacitor) completely based on lateral 2D materials architecture and perform numerical study of the capacitor with a particular emphasis on its di erences with the conventional 3D MIS electrostatics. The space-charge density features a long charge-tail extending into the bulk of the semiconductor as opposed to the rapid decay in 3D capacitor. Equivalently, total space-charge and semiconductor capacitance densities are atleast an order of magnitude more in 2D semiconductor. In contrast to the bulk capacitor, expansion of maximum depletion width in 2D semiconductor is observed with increasing doping concentration due to lower electrostatic screening. The heuristic approach of performance analysis(2D vs 3D) for digital-logic transistor suggest higher ON-OFF current ratio in the long-channel limit even without third dimension and considerable room to maximise the performance of short-channel transistor. The present results could potentially trigger the exploration of new family of co-planar at transistors that could play a signi significant role in the future low-power and/or high performance electronics.<br>


Nanophotonics ◽  
2020 ◽  
Vol 9 (16) ◽  
pp. 4719-4728
Author(s):  
Tao Deng ◽  
Shasha Li ◽  
Yuning Li ◽  
Yang Zhang ◽  
Jingye Sun ◽  
...  

AbstractThe molybdenum disulfide (MoS2)-based photodetectors are facing two challenges: the insensitivity to polarized light and the low photoresponsivity. Herein, three-dimensional (3D) field-effect transistors (FETs) based on monolayer MoS2 were fabricated by applying a self–rolled-up technique. The unique microtubular structure makes 3D MoS2 FETs become polarization sensitive. Moreover, the microtubular structure not only offers a natural resonant microcavity to enhance the optical field inside but also increases the light-MoS2 interaction area, resulting in a higher photoresponsivity. Photoresponsivities as high as 23.8 and 2.9 A/W at 395 and 660 nm, respectively, and a comparable polarization ratio of 1.64 were obtained. The fabrication technique of the 3D MoS2 FET could be transferred to other two-dimensional materials, which is very promising for high-performance polarization-sensitive optical and optoelectronic applications.


2021 ◽  
Author(s):  
Lixiang Han ◽  
Mengmeng Yang ◽  
Peiting Wen ◽  
Wei Gao ◽  
nengjie huo ◽  
...  

One dimensional (1D)-two dimensional (2D) van der Waals (vdWs) mixed-dimensional heterostructures with advantages of atomically sharp interface, high quality and good compatibility have attracted tremendous attention in recent years. The...


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