Charge transport in a two-dimensional hybrid metal halide thiocyanate compound

2017 ◽  
Vol 5 (24) ◽  
pp. 5930-5938 ◽  
Author(s):  
John G. Labram ◽  
Naveen R. Venkatesan ◽  
Christopher J. Takacs ◽  
Hayden A. Evans ◽  
Erin E. Perry ◽  
...  

Time-resolved microwave conductivity reveals good carrier mobility and long carrier lifetimes in the layered organic metal halide compound (CH3NH3)2Pb(SCN)2I2.

2020 ◽  
Vol 8 (31) ◽  
pp. 10761-10766
Author(s):  
Shirsopratim Chattopadhyay ◽  
Robert S. Kokenyesi ◽  
Min Ji Hong ◽  
C Lowell Watts ◽  
John G. Labram

A strategy is demonstrated to evaluate the carrier mobility in-plane and out-of-plane using contactless time resolved microwave conductivity.


2015 ◽  
Vol 6 (32) ◽  
pp. 5860-5868 ◽  
Author(s):  
Takahiro Fukumatsu ◽  
Akinori Saeki ◽  
Shu Seki

Non-contact measurements with time-resolved microwave conductivity and absorption spectroscopy offer direct access to the charge carrier mobility in conjugated backbones.


Author(s):  
Fan Zhang ◽  
Quan Zhang ◽  
Xin Liu ◽  
Liang Qin ◽  
Yufeng Hu ◽  
...  

Two-dimensional layered Sn-based perovskites with superior carrier mobility and excellent compatibility with the horizontal charge transport in field-effect transistors are promising channel materials. However, ambipolar characteristics cannot be achieved and...


2016 ◽  
Vol 45 (1) ◽  
pp. 118-151 ◽  
Author(s):  
Song-Lin Li ◽  
Kazuhito Tsukagoshi ◽  
Emanuele Orgiu ◽  
Paolo Samorì

This review presents recent progress on charge transport properties, carrier scattering mechanisms, and carrier mobility engineering of two-dimensional transition metal chalcogenides.


2019 ◽  
Vol 48 (37) ◽  
pp. 14019-14026 ◽  
Author(s):  
Naveen R. Venkatesan ◽  
Ali Mahdi ◽  
Brian Barraza ◽  
Guang Wu ◽  
Michael L. Chabinyc ◽  
...  

Two hybrid halide Ruddlesden–Popper compounds using the cation 2-(4-biphenyl)ethylammonium show higher yield-carrier mobility products by time-resolved microwave conductivity than compounds with n-butylammonium cations.


2019 ◽  
Vol 5 (5) ◽  
pp. eaaw5558 ◽  
Author(s):  
Yang Lan ◽  
Benjamin J. Dringoli ◽  
David A. Valverde-Chávez ◽  
Carlito S. Ponseca ◽  
Mark Sutton ◽  
...  

Hybrid organic-inorganic halide perovskites have shown remarkable optoelectronic properties, exhibiting an impressive tolerance to defects believed to originate from correlated motion of charge carriers and the polar lattice forming large polarons. Few experimental techniques are capable of directly probing these correlations, requiring simultaneous sub–millielectron volt energy and femtosecond temporal resolution after absorption of a photon. Here, we use time-resolved multi-THz spectroscopy, sensitive to the internal excitations of the polaron, to temporally and energetically resolve the coherent coupling of charges to longitudinal optical phonons in single-crystal CH3NH3PbI3 (MAPI). We observe room temperature intraband quantum beats arising from the coherent displacement of charge from the coupled phonon cloud. Our measurements provide strong evidence for the existence of polarons in MAPI at room temperature, suggesting that electron/hole-phonon coupling is a defining aspect of the hybrid metal-halide perovskites contributing to the protection from scattering and enhanced carrier lifetimes that define their usefulness in devices.


2021 ◽  
Author(s):  
Ying Li ◽  
Zhifeng Shi ◽  
Wenqing Liang ◽  
Jingli Ma ◽  
Xu Chen ◽  
...  

Recently, metal-halide perovskites have emerged as promising materials for photodetectors (PDs) applications owing to their superior optoelectronic properties, such as ambipolar charge transport characteristics, high carrier mobility, and so on....


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