orientational averaging
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scholarly journals Efficient orientational averaging of nonlinear optical signals in multi-chromophore systems

2017 ◽  
Vol 147 (4) ◽  
pp. 044114 ◽  
Author(s):  
Maxim F. Gelin ◽  
Raffaele Borrelli ◽  
Wolfgang Domcke
Keyword(s):  
Nonlinear Optical ◽  
Optical Signals ◽  
Orientational Averaging

Time-resolved stimulated emission depletion in two-photon excited states

2003 ◽  
Vol 31 (5) ◽  
pp. 1047-1051 ◽  
Author(s):  
A.J. Bain ◽  
R.J. Marsh ◽  
D.A. Armoogum ◽  
O. Mongin ◽  
L. Porrès ◽  
...  
Keyword(s):  
Fluorescence Spectroscopy ◽  
Excited States ◽  
Stimulated Emission ◽  
Molecular Probe ◽  
Time Resolved Fluorescence ◽  
Time Resolved ◽  
New Approach ◽  
Two Photon ◽  
Orientational Averaging ◽  
Stimulated Emission Depletion

A new approach to time-resolved fluorescence spectroscopy based on stimulated emission depletion (STED) of two-photon excited states is presented. Combined with time-resolved detection, STED can circumvent orientational averaging constraints and spontaneous emission selection rules inherent in all conventional techniques. Applications of STED to the study of molecular probe dynamics are presented, together with studies of STED dynamics in a new push–push two-photon chromophore.

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