Monolithic tandem solar cells comprising electrodeposited CuInSe2 and perovskite solar cells with a nanoparticulate ZnO buffer layer

2017 ◽  
Vol 5 (36) ◽  
pp. 19439-19446 ◽  
Author(s):  
Yoon Hee Jang ◽  
Jang Mi Lee ◽  
Jung Woo Seo ◽  
Inho Kim ◽  
Doh-Kwon Lee

Monolithically integrated, 2-terminal CuInSe2–perovskite tandem solar cells are successfully fabricated using low-cost solution processes, demonstrating higher efficiency than the constituent single-junction devices.

2021 ◽  
Vol 38 (10) ◽  
pp. 107801
Author(s):  
Zihan Qu ◽  
Fei Ma ◽  
Yang Zhao ◽  
Xinbo Chu ◽  
Shiqi Yu ◽  
...  

In the last decade, perovskite solar cells (PSCs) have greatly drawn researchers’ attention, with the power conversion efficiency surging from 3.8% to 25.5%. PSCs possess the merits of low cost, simple fabrication process and high performance, which could be one of the most promising photovoltaic technologies in the future. In this review, we focus on the summary of the updated progresses in single junction PSCs including efficiency, stability and large area module. Then, the important progresses in tandem solar cells are briefly discussed. A prospect into the future of the field is also included.


Author(s):  
Erkan Aydin ◽  
Jiang Liu ◽  
Esma Ugur ◽  
RANDI AZMI ◽  
George T Harrison ◽  
...  

Translating the high power conversion efficiencies of single-junction perovskite solar cells in their classic, non-inverted (n-i-p) architecture to efficient monolithic n-i-p perovskite/silicon tandem solar cells with high current densities has...


Author(s):  
Paulo Ernesto Marchezi ◽  
Francineide Lopes de Araújo ◽  
Rodrigo Szostak ◽  
José Carlos Germino ◽  
Eralci Moreira Terézio ◽  
...  

Mixed halide perovskites of the type CsxFA1-xPb(BryI1-y)3 are promising materials for highly efficient single junction and tandem solar cells. This work details how RGO interacts with the perovskite, influencing film...


Polymers ◽  
2020 ◽  
Vol 12 (1) ◽  
pp. 145 ◽  
Author(s):  
Lin Hu ◽  
Jiaxing Song ◽  
Xinxing Yin ◽  
Zhen Su ◽  
Zaifang Li

Solution-processed polymer solar cells (PSCs) have attracted dramatically increasing attention over the past few decades owing to their advantages of low cost, solution processability, light weight, and excellent flexibility. Recent progress in materials synthesis and devices engineering has boosted the power conversion efficiency (PCE) of single-junction PSCs over 17%. As an emerging technology, it is still a challenge to prepare solution-processed flexible electrodes for attractive flexible PSCs. Poly(3,4-ethylenedioxythiophene): poly(styrenesulfonate) (PEDOT:PSS) is one of the most promising candidates for electrodes due to its high conductivity (>4000 S/cm), excellent transmittance (>90%), intrinsically high work function (WF > 5.0 eV), and aqueous solution processability. To date, a great number of single-junction PSCs based on PEDOT:PSS electrodes have realized a PCE over 12%. In this review, we introduce the current research on the conductive complex PEDOT:PSS as well as trace the development of PEDOT:PSS used in electrodes for high performance PSCs and perovskite solar cells. We also discuss and comment on the aspects of conductivity, transmittance, work-function adjustment, film preparing methods, and device fabrications. A perspective on the challenges and future directions in this field is be offered finally.


2016 ◽  
Vol 1 (4) ◽  
pp. 370-376 ◽  
Author(s):  
T. Todorov ◽  
O. Gunawan ◽  
S. Guha

For decades, the appealing potential of tandem solar cells for efficiencies beyond the single-junction Shockley–Queisser limit has led researchers to develop thin film tandem solutions for high performance low cost solar cells.


MRS Advances ◽  
2018 ◽  
Vol 3 (52) ◽  
pp. 3111-3119 ◽  
Author(s):  
Ramez H. Ahangharnejhad ◽  
Zhaoning Song ◽  
Adam B. Phillips ◽  
Suneth C. Watthage ◽  
Zahrah S. Almutawah ◽  
...  

Abstract:Monolithic integrated thin film tandem solar cells consisting of a high bandgap perovskite top cell and a low bandgap thin film bottom cell are expected to reach higher power conversion efficiencies (PCEs) with lower manufacturing cost and environmental impacts than the market-dominant crystalline silicon photovoltaics. There have been several demonstrations of 4-terminal and 2-terminal perovskite tandem devices with CuInGaSe2 (CIGS) or CuInSe2 (CIS) and, similar to the other tandem structures, the optimization of this device relies on optimal choice for the perovskite bandgap and thickness. Therefore, further advancement will be enabled by tuning the perovskite absorber to maximize the photocurrent limited by the current match condition. Here, we systematically study the optical absorption and transmission of perovskite thin films with varying absorber band gap. Based on these results, we model the photocurrent generations in both perovskite and CIS subcells and estimate the performances of projected tandem devices by considering the ideally functioning perovskite and CIS device. Our results show that for perovskite layers with 500 nm thickness the optimal bandgap is around 1.6 eV. With these configurations, PCEs above 20% could be achieved by monolithically integrated perovskite/CIS tandem solar cells. Also by modelling the absorption at every layer we calculate the quantum efficiency at each subcell in addition to tracking optical losses.


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