Gas turbine related technologies for carbon capture

Author(s):  
R. Peter Lindstedt
Keyword(s):  
Energy ◽  
2012 ◽  
Vol 45 (1) ◽  
pp. 125-133 ◽  
Author(s):  
Tadeusz Chmielniak ◽  
Sebastian Lepszy ◽  
Katarzyna Wójcik

Author(s):  
Ji Ho Ahn ◽  
Tong Seop Kim

Owing to the increasing consumption of fossil fuels and emission of greenhouse gases, interests in highly efficient and low carbon emitting power systems are growing fast. Several research groups have been suggesting advanced systems based on fuel cells and have also been applying carbon capture and storage technology to satisfy the demand for clean energy. In this study, the performance of a hybrid system, which is a combination of a molten carbonate fuel cell (MCFC) with oxy-combustion carbon capture and an indirectly fired micro gas turbine (MGT) was predicted. A 2.5MW MCFC system that is used in commercial applications was used as the reference system so that the results of the study could be applicable to practical situations. The ambient pressure type hybrid system was modeled by referring to the design parameters of an MGT that is currently being developed. A semi-closed type design characterized by flow recirculation was adopted for this hybrid system. A part of the recirculating gas is converted into liquefied carbon dioxide and captured for storage at the carbon separation unit. Almost 100% carbon dioxide capture is possible with this system. In these systems, the output power of the fuel cell is larger than in the normal hybrid system without carbon capture because the partial pressure of carbon dioxide increases. The increased cell power partially compensates for the power loss due to the carbon capture and MGT power reduction. The dependence of net system efficiency of the oxy-hybrid on compressor pressure ratio is marginal, especially beyond an optimal value.


Author(s):  
Walter W. Shelton ◽  
Robin W. Ames ◽  
Richard A. Dennis ◽  
Charles W. White ◽  
John E. Plunkett ◽  
...  

The U.S. Department of Energy’s (DOE) provides a worldwide leadership role in the development of advanced fossil fuel-based energy conversion technologies, with a focus on electric power generation with carbon capture and storage (CCS). As part of DOE’s Office of Fossil Energy, the National Energy Technology Laboratory (NETL) implements research, development, and demonstration (RD&D) programs that address the challenges of reducing greenhouse gas emissions. To meet these challenges, NETL evaluates advanced power cycles that will maximize system efficiency and performance, while minimizing CO2 emissions and the costs of CCS. NETL’s Hydrogen Turbine Program has sponsored numerous R&D projects in support of Advanced Hydrogen Turbines (AHT). Turbine systems and components targeted for development include combustor technology, materials research, enhanced cooling technology, coatings development, and more. The R&D builds on existing gas turbine technologies and is intended to develop and test the component technologies and subsystems needed to validate the ability to meet the Turbine Program goals. These technologies are key components of AHTs, which enable overall plant efficiency and cost of electricity (COE) improvements relative to an F-frame turbine-based Integrated Gasification Combined Cycle (IGCC) reference plant equipped with carbon capture (today’s state-of-the-art). This work has also provided the basis for estimating future IGCC plant performance based on a Transformational Hydrogen Turbine (THT) with a higher turbine inlet temperature, enhanced material capabilities, reduced air cooling and leakage, and higher pressure ratios than the AHT. IGCC cases from using system-level AHT and THT gas turbine models were developed for comparisons with an F-frame turbine-based IGCC reference case and for an IGCC pathway study. The IGCC pathway is presented in which the reference case (i.e. includes F-frame turbine) is sequentially-modified through the incorporation of advanced technologies. Advanced technologies are considered to be either 2nd Generation or Transformational, if they are anticipated to be ready for demonstration by 2025 and 2030, respectively. The current results included the THT, additional potential transformational technologies related to IGCC plant sections (e.g. air separation, gasification, gas cleanup, carbon capture, NOx reduction) are being considered by NETL and are topics for inclusion in future reports.


Author(s):  
Ji Ho Ahn ◽  
Tong Seop Kim

Owing to the increasing consumption of fossil fuels and emission of greenhouse gases, interests in highly efficient and low carbon emitting power systems are growing fast. Several research groups have been suggesting advanced systems based on fuel cells and have also been applying carbon capture and storage technology to satisfy the demand for clean energy. In this study, the performance of a hybrid system, which is a combination of a molten carbonate fuel cell (MCFC) with oxy-combustion carbon capture and an indirectly fired micro gas turbine (MGT), was predicted. A 2.5 MW MCFC system that is used in commercial applications was used as the reference system so that the results of the study could be applied to practical situations. The ambient pressure type hybrid system was modeled by referring to the design parameters of an MGT that is currently being developed. A semi-closed type design characterized by flow recirculation was adopted for this hybrid system. A part of the recirculating gas is converted into liquefied carbon dioxide and captured for storage at the carbon separation unit (CSU). Almost 100% carbon dioxide capture is possible with this system. In these systems, the output power of the fuel cell is larger than in the normal hybrid system without carbon capture because the partial pressure of carbon dioxide increases. The increased cell power partially compensates for the power loss due to the carbon capture and MGT power reduction. The dependence of net system efficiency of the oxy-hybrid on compressor pressure ratio is marginal, especially beyond an optimal value.


Author(s):  
S. Can Gülen ◽  
Chris Hall

This paper describes a gas turbine combined cycle (GTCC) power plant system, which addresses the three key design challenges of postcombustion CO2 capture from the stack gas of a GTCC power plant using aqueous amine-based scrubbing method by offering the following: (i) low heat recovery steam generator (HRSG) stack gas temperature, (ii) increased HRSG stack gas CO2 content, and (iii) decreased HRSG stack gas O2 content. This is achieved by combining two bottoming cycle modifications in an inventive manner, i.e., (i) high supplementary (duct) firing in the HRSG and (ii) recirculation of the HRSG stack gas. It is shown that, compared to an existing natural gas-fired GTCC power plant with postcombustion capture, it is possible to reduce the CO2 capture penalty—power diverted away from generation—by almost 65% and the overall capital cost ($/kW) by about 35%.


Energy ◽  
2016 ◽  
Vol 115 ◽  
pp. 1138-1147 ◽  
Author(s):  
Thom Best ◽  
Karen N. Finney ◽  
Derek B. Ingham ◽  
Mohamed Pourkashanian

Author(s):  
Ji Ho Ahn ◽  
Ji Hun Jeong ◽  
Tong Seop Kim

The demand for clean energy continues to increase as the human society becomes more aware of environmental challenges such as global warming. Various power systems based on high-temperature fuel cells have been proposed, especially hybrid systems combining a fuel cell with a gas turbine, and research on carbon capture and storage technology to prevent the emission of greenhouse gases is already underway. This study suggests a new method to innovatively enhance the efficiency of a molten carbonate fuel cell/micro gas turbine hybrid system including carbon capture. The key technology adopted to improve the net cycle efficiency is off-gas recirculation. The hybrid system incorporating oxy-combustion capture was devised, and its performance was compared with that of a post-combustion system based on a hybrid system. A molten carbonate fuel cell system based on a commercial unit was modeled. Externally supplied water for reforming was not needed as a result of the presence of the water vapor in the recirculated anode off-gas. The analyses confirmed that the thermal efficiencies of all the systems (MCFC stand-alone, hybrid, hybrid with oxy-combustion capture, hybrid with post-combustion capture) were significantly improved by introducing the off-gas recirculation. In particular, the largest efficiency improvement was observed for the oxy-combustion hybrid system. Its efficiency is over 57% and is even higher than that of the post-combustion hybrid system.


Author(s):  
A. M. Elkady ◽  
A. R. Brand ◽  
C. L. Vandervort ◽  
A. T. Evulet

In a carbon constrained world there is a need for capturing and sequestering CO2. Post-combustion carbon capture via Exhaust Gas Recirculation (EGR) is considered a feasible means of reducing emission of CO2 from power plants. Exhaust Gas Recirculation is an enabling technology for increasing the CO2 concentration within the gas turbine cycle and allow the decrease of the size of the separation plant, which in turn will enable a significant reduction in CO2 capture cost. This paper describes the experimental work performed to better understand the risks of utilizing EGR in combustors employing dry low emissions (DLE) technologies. A rig was built for exploring the capability of premixers to operate in low O2 environment, and a series of experiments in a visually accessible test rig was performed at representative aeroderivative gas turbine pressures and temperatures. Experimental results include the effect of applying EGR on operability, efficiency and emissions performance under conditions of up to 40% EGR. Findings confirm the viability of EGR for enhanced CO2 capture; In addition, we confirm benefits of NOx reduction while complying with CO emissions in DLE combustors under low oxygen content oxidizer.


Author(s):  
Muhammad Akram ◽  
Bhupendra Khandelwal ◽  
Simon Blakey ◽  
Christopher W. Wilson

Carbon capture is getting increased attention recently due to the fact that it seems to be the only answer to decrease emissions. Gas turbines exhaust have 3–5 % concentration of CO2 which is very low to be captured by an amine carbon capture plant effectively. The amine based plants are most effective at around 10 – 15% CO2 in the flue gas. In order to increase the concentration of CO2 in the exhaust of the gas turbine, part of the exhaust gas needs to be recycled back to the air inlet. On reaching the concentration of CO2 around 10% it can be fed to the amine capture plant for effective carbon capture. A 100 kWe (plus 150 kW hot water) CHP gas turbine Turbec T100 is installed at the Low Carbon Combustion Centre of the University of Sheffield. The turbine set up will be modified to make it CO2 capture ready. The exhaust gases obtained will be piped to amine capture plant for testing capture efficiency. Preliminary calculations have been done and presented in this paper. The thermodynamic properties of CO2 are different from nitrogen and will have an effect on compressor, combustor and turbine performance. Preliminary calculations of recycle ratios and other performance based parameters have been presented in this paper. This paper also covers the aspects of turbine set up machinery which needs to be modified and what kind of modifications may be needed.


Author(s):  
Felipe Bolaños ◽  
Dieter Winkler ◽  
Felipe Piringer ◽  
Timothy Griffin ◽  
Rolf Bombach ◽  
...  

The combustion of hydrogen-rich fuels (> 80 % vol. H2), relevant for gas turbine cycles with “pre-combustion” carbon capture, creates great challenges in the application of standard lean premix combustion technology. The significant higher flame speed and drastically reduced auto-ignition delay time of hydrogen compared to those of natural gas, which is normally burned in gas turbines, increase the risk of higher NOX emissions and material damage due to flashback. Combustion concepts for gas turbines operating on hydrogen fuel need to be adapted to assure safe and low-emission combustion. A rich/lean (R/L) combustion concept with integrated heat transfer that addresses the challenges of hydrogen combustion has been investigated. A sub-scale, staged burner with full optical access has been designed and tested at gas turbine relevant conditions (flame temperature of 1750 K, preheat temperature of 400 °C and a pressure of 8 bar). Results of the burner tests have confirmed the capability of the rich/lean staged concept to reduce the NOx emissions for undiluted hydrogen fuel. The NOx emissions were reduced from 165 ppm measured without staging (fuel pre-conversion) to 23 ppm for an R/L design having a fuel-rich hydrogen pre-conversion of 50 % at a constant power of 8.7 kW. In the realized R/L concept the products of the first rich stage, which is ignited by a Pt/Pd catalyst (under a laminar flow, Re ≈ 1900) are combusted in a diffusion-flame-like lean stage (turbulent flow Re ≈ 18500) without any flashback risk. The optical accessibility of the reactor has allowed insight into the combustion processes of both stages. Applying OH-LIF and OH*-chemiluminescence optical techniques, it was shown that mainly homogeneous reactions at rich conditions take place in the first stage, questioning the importance of a catalyst in the system, and opening a wide range of optimization possibilities. The promising results obtained in this study suggest that such a rich/lean staged burner with integrated heat transfer could help to develop a new generation of gas turbine burners for safe and clean combustion of H2-rich fuels.


Sign in / Sign up

Export Citation Format

Share Document