scholarly journals Subvisible cirrus clouds – a dynamical system approach

2016 ◽  
Author(s):  
E. J. Spreitzer ◽  
M. P. Marschalik ◽  
P. Spichtinger
Keyword(s):  
Cloud Model ◽  
Three Dimensional ◽  
Complex Model ◽  
Cirrus Clouds ◽  
Diffusional Growth ◽  
Ice Clouds ◽  
Formation Pathway ◽  
Microphysical Properties ◽  
Tropopause Region ◽  
Homogeneous Freezing

Abstract. Ice clouds, so-called cirrus clouds, occur very frequently in the tropopause region. A special class are subvisible cirrus clouds with an optical depth lower than 0.03. Obviously, the ice crystal number concentration of these clouds is very low. The dominant pathway for these clouds is not known well. It is often assumed that heterogeneous nucleation at solid aerosol particles is the preferred mechanism although homogeneous freezing of aqueous solution droplets might be possible. For investigating subvisible cirrus clouds as formed by homogeneous freezing we develop a simple analytical cloud model from first principles; the model consists of a three dimensional set of ordinary differential equations, including the relevant processes as ice nucleation, diffusional growth and sedimentation, respectively. The model is integrated numerically and is investigated using theory of dynamical systems. We found two different states for the long-term behaviour of subvisible cirrus clouds, i.e. an attractor case and a limit cycle scenario. The transition between the states constitutes a Hopf bifurcation and is determined by environmental conditions as vertical updraughts and temperature. In both cases, the microphysical properties of the simulated clouds agree reasonably well with simulations using a complex model, with former analytical studies and with observations of subvisible cirrus. In addition, the model can also be used for explaining complex model simulations close to the bifurcation qualitatively. Finally, the results indicate that homogeneous nucleation might be a possible formation pathway for subvisible cirrus clouds.

scholarly journals Subvisible cirrus clouds – a dynamical system approach

2017 ◽  
Vol 24 (3) ◽  
pp. 307-328 ◽  
Author(s):  
Elisa Johanna Spreitzer ◽  
Manuel Patrik Marschalik ◽  
Peter Spichtinger
Keyword(s):  
Low Temperature ◽  
Differential Equations ◽  
Temperature Regime ◽  
Large Scale ◽  
Cloud Model ◽  
Three Dimensional ◽  
Cirrus Clouds ◽  
Diffusional Growth ◽  
Detailed Model ◽  
Homogeneous Freezing

Abstract. Ice clouds, so-called cirrus clouds, occur very frequently in the tropopause region. A special class are subvisible cirrus clouds with an optical depth lower than 0.03, associated with very low ice crystal number concentrations. The dominant pathway for the formation of these clouds is not known well. It is often assumed that heterogeneous nucleation on solid aerosol particles is the preferred mechanism although homogeneous freezing of aqueous solution droplets might be possible, since these clouds occur in the low-temperature regime T < 235 K. For investigating subvisible cirrus clouds as formed by homogeneous freezing we develop a reduced cloud model from first principles, which is close enough to complex models but is also simple enough for mathematical analysis. The model consists of a three-dimensional set of ordinary differential equations, and includes the relevant processes as ice nucleation, diffusional growth and sedimentation. We study the formation and evolution of subvisible cirrus clouds in the low-temperature regime as driven by slow vertical updraughts (0 < w ≤ 0. 05 m s−1). The model is integrated numerically and also investigated by means of theory of dynamical systems. We found two qualitatively different states for the long-term behaviour of subvisible cirrus clouds. The first state is a stable focus; i.e. the solution of the differential equations performs damped oscillations and asymptotically reaches a constant value as an equilibrium state. The second state is a limit cycle in phase space; i.e. the solution asymptotically approaches a one-dimensional attractor with purely oscillatory behaviour. The transition between the states is characterised by a Hopf bifurcation and is determined by two parameters – vertical updraught velocity and temperature. In both cases, the properties of the simulated clouds agree reasonably well with simulations from a more detailed model, with former analytical studies, and with observations of subvisible cirrus, respectively. The reduced model can also provide qualitative interpretations of simulations with a complex and more detailed model at states close to bifurcation qualitatively. The results indicate that homogeneous nucleation is a possible formation pathway for subvisible cirrus clouds. The results motivate a minimal model for subvisible cirrus clouds (SVCs), which might be used in future work for the development of parameterisations for coarse large-scale models, representing structures of clouds.

scholarly journals Thermodynamic phase retrieval of convective clouds: impact of sensor viewing geometry and vertical distribution of cloud properties

2013 ◽  
Vol 6 (3) ◽  
pp. 539-547 ◽  
Author(s):  
E. Jäkel ◽  
J. Walter ◽  
M. Wendisch
Keyword(s):  
Phase Retrieval ◽  
Near Infrared ◽  
Three Dimensional ◽  
Ice Clouds ◽  
Convective Clouds ◽  
Microphysical Properties ◽  
Cloud Properties ◽  
Reflectivity Spectra ◽  
Vertical Distributions ◽  
Thermodynamic Phase

Abstract. The sensitivity of passive remote sensing measurements to retrieve microphysical parameters of convective clouds, in particular their thermodynamic phase, is investigated by three-dimensional (3-D) radiative transfer simulations. The effects of different viewing geometries and vertical distributions of the cloud microphysical properties are investigated. Measurement examples of spectral solar radiance reflected by cloud sides (passive) in the near-infrared (NIR) spectral range are performed together with collocated lidar observations (active). The retrieval method to distinguish the cloud thermodynamic phase (liquid water or ice) exploits different slopes of cloud side reflectivity spectra of water and ice clouds in the NIR. The concurrent depolarization backscattering lidar provides geometry information about the cloud distance and height as well as the depolarization.

scholarly journals UV Raman lidar measurements of relative humidity for the characterization of cirrus cloud microphysical properties

2009 ◽  
Vol 9 (22) ◽  
pp. 8799-8811 ◽  
Author(s):  
P. Di Girolamo ◽  
D. Summa ◽  
R.-F. Lin ◽  
T. Maestri ◽  
R. Rizzi ◽  
...  
Keyword(s):  
Relative Humidity ◽  
Cloud Model ◽  
Cirrus Clouds ◽  
Cloud Layer ◽  
Cirrus Cloud ◽  
Raman Lidar ◽  
Heating Rates ◽  
Night Time ◽  
Microphysical Properties ◽  
Lidar Measurements

Abstract. Raman lidar measurements performed in Potenza by the Raman lidar system BASIL in the presence of cirrus clouds are discussed. Measurements were performed on 6 September 2004 in the frame of the Italian phase of the EAQUATE Experiment. The major feature of BASIL is represented by its capability to perform high-resolution and accurate measurements of atmospheric temperature and water vapour, and consequently relative humidity, both in daytime and night-time, based on the application of the rotational and vibrational Raman lidar techniques in the UV. BASIL is also capable to provide measurements of the particle backscatter and extinction coefficient, and consequently lidar ratio (at the time of these measurements, only at one wavelength), which are fundamental to infer geometrical and microphysical properties of clouds. A case study is discussed in order to assess the capability of Raman lidars to measure humidity in presence of cirrus clouds, both below and inside the cloud. While air inside the cloud layers is observed to be always under-saturated with respect to water, both ice super-saturation and under-saturation conditions are found inside these clouds. Upper tropospheric moistening is observed below the lower cloud layer. The synergic use of the data derived from the ground based Raman Lidar and of spectral radiances measured by the NAST-I Airborne Spectrometer allows the determination of the temporal evolution of the atmospheric cooling/heating rates due to the presence of the cirrus cloud. Lidar measurements beneath the cirrus cloud layer have been interpreted using a 1-D cirrus cloud model with explicit microphysics. The 1-D simulations indicate that sedimentation-moistening has contributed significantly to the moist anomaly, but other mechanisms are also contributing. This result supports the hypothesis that the observed mid-tropospheric humidification is a real feature which is strongly influenced by the sublimation of precipitating ice crystals. Results illustrated in this study demonstrate that Raman lidars, like the one used in this study, can resolve the spatial and temporal scales required for the study of cirrus cloud microphysical processes and appear sensitive enough to reveal and quantify upper tropospheric humidification associated with cirrus cloud sublimation.

Impact of nucleation rates and diffusional growth on ice nucleation events

2020 ◽  
Author(s):  
Peter Spichtinger
Keyword(s):  
Nucleation Rate ◽  
Homogeneous Nucleation ◽  
Water Saturation ◽  
Direct Interaction ◽  
Ice Crystal ◽  
Diffusional Growth ◽  
Cloud Droplets ◽  
Formation Pathway ◽  
Tropopause Region ◽  
The Impact

&lt;p&gt;Cirrus clouds in the tropopause region form via two major different pathways, i.e. freezing super-cooled cloud droplets (liquid origin) or nucleating ice crystals at humidities below water saturation (in situ formation). The latter case takes place in the low temperature regime (T&lt;235K) and it is assumed that in this regime homogeneous freezing of supercooled solution droplets (short: homogeneous nucleation) is the dominant formation pathway. For homogeneous nucleation, a nucleation rate has been derived from laboratory experiments, based on water activity. The formulation of the nucleation rate is reassessed and simple but robust approximations are presented, which can be used in less complex models without a direct interaction with aerosols. The impact of nucleation rates and the formulation of diffusional growth for idealized nucleation rates is investigated. It can be found that the absolute value of the nucleation rate has almost no impact on the produced ice crystal number concentrations, whereas the steepness of the rate is much more important. Finally, it turns out that the formulation of diffusional growth affects nucleation events crucially in terms of produced ice crystal numbers.&lt;/p&gt;

scholarly journals Comparison of IAGOS in-situ water vapour measurements and ECMWF ERA-Interim Reanalysis data

2019 ◽  
Author(s):  
Philipp Reutter ◽  
Patrick Neis ◽  
Susanne Rohs ◽  
Bastien Sauvage
Keyword(s):  
Water Vapour ◽  
Spatial Resolution ◽  
Three Dimensional ◽  
Reanalysis Data ◽  
Cirrus Clouds ◽  
Data Sets ◽  
The North ◽  
Tropopause Region ◽  
Good Agreement

Abstract. Cirrus clouds and their potential formation regions, so-called ice-supersaturated regions (ISSRs) occur frequently in the tropopause region. It is assumed that ISSRs and cirrus clouds can change the tropopause structure by diabatic processes, driven by latent heating due to phase transition and interaction with radiation. For many research questions a three-dimensional picture including a sufficient temporal resolution of the water vapour fields in the tropopause region is required. This requirement is fulfilled nowadays by reanalysis products such as the European Centre for Medium-Range Weather Forecasts (ECMWF) ERA-Interim reanalysis. However, for a meaningful investigation of water vapour in the tropopause region a comparison of the reanalysis data with measurement is advisable, since it is difficult to measure water vapour and to assimilate meaningful measurements into reanalysis products. Here, we present an intercomparison of high-resolution in-situ measurements aboard passenger aircraft within the European Research Infrastructure IAGOS (In-service Aircraft for a Global Observing System; http://www.iagos.org) with ERA-Interim. Temperature and humidity data over the North Atlantic from 2000 to 2010 are compared relative to the dynamical tropopause. The comparison of the temperature shows a good agreement between measurement and ERA-Interim. While ERA-Interim can reproduce the main features of the water vapour measurements of IAGOS, the variability of the data is underestimated by the reanalysis data. The combination of temperature and water vapour leads to the relative humidity with respect to ice (RHi). Here ERA-Interim deviates from the measurements concerning values of larger than RHi=100 %, both in number and strength of supersaturation. The comparison of ISSR pathlengths shows distinct differences, which can be traced back to the spatial resolution of both data sets. IAGOS shows significantly more smaller ISSRs compared to ERA-Interim. A good agreement begins only at pathlengths in the order of the ERA-Interim spatial resolution and larger.

scholarly journals Thermodynamic phase retrieval of convective clouds: impact of sensor viewing geometry and vertical distribution of cloud properties

2012 ◽  
Vol 5 (5) ◽  
pp. 7729-7752
Author(s):  
E. Jäkel ◽  
J. Walter ◽  
M. Wendisch
Keyword(s):  
Phase Retrieval ◽  
Near Infrared ◽  
Three Dimensional ◽  
Ice Clouds ◽  
Convective Clouds ◽  
Microphysical Properties ◽  
Cloud Properties ◽  
Index Measurement ◽  
Microphysical Parameters ◽  
Thermodynamic Phase

Abstract. The potential to use combined passive and active remote sensing measurements to retrieve microphysical parameters of convective clouds in particular thermodynamic phase, is investigated by three-dimensional (3-D) radiative transfer simulations. The 3-D simulations are used to quantify the effect of different viewing geometries and distributions of the cloud microphysical properties on the derived ice index. Measurement examples of spectral solar and radiance reflected by cloud sides (passive) in the near-infrared (NIR) spectral range are synchronized with collocated Lidar observations (active). A retrieval method to distinguish the cloud thermodynamic phase (liquid water or ice) using the reported reflectivity measurements is applied which uses the different spectral slopes of water and ice clouds in the NIR. The concurrent depolarization backscattering Lidar provides geometry information about the cloud distance and height as well as the depolarization.

scholarly journals The origin of midlatitude ice clouds and the resulting influence on their microphysical properties

2015 ◽  
Vol 15 (23) ◽  
pp. 34243-34281 ◽  
Author(s):  
A. E. Luebke ◽  
A. Afchine ◽  
A. Costa ◽  
J. Meyer ◽  
C. Rolf ◽  
...  
Keyword(s):  
Bimodal Distribution ◽  
Cirrus Clouds ◽  
Ice Crystals ◽  
Radiative Properties ◽  
Ice Crystal ◽  
Ice Clouds ◽  
Microphysical Properties ◽  
Ice Crystal Size ◽  
Ice Water

Abstract. The radiative role of ice clouds in the atmosphere is known to be important, but uncertainties remain concerning the magnitude and net effects. However, through measurements of the microphysical properties of cirrus clouds, we can better characterize them, which can ultimately allow for their radiative properties to be more accurately ascertained. It has recently been proposed that there are two types of cirrus clouds – in situ and liquid origin. In this study, we present observational evidence to show that two distinct types of cirrus do exist. Airborne, in situ measurements of cloud ice water content (IWC), ice crystal concentration (Nice), and ice crystal size from the 2014 ML-CIRRUS campaign provide cloud samples that have been divided according to their origin type. The key features that set liquid origin cirrus apart from the in situ origin cirrus are a higher frequency of high IWC (> 100 ppmv), higher Nice values, and larger ice crystals. A vertical distribution of Nice shows that the in situ origin cirrus clouds exhibit a median value of around 0.1 cm−3, while the liquid origin concentrations are slightly, but notably higher. The median sizes of the crystals contributing the most mass are less than 200 μm for in situ origin cirrus, with some of the largest crystals reaching 550 μm in size. The liquid origin cirrus, on the other hand, were observed to have median diameters greater than 200 μm, and crystals that were up to 750 μm. An examination of these characteristics in relation to each other and their relationship to temperature provides strong evidence that these differences arise from the dynamics and conditions in which the ice crystals formed. Additionally, the existence of these two groups in cirrus cloud populations may explain why a bimodal distribution in the IWC-temperature relationship has been observed. We hypothesize that the low IWC mode is the result of in situ origin cirrus and the high IWC mode is the result of liquid origin cirrus.

scholarly journals The origin of midlatitude ice clouds and the resulting influence on their microphysical properties

2016 ◽  
Vol 16 (9) ◽  
pp. 5793-5809 ◽  
Author(s):  
Anna E. Luebke ◽  
Armin Afchine ◽  
Anja Costa ◽  
Jens-Uwe Grooß ◽  
Jessica Meyer ◽  
...  
Keyword(s):  
Bimodal Distribution ◽  
Cirrus Clouds ◽  
Ice Crystals ◽  
Radiative Properties ◽  
Ice Crystal ◽  
Ice Clouds ◽  
Microphysical Properties ◽  
Ice Crystal Size ◽  
Ice Water

Abstract. The radiative role of ice clouds in the atmosphere is known to be important, but uncertainties remain concerning the magnitude and net effects. However, through measurements of the microphysical properties of cirrus clouds, we can better characterize them, which can ultimately allow for their radiative properties to be more accurately ascertained. Recently, two types of cirrus clouds differing by formation mechanism and microphysical properties have been classified – in situ and liquid origin cirrus. In this study, we present observational evidence to show that two distinct types of cirrus do exist. Airborne, in situ measurements of cloud ice water content (IWC), ice crystal concentration (Nice), and ice crystal size from the 2014 ML-CIRRUS campaign provide cloud samples that have been divided according to their origin type. The key features that set liquid origin cirrus apart from the in situ origin cirrus are higher frequencies of high IWC ( > 100 ppmv), higher Nice values, and larger ice crystals. A vertical distribution of Nice shows that the in situ origin cirrus clouds exhibit a median value of around 0.1 cm−3, while the liquid origin concentrations are slightly, but notably higher. The median sizes of the crystals contributing the most mass are less than 200 µm for in situ origin cirrus, with some of the largest crystals reaching 550 µm in size. The liquid origin cirrus, on the other hand, were observed to have median diameters greater than 200 µm, and crystals that were up to 750 µm. An examination of these characteristics in relation to each other and their relationship to temperature provides strong evidence that these differences arise from the dynamics and conditions in which the ice crystals formed. Additionally, the existence of these two groups in cirrus cloud populations may explain why a bimodal distribution in the IWC-temperature relationship has been observed. We hypothesize that the low IWC mode is the result of in situ origin cirrus and the high IWC mode is the result of liquid origin cirrus.

scholarly journals Validation of cloud property retrievals with simulated satellite radiances: a case study for SEVIRI

2010 ◽  
Vol 10 (9) ◽  
pp. 21931-21988 ◽  
Author(s):  
L. Bugliaro ◽  
T. Zinner ◽  
C. Keil ◽  
B. Mayer ◽  
R. Hollmann ◽  
...  
Keyword(s):  
Standard Deviation ◽  
Three Dimensional ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Cloud Detection ◽  
Ice Clouds ◽  
Cloud Property ◽  
Microphysical Properties ◽  
Cloud Properties ◽  
Weather Model

Abstract. Validation of cloud properties retrieved from passive spaceborne imagers is essential for cloud and climate applications but complicated due to the large differences in scale and observation geometry between the satellite footprint and the independent ground based or airborne observations. Here we illustrate and demonstrate an alternative approach: starting from the output of the COSMO-EU weather model of the German Weather Service realistic three-dimensional cloud structures at a spatial scale of 2.33 km are produced by statistical downscaling and microphysical properties are associated to them. The resulting data sets are used as input to the one-dimensional radiative transfer model libRadtran to simulate radiance observations for all eleven low resolution channels of MET-8/SEVIRI. At this point, both cloud properties and satellite radiances are known such that cloud property retrieval results can be tested and tuned against the objective input "truth". As an example, we validate a cloud property retrieval of the Institute of Atmospheric Physics of DLR and that of EUMETSAT's Climate Monitoring Science Application Facility CMSAF. Cloud detection and cloud phase assignment perform well. By both retrievals 88% of the pixels are correctly classified as clear or cloudy. The DLR algorithm assigns the correct thermodynamic phase to 95% of the cloudy pixels and the CMSAF retrieval to 79%. Cloud top temperature is slightly overestimated by the DLR code (+3.1 K mean difference with a standard deviation of 10.6 K) and underestimated by the CMSAF code (−16.4 K with a standard deviation of 37.3 K). Both retrievals account reasonably well for the distribution of optical thickness for both water and ice clouds, with a tendency to underestimation for the DLR and to overestimation for the CMSAF algorithm. Cloud effective radii are most difficult to evaluate and not always the algorithms are able to produce realistic values. The CMSAF cloud water path, which is a combination of the last two quantities, is particularly accurate for ice clouds, while water clouds are overestimated, mainly because of the effective radius overestimation for water clouds.

scholarly journals Cloud chamber experiments on the origin of ice crystal complexity in cirrus clouds

2015 ◽  
Vol 15 (21) ◽  
pp. 30511-30561 ◽  
Author(s):  
M. Schnaiter ◽  
E. Järvinen ◽  
P. Vochezer ◽  
A. Abdelmonem ◽  
R. Wagner ◽  
...  
Keyword(s):  
Light Scattering ◽  
Cloud Chamber ◽  
Cirrus Clouds ◽  
Atmospheric Conditions ◽  
Ice Crystal ◽  
Ice Clouds ◽  
Spatially Resolved ◽  
Microphysical Properties ◽  
Institute Of Technology ◽  
Low Sensitivity

Abstract. This study reports on the origin of ice crystal complexity and its influence on the angular light scattering properties of cirrus clouds. Cloud simulation experiments were conducted at the AIDA (Aerosol Interactions and Dynamics in the Atmosphere) cloud chamber of the Karlsruhe Institute of Technology (KIT). A new experimental procedure was applied to grow and sublimate ice particles at defined super- and subsaturated ice conditions and for temperatures in the −40 to −60 °C range. The experiments were performed for ice clouds generated via homogeneous and heterogeneous initial nucleation. Ice crystal complexity was deduced from measurements of spatially resolved single particle light scattering patterns by the latest version of the Small Ice Detector (SID-3). It was found that a high ice crystal complexity is dominating the microphysics of the simulated clouds and the degree of this complexity is dependent on the available water vapour during the crystal growth. Indications were found that the crystal complexity is influenced by unfrozen H2SO4/H2O residuals in the case of homogeneous initial ice nucleation. Angular light scattering functions of the simulated ice clouds were measured by the two currently available airborne polar nephelometers; the Polar Nephelometer (PN) probe of LaMP and the Particle Habit Imaging and Polar Scattering (PHIPS-HALO) probe of KIT. The measured scattering functions are featureless and flat in the side- and backward scattering directions resulting in low asymmetry parameters g around 0.78. It was found that these functions have a rather low sensitivity to the crystal complexity for ice clouds that were grown under typical atmospheric conditions. These results have implications for the microphysical properties of cirrus clouds and for the radiative transfer through these clouds.

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