Application of cylindrical IE-GSTC to physical metasurfaces

<div>This work validates cylindrical IE-GSTC by applying it to physical metasurfaces, i.e. metasurfaces defined by material properties and dimensions rather than by susceptibility tensor components. Previously reported IE-GSTC which was formulated for zero thickness GSTC discontinuity is extended to handle finite thickness of physical metasurfaces. A simple analytical approach is used to extract the bianisotropic susceptibility tensor of concentric, multilayered, magneto-dielectric shell. Plane wave scattering by a physical metasurface constructed of four segments of multilayered, magneto-dielectric metasurface scatterers is used as an example problem to validate cylindrical IEGSTC. A second example considers an opening on the cylindrical metasurface, confirming IE-GSTC can handle metasurfaces with openings. Good agreement is obtained between IE-GSTC results and full wave simulation results for both cases.</div>

Application of cylindrical IE-GSTC to physical metasurfaces

<div>This work validates cylindrical IE-GSTC by applying it to physical metasurfaces, i.e. metasurfaces defined by material properties and dimensions rather than by susceptibility tensor components. Previously reported IE-GSTC which was formulated for zero thickness GSTC discontinuity is extended to handle finite thickness of physical metasurfaces. A simple analytical approach is used to extract the bianisotropic susceptibility tensor of concentric, multilayered, magneto-dielectric shell. Plane wave scattering by a physical metasurface constructed of four segments of multilayered, magneto-dielectric metasurface scatterers is used as an example problem to validate cylindrical IEGSTC. A second example considers an opening on the cylindrical metasurface, confirming IE-GSTC can handle metasurfaces with openings. Good agreement is obtained between IE-GSTC results and full wave simulation results for both cases.</div>

Optical detection of the susceptibility tensor in two-dimensional crystals

The out-of-plane optical constants of monolayer two-dimensional materials have proven to be experimentally elusive. Owing to their reduced dimensionality, optical measurements have limited sensitivity to these properties which are hidden by the optical response of the substrate. Therefore, there remains an absence of scientific consensus on how to correctly model these crystals. Here we perform an experiment on the optical response of a single-layer two-dimensional crystal that addresses these problems. We successfully remove the substrate contribution to its optical response by a step deposition of a monolayer crystal inside a thick polydimethylsiloxane prism. This allows for a reliable determination of both the in-plane and the out-of-plane components of its surface susceptibility tensor. Our results prescribe one clear theoretical model for these crystals. This precise characterization of their optical properties will be relevant to future progresses in photonics and optoelectronics with two-dimensional materials.

Application of cylindrical IE-GSTC to physical metasurfaces

<div>This work validates cylindrical IE-GSTC by applying it to physical metasurfaces, i.e. metasurfaces defined by material properties and dimensions rather than by susceptibility tensor components. Previously reported IE-GSTC which was formulated for zero thickness GSTC discontinuity is extended to handle finite thickness of physical metasurfaces. A simple analytical approach is used to extract the bianisotropic susceptibility tensor of concentric, multilayered, magneto-dielectric shell. Plane wave scattering by a physical metasurface constructed of four segments of multilayered, magneto-dielectric metasurface scatterers is used as an example problem to validate cylindrical IEGSTC. A second example considers an opening on the cylindrical metasurface, confirming IE-GSTC can handle metasurfaces with openings. Good agreement is obtained between IE-GSTC results and full wave simulation results for both cases.</div>

Optical detection of the susceptibility tensor in two-dimensional crystals

The out-of-plane optical constants of two-dimensional materials have proven to be experimentally elusive. Owing to the reduced dimensionality of a monolayer, optical measurements have limited sensitivity to these properties, which are hidden by the optical response of the substrate. Therefore, there remains an absence of scientific consensus on how to correctly model these materials. Theoretical descriptions span from isotropic three-dimensional slabs to two-dimensional surface currents with a null out-of-plane surface susceptibility. Here we perform a smoking gun experiment on the optical response of a single-layer two-dimensional crystal that addresses these problems. We successfully remove the substrate contribution to the optical response of these materials by a step deposition of a monolayer crystal inside a thick polydimethylsiloxane prism. This allows for a reliable determination of both the in-plane and the out-of-plane components of the monolayer surface susceptibility tensor. Our results prescribe one clear theoretical model for these types of material. This work creates opportunities for a precise characterization of the optical properties of two-dimensional crystals in all the optical domains such as the nonlinear response, surface wave phenomena or magneto-optical Kerr effect. Our assay will be relevant to future progresses in photonics and optoelectronics with 2D materials.

Application of cylindrical IE-GSTC to physical metasurfaces

<div>This work validates cylindrical IE-GSTC by applying it to physical metasurfaces, i.e. metasurfaces defined by material properties and dimensions rather than by susceptibility tensor components. Previously reported IE-GSTC which was formulated for zero thickness GSTC discontinuity is extended to handle finite thickness of physical metasurfaces. A simple analytical approach is used to extract the bianisotropic susceptibility tensor of concentric, multilayered, magneto-dielectric shell. Plane wave scattering by a physical metasurface constructed of four segments of multilayered, magneto-dielectric metasurface scatterers is used as an example problem to validate cylindrical IEGSTC. A second example considers an opening on the cylindrical metasurface, confirming IE-GSTC can handle metasurfaces with openings. Good agreement is obtained between IE-GSTC results and full wave simulation results for both cases.</div>

Application of cylindrical IE-GSTC to physical metasurfaces

<div>This work validates cylindrical IE-GSTC by applying it to physical metasurfaces, i.e. metasurfaces defined by material properties and dimensions rather than by susceptibility tensor components. Previously reported IE-GSTC which was formulated for zero thickness GSTC discontinuity is extended to handle finite thickness of physical metasurfaces. A simple analytical approach is used to extract the bianisotropic susceptibility tensor of concentric, multilayered, magneto-dielectric shell. Plane wave scattering by a physical metasurface constructed of four segments of multilayered, magneto-dielectric metasurface scatterers is used as an example problem to validate cylindrical IEGSTC. A second example considers an opening on the cylindrical metasurface, confirming IE-GSTC can handle metasurfaces with openings. Good agreement is obtained between IE-GSTC results and full wave simulation results for both cases.</div>

Magnetically induced ring currents in metallocenothiaporphyrins

The magnetically induced current-density susceptibility tensor (CDT) of the lowest singlet and triplet states of the metallocenothiaporphyrins, where the metal is V, Cr, Mn, Fe, Co, Ni, Mo, Tc, Ru,...