Aerosol Atmospheric Rivers: Climatology, Event Characteristics, and Detection Algorithm Sensitivities

Leveraging the concept of atmospheric rivers (ARs), a detection technique based on a widely utilized global algorithm to detect ARs (Guan et al., 2018; Guan and Waliser, 2015, 2019) was recently developed to detect aerosol atmospheric rivers (AARs) using the Modern-Era Retrospective analysis for Research and Applications, Version 2 reanalysis (Chakraborty et al., 2021a). The current study further characterizes and quantifies various details of AARs that were not provided in that study, such as AARs’ seasonality, event characteristics, vertical profiles of aerosol mass mixing ratio and wind speed, and the fraction of total annual aerosol transport conducted by AARs. Analysis is also performed to quantify the sensitivity of AAR detection to the criteria and thresholds used by the algorithm. AARs occur more frequently over, and typically extend from, regions with higher aerosol emission. For a number of planetary-scale pathways that exhibit large climatological aerosol transport, AARs contribute 40–80 % to the total annual transport. DU AARs are more frequent in boreal spring, SS AARs are often more frequent during the boreal winter (summer) in the Northern (Southern) Hemisphere, CA AARs are more frequent during dry seasons and often originate from the global rainforests and industrial areas, and SU AARs are present in the Northern Hemisphere during all seasons. For most aerosol types, the mass mixing ratio within AARs is highest near the surface and decreases monotonically with altitude. However, DU and CA AARs over or near the African continent exhibit peaks in their aerosol mixing ratio profiles around 700 hPa. AAR event characteristics are mostly independent of species with mean length, width, and length/width ratio around 4000 km, 600 km, and 8, respectively.

The transport of bioaerosols observed by wideband integrated bioaerosol sensor and coherent Doppler lidar

Bioaerosols are usually defined as aerosols derived from biological systems such as bacteria, fungi, and viruses. They play an important role in atmospheric physical and chemical processes including ice nucleation and cloud condensation. As such, their dispersion affects not only public health but regional climate as well. Lidar is an effective technique for aerosol detection and pollution monitoring. It is also used to profile the vertical distribution of wind vectors. In this paper, a coherent Doppler wind lidar (CDWL) was deployed for wind and aerosol detection in Hefei, China, from 11 to 20 March in 2020. A wideband integrated bioaerosol sensor (WIBS) was deployed to monitor variations in local fluorescent bioaerosol levels. During observation, three aerosol transport events were captured. The WIBS data show that during these transport events, several types of fluorescent aerosol particles exhibit abnormal increases in either their concentration, number fractions to total particles, or number fractions to whole fluorescent aerosols. These increases are attributed to transported external fluorescent bioaerosols instead of local bioaerosols. Based on the Hybrid Single Particle Lagrangian Integrated Trajectory (HYSPLIT) backward trajectory model and the characteristics of external aerosols in WIBS, their possible sources, transport paths, and components are discussed. This work proves the influence of external aerosol transport on local high particulate matter (PM) pollution and fluorescent aerosol particle composition. The combination of WIBS and CDWL expands the aerosol monitoring parameters and proves to be a potential method for the real-time monitoring of fluorescent biological aerosol transport events. It contributes to the further understanding of bioaerosol transport.

Study of Planetary Boundary Layer and Aerosol Transport Using Ceilometer and Air Quality Modelling in New South Wales (NSW), Australia

The planetary boundary layer height (PBLH) is one of the key factors in influencing the dispersion of the air pollutants in the troposphere and hence the air pollutant concentration on ground level. For this reason, accurate air pollutant concentration depends on the performance of PBLH prediction. Recently, ceilometer, a lidar instrument to measure cloud base height, has been used by atmospheric scientists and air pollution control authorities to determine the mixing level height (MLH) in improving forecasting and understanding the evolution of aerosol layers above ground at a site. In this study, ceilometer data at an urban (Lidcombe) and a rural (Merriwa) location in the New South Wales, Australia was used to validate the PBLH prediction from two air quality models (CCAM-CTM and WRF-CMAQ) as well as to understand the aerosol transport from sources to receptor point at Merriwa for the three case studies where high PM10 concentration was detected in each of the three days. The results show that the PBLH prediction by the two air quality models corresponds reasonably well with observed ceilometer data and the cause and source of high PM10 concentration at Merriwa can be found by using ceilometer MLH data to corroborate with back trajectory analysis of transport of aerosols to the receptor point at Merriwa. Of the three case studies, one had aerosol source from north and north west of Merriwa in remote NSW where windblown dust is the main source, and the other two had sources from south and south east of Merriwa where anthropogenic sources dominate,

Aerosol transport pathways and source attribution in China during the COVID-19 outbreak

Due to the coronavirus disease 2019 (COVID-19) pandemic, human activities and industrial productions were strictly restricted during January–March 2020 in China. Despite the fact that anthropogenic aerosol emissions largely decreased, haze events still occurred. Characterization of aerosol transport pathways and attribution of aerosol sources from specific regions are beneficial to air quality and pandemic control strategies. This study establishes source–receptor relationships in various regions covering all of China during the COVID-19 outbreak based on the Community Atmosphere Model version 5 with Explicit Aerosol Source Tagging (CAM5-EAST). Our analysis shows that PM2.5 burden over the North China Plain between 30 January and 19 February is mostly contributed by local emissions (40 %–66 %). For other regions in China, PM2.5 burden is largely contributed from nonlocal sources. During the most polluted days of the COVID-19 outbreak, local emissions within the North China Plain and eastern China contributed 66 % and 87 % to the increase in surface PM2.5 concentrations, respectively. This is associated with the anomalous mid-tropospheric high pressure at the location of the climatological East Asia trough and the consequently weakened winds in the lower troposphere, leading to the local aerosol accumulation. The emissions outside China, especially those from South Asia and Southeast Asia, contribute over 50 % to the increase in PM2.5 concentration in southwestern China through transboundary transport during the most polluted day. As the reduction in emissions in the near future is desirable, aerosols from long-range transport and unfavorable meteorological conditions are increasingly important to regional air quality and need to be taken into account in clean-air plans.

Polydisperse Aerosol Transport and Deposition in Upper Airways of Age-Specific Lung

A comprehensive understanding of airflow characteristics and particle transport in the human lung can be useful in modelling to inform clinical diagnosis, treatment, and management, including prescription medication and risk assessment for rehabilitation. One of the difficulties in clinical treatment of lung disorders lies in the patients’ variable physical lung characteristics caused by age, amongst other factors, such as different lung sizes. A precise understanding of the comparison between different age groups with various flow rates is missing in the literature, and this study aims to analyse the airflow and aerosol transport within the age-specific lung. ANSYS Fluent solver and the large-eddy simulation (LES) model were employed for the numerical simulation. The numerical model was validated with the available literature and the computational results showed airway size-reduction significantly affected airflow and particle transport in the upper airways. This study reports higher deposition at the mouth-throat region for larger diameter particles. The overall deposition efficiency (DE) increased with airway size reduction and flow rate. Lung aging effected the pressure distribution and a higher pressure drop was reported for the aged lung as compared to the younger lung. These findings could inform medical management through individualised simulation of drug-aerosol delivery processes for the patient-specific lung.

Aerosol transport pathways and source attribution in China during the COVID-19 outbreak

Due to the coronavirus disease 2019 (COVID-19) pandemic, human activities and industrial productions were strictly restricted during January–March 2020 in China. Despite the fact that anthropogenic aerosol emissions largely decreased, haze events still occurred. Characterization of aerosol transport pathways and attribution of aerosol sources from specific regions are beneficial to the air quality and pandemic control strategies. This study establishes source-receptor relationships in various regions of China during the COVID-19 outbreak based on the Community Atmosphere Model version 5 with Explicit Aerosol Source Tagging (CAM5-EAST). Our analysis shows that PM2.5 burden over the North China Plain between January 30 and February 19 is largely contributed by local emissions (40–66 %). For other regions in China, PM2.5 burden is largely contributed from non-local sources. During the polluted days of COVID-19 outbreak, local emissions within North China Plain and Eastern China, respectively, contribute 66 % and 87 % to the increase in surface PM2.5 concentrations. This is associated with the anomalous mid-tropospheric high pressure at the location of climatological East Asia trough and the consequently weakened winds in the lower troposphere, leading to the local aerosol accumulation. The emissions outside China, especially from South and Southeast Asia, contribute over 50 % to the increase in PM2.5 concentration in Southwestern China through transboundary transport during the polluted day. As the reduction in emissions in the near future, aerosols from long-range transport together with unfavorable meteorological conditions are increasingly important to regional air quality and need to be taken into account in clean air plans.