scholarly journals Development of CarbonTracker Europe-CH<sub>4</sub> – Part 2: global methane emission estimates and their evaluation for 2000–2012

2016 ◽  
Author(s):  
Aki Tsuruta ◽  
Tuula Aalto ◽  
Leif Backman ◽  
Janne Hakkarainen ◽  
Ingrid T. van der Laan-Luijkx ◽  
...  
Keyword(s):  
North American ◽  
Transport Model ◽  
Vertical Mixing ◽  
Total Carbon ◽  
In Situ Observation ◽  
Convection Scheme ◽  
Temperate Region ◽  
Northern Latitude ◽  
The North

Abstract. Gobal methane emissions were estimated for 2000–2012 using the CarbonTracker Europe-CH4 (CTE-CH4) data assimilation system. In CTE-CH4, the anthropogenic and biosphere emissions of CH4 are simultaneously constrained by global atmospheric in-situ methane mole fraction observations. We use three configurations developed in Tsuruta et al. (2016) to assess the sensitivity of the CH4 flux estimates to (a) the number of unknown flux scaling factors to be optimized which in turn depends on the choice of underlying land-ecosystem map, and (b) on the parametrization of vertical mixing in the 30 atmospheric transport model TM5. The posterior emission estimates were evaluated by comparing simulations to surface in-situ observation sites, to profile observations made by aircraft, to dry air total column-averaged mole fractions (XCH4) observations from the Total Carbon Column Observing Network (TCCON), and to XCH4 retrievals from the Greenhouse gases Observing SATellite (GOSAT). Our estimated posterior mean global total emissions during 2000–2012 are 516 ± 51 Tg CH4 yr−1, and emission estimates during 2007–2012 are 18 Tg CH4 yr−1 greater than those from 2001–2006, mainly driven by an 35 increase in emissions from the south America temperate region, the Asia temperate region and Asia tropics. The sensitivity of the flux estimates to the underlying ecosystem map was large for the Asia temperate region and Australia, but not significant in the northern latitude regions, i.e. the north American boreal region, the north American temperate region and Europe. Instead, the posterior estimates for the northern latitude regions show larger sensitivity to the choice of convection scheme in TM5. The Gregory et al. (2000) mixing scheme with faster interhemispheric exchange leads to higher estimated CH4 emissions at northern latitudes, and lower emissions in southern latitudes, compared to the estimates using Tiedtke (1989) convection scheme. Our evaluation with non-assimilated observations showed that posterior mole fractions were better matched with the 5 observations when Gregory et al. (2000) convection scheme was used.

scholarly journals Global methane emission estimates for 2000–2012 from CarbonTracker Europe-CH<sub>4</sub> v1.0

2017 ◽  
Vol 10 (3) ◽  
pp. 1261-1289 ◽  
Author(s):  
Aki Tsuruta ◽  
Tuula Aalto ◽  
Leif Backman ◽  
Janne Hakkarainen ◽  
Ingrid T. van der Laan-Luijkx ◽  
...  
Keyword(s):  
Data Assimilation ◽  
Transport Model ◽  
Atmospheric Transport ◽  
Vertical Mixing ◽  
The United States ◽  
Total Carbon ◽  
Ch4 Emissions ◽  
Data Assimilation System ◽  
Assimilation System

Abstract. We present a global distribution of surface methane (CH4) emission estimates for 2000–2012 derived using the CarbonTracker Europe-CH4 (CTE-CH4) data assimilation system. In CTE-CH4, anthropogenic and biospheric CH4 emissions are simultaneously estimated based on constraints of global atmospheric in situ CH4 observations. The system was configured to either estimate only anthropogenic or biospheric sources per region, or to estimate both categories simultaneously. The latter increased the number of optimizable parameters from 62 to 78. In addition, the differences between two numerical schemes available to perform turbulent vertical mixing in the atmospheric transport model TM5 were examined. Together, the system configurations encompass important axes of uncertainty in inversions and allow us to examine the robustness of the flux estimates. The posterior emission estimates are further evaluated by comparing simulated atmospheric CH4 to surface in situ observations, vertical profiles of CH4 made by aircraft, remotely sensed dry-air total column-averaged mole fraction (XCH4) from the Total Carbon Column Observing Network (TCCON), and XCH4 from the Greenhouse gases Observing Satellite (GOSAT). The evaluation with non-assimilated observations shows that posterior XCH4 is better matched with the retrievals when the vertical mixing scheme with faster interhemispheric exchange is used. Estimated posterior mean total global emissions during 2000–2012 are 516 ± 51 Tg CH4 yr−1, with an increase of 18 Tg CH4 yr−1 from 2000–2006 to 2007–2012. The increase is mainly driven by an increase in emissions from South American temperate, Asian temperate and Asian tropical TransCom regions. In addition, the increase is hardly sensitive to different model configurations ( <  2 Tg CH4 yr−1 difference), and much smaller than suggested by EDGAR v4.2 FT2010 inventory (33 Tg CH4 yr−1), which was used for prior anthropogenic emission estimates. The result is in good agreement with other published estimates from inverse modelling studies (16–20 Tg CH4 yr−1). However, this study could not conclusively separate a small trend in biospheric emissions (−5 to +6.9 Tg CH4 yr−1) from the much larger trend in anthropogenic emissions (15–27 Tg CH4 yr−1). Finally, we find that the global and North American CH4 balance could be closed over this time period without the previously suggested need to strongly increase anthropogenic CH4 emissions in the United States. With further developments, especially on the treatment of the atmospheric CH4 sink, we expect the data assimilation system presented here will be able to contribute to the ongoing interpretation of changes in this important greenhouse gas budget.

scholarly journals Automated Quality Control of In Situ Soil Moisture from the North American Soil Moisture Database Using NLDAS-2 Products

2015 ◽  
Vol 54 (6) ◽  
pp. 1267-1282 ◽  
Author(s):  
Youlong Xia ◽  
Trent W. Ford ◽  
Yihua Wu ◽  
Steven M. Quiring ◽  
Michael B. Ek
Keyword(s):  
Quality Control ◽  
Soil Moisture ◽  
North American ◽  
Soil Layer ◽  
Control Procedure ◽  
Multiple Model ◽  
Quality Control Procedure ◽  
The North ◽  
Automated Quality Control

AbstractThe North American Soil Moisture Database (NASMD) was initiated in 2011 to provide support for developing climate forecasting tools, calibrating land surface models, and validating satellite-derived soil moisture algorithms. The NASMD has collected data from over 30 soil moisture observation networks providing millions of in situ soil moisture observations in all 50 states, as well as Canada and Mexico. It is recognized that the quality of measured soil moisture in NASMD is highly variable because of the diversity of climatological conditions, land cover, soil texture, and topographies of the stations, and differences in measurement devices (e.g., sensors) and installation. It is also recognized that error, inaccuracy, and imprecision in the data can have significant impacts on practical operations and scientific studies. Therefore, developing an appropriate quality control procedure is essential to ensure that the data are of the best quality. In this study, an automated quality control approach is developed using the North American Land Data Assimilation System, phase 2 (NLDAS-2), Noah soil porosity, soil temperature, and fraction of liquid and total soil moisture to flag erroneous and/or spurious measurements. Overall results show that this approach is able to flag unreasonable values when the soil is partially frozen. A validation example using NLDAS-2 multiple model soil moisture products at the 20-cm soil layer showed that the quality control procedure had a significant positive impact in Alabama, North Carolina, and west Texas. It had a greater impact in colder regions, particularly during spring and autumn. Over 433 NASMD stations have been quality controlled using the methodology proposed in this study, and the algorithm will be implemented to control data quality from the other ~1200 NASMD stations in the near future.

Paleomagnetism of the Lawrenceton Formation volcanic rocks, Silurian Botwood Group, Change Islands, Newfoundland

1989 ◽  
Vol 26 (2) ◽  
pp. 296-304 ◽  
Author(s):  
Julie E. Gales ◽  
Ben A. van der Pluijm ◽  
Rob Van der Voo
Keyword(s):  
North American ◽  
Volcanic Rocks ◽  
Mobile Belt ◽  
Structural Mapping ◽  
Polar Wander ◽  
The North ◽  
Apparent Polar Wander Path ◽  
Paleomagnetic Study ◽  
North American Craton

Paleomagnetic sampling of the Lawrenceton Formation of the Silurian Botwood Group in northeastern Newfoundland was combined with detailed structural mapping of the area in order to determine the deformation history and make adequate structural corrections to the paleomagnetic data.Structural analysis indicates that the Lawrenceton Formation experienced at least two folding events: (i) a regional northeast–southwest-trending, Siluro-Devonian folding episode that produced a well-developed axial-plane cleavage; and (ii) an episode of local north-trending folding. Bedding – regional cleavage relationships indicate that the latter event is older than the regional folding.Thermal demagnetization of the Lawrenceton Formation yielded univectorial southerly and shallow directions (in situ). A fold test on an early mesoscale fold indicates that the magnetization of the Botwood postdates this folding event. However, our results, combined with an earlier paleomagnetic study of nearby Lawrenceton Formation rocks, demonstrate that the magnetization predates the regional folding. Therefore, we conclude that the magnetization occurred subsequent to the local folding but prior to the period of regional folding.While a tectonic origin for local folding cannot be entirely excluded, the subaerial nature of these volcanics, the isolated occurrence of these folds, and the absence of similar north-trending folds in other areas of eastern Notre Dame Bay suggest a syndepositional origin. Consequently, the magnetization may be nearly primary. Our study yields a characteristic direction of D = 175°, I = +43°, with a paleopole (16°N, 131 °E) that plots near the mid-Silurian track of the North American apparent polar wander path. This result is consistent with an early origin for the magnetization and supports the notion that the Central Mobile Belt of Newfoundland was adjacent to the North American craton, in its present-day position, since the Silurian.

scholarly journals In situ observation of atmospheric oxygen and carbon dioxide in the North Pacific using a cargo ship

2018 ◽  
Vol 18 (13) ◽  
pp. 9283-9295 ◽  
Author(s):  
Yu Hoshina ◽  
Yasunori Tohjima ◽  
Keiichi Katsumata ◽  
Toshinobu Machida ◽  
Shin-ichiro Nakaoka
Keyword(s):  
Carbon Dioxide ◽  
Mole Fraction ◽  
North Pacific ◽  
Atmospheric Oxygen ◽  
The United States ◽  
In Situ Observation ◽  
Airflow Rate ◽  
The North ◽  
The North Pacific

Abstract. Atmospheric oxygen (O2) and carbon dioxide (CO2) variations in the North Pacific were measured aboard a cargo ship, the New Century 2 (NC2), while it cruised between Japan and the United States between December 2015 and November 2016. A fuel cell analyzer and a nondispersive infrared analyzer were used for the measurement of O2 and CO2, respectively. To achieve parts-per-million precision for the O2 measurements, we precisely controlled the flow rates of the sample and reference air introduced into the analyzers and the outlet pressure. A relatively low airflow rate (10 cm3 min−1) was adopted to reduce the consumption rate of the reference gases. In the laboratory, the system achieved measurement precisions of 3.8 per meg for δ(O2 ∕ N2), which is commonly used to express atmospheric O2 variation, and 0.1 ppm for the CO2 mole fraction. After the in situ observation started aboard NC2, we found that the ship's motion caused false wavy variations in the O2 signal with an amplitude of more than several tens of ppm and a period of about 20 s. Although we have not resolved the problem at this stage, hourly averaging considerably suppressed the variation associated with ship motion. Comparison between the in situ observation and flask sampling of air samples aboard NC2 showed that the averaged differences (in situ–flask) and the standard deviations (±1σ) are −2.8 ± 9.4 per meg for δ(O2 ∕ N2) and −0.02 ± 0.33 ppm for the CO2 mole fraction. We compared 1 year of in situ data for atmospheric potential oxygen (APO; O2 +1.1×CO2) obtained from the broad middle-latitude region (140∘ E–130∘ W, 29∘ N–45∘ N) with previous flask sampling data from the North Pacific. This comparison showed that longitudinal differences in the seasonal amplitude of APO, ranging from 51 to 73 per meg, were smaller than the latitudinal differences.

scholarly journals On the Variability of the Circulation and Water Mass Properties in the Eastern Levantine Sea between September 2016–August 2017

Water ◽  
2019 ◽  
Vol 11 (9) ◽  
pp. 1741 ◽  
Author(s):  
Mauri ◽  
Sitz ◽  
Gerin ◽  
Poulain ◽  
Hayes ◽  
...  
Keyword(s):  
High Salinity ◽  
Autonomous Systems ◽  
Vertical Mixing ◽  
The North ◽  
Levantine Sea ◽  
Surface Circulation ◽  
Basin Scale ◽  
Geographical Position ◽  
Surface Drifters

The surface circulation and the thermohaline properties of the water masses of the eastern Levantine Sea (Mediterranean Sea) were monitored with mobile autonomous systems (surface drifters and gliders) during the period September 2016–August 2017. The drifters provided data for more than a year and revealed complex circulation features at scales ranging from the basin scale to the sub-mesoscale. Three drifters were captured in a semi-permanent gyre (Cyprus Eddy) allowing a quantitative study of its kinematics. During the experiment, three gliders were operated, in two different periods: September to December 2016 and February to March 2017. The autonomous instruments crossed the prevailing sub-basin structures several times. The collected in-situ observations were analyzed and interpreted in concert with remote sensing products (sea surface temperature and altimetry). The evolution of some of the prevailing features confirmed the complexity of the circulation of the basin. The Cyprus Eddy is the most persistent anticyclone, moving its geographical position and sometimes merging with the North Shikmona Eddy in a bigger structure. The gliders sampled this wide anticyclonic feature revealing its vertical structure in the two different periods. In fall, in stratified conditions, a high salinity core is evident below the thermocline. The isopycnals are characterized by an upward bending over the high salinity lens and a downward bending below it, typical of an anticyclonic modewater eddy. In winter, the core disappears following the vertical mixing that, homogenizes the upper Cyprus Eddy water down to 300 m.

scholarly journals Towards better error statistics for atmospheric inversions of methane surface fluxes

2013 ◽  
Vol 13 (14) ◽  
pp. 7115-7132 ◽  
Author(s):  
A. Berchet ◽  
I. Pison ◽  
F. Chevallier ◽  
P. Bousquet ◽  
S. Conil ◽  
...  
Keyword(s):  
Expert Knowledge ◽  
Transport Model ◽  
Vertical Mixing ◽  
Real Data ◽  
Surface Fluxes ◽  
Error Statistics ◽  
The North ◽  
Error Covariance ◽  
Methane Fluxes ◽  
General Statistical

Abstract. We adapt general statistical methods to estimate the optimal error covariance matrices in a regional inversion system inferring methane surface emissions from atmospheric concentrations. Using a minimal set of physical hypotheses on the patterns of errors, we compute a guess of the error statistics that is optimal in regard to objective statistical criteria for the specific inversion system. With this very general approach applied to a real-data case, we recover sources of errors in the observations and in the prior state of the system that are consistent with expert knowledge while inferred from objective criteria and with affordable computation costs. By not assuming any specific error patterns, our results depict the variability and the inter-dependency of errors induced by complex factors such as the misrepresentation of the observations in the transport model or the inability of the model to reproduce well the situations of steep gradients of concentrations. Situations with probable significant biases (e.g., during the night when vertical mixing is ill-represented by the transport model) can also be diagnosed by our methods in order to point at necessary improvement in a model. By additionally analysing the sensitivity of the inversion to each observation, guidelines to enhance data selection in regional inversions are also proposed. We applied our method to a recent significant accidental methane release from an offshore platform in the North Sea and found methane fluxes of the same magnitude than what was officially declared.

scholarly journals Turbulence and hypoxia contribute to dense zooplankton scattering layers in Patagonian Fjord System

2017 ◽  
Author(s):  
Iván Pérez-Santos ◽  
Leonardo Castro ◽  
Nicolás Mayorga ◽  
Lauren Ross ◽  
Luis Cubillos ◽  
...  
Keyword(s):  
Water Column ◽  
Vertical Mixing ◽  
Acoustic Doppler Current Profiler ◽  
Eddy Diffusivity ◽  
Future Research ◽  
Dense Layer ◽  
The North ◽  
Diel Vertical Migrations ◽  
And Migration

Abstract. The Puyuhuapi Fjord is an atypical fjord, with two mouths, located in northern Patagonia (44.7° S). One mouth lies to the south, close to the Pacific Ocean, whilst the second connects with the Jacaf Channel to the north where a shallow sill inhibits deep water ventilation contributing to the hypoxic conditions below ~ 100 m depth. Acoustic Doppler Current Profiler moorings, scientific echo sounder transects, and in-situ abundance measurements were used to study zooplankton assemblages and migration patterns along Puyuhuapi Fjord and Jacaf Channel. The acoustic records and in-situ zooplankton data revealed diel vertical migrations of siphonophores, euphausiids and copepods. A dense layer of zooplankton was observed along Puyuhuapi Fjord between the surface and the top of the hypoxic layer (~ 100 m), which acted as a physic-chemical barrier to the distribution and migration of the zooplankton. Aggregations of zooplankton and fishes were generally more abundant around the sill in Jacaf Channel than anywhere within Puyuhuapi Fjord. In particular, zooplanktons were distributed throughout the entire water column to ~ 200 m depth, with no evidence of a hypoxic boundary. Turbulence measurements taken near the sill in the Jacaf Channel indicated high turbulent kinetic energy dissipation rates (ε ~ 10−4 W kg−1) and vertical diapycnal eddy diffusivity (Kρ ~ 10−2 m2 s−1) values. These elevated vertical mixing ensures that the water column well oxygenated and promotes zooplanktons aggregation. The sill region represents a major topographic contrast between the two fjords, and we suggest that this is an feature for future research on carbon export and fluxes in these fjords.

Analysis of the impact of biomass burning emissions on global ozone production in the upper troposphere with MOCAGE CTM and IAGOS airborne data.

2020 ◽  
Author(s):  
Martin Cussac ◽  
Virginie Marécal ◽  
Valérie Thouret ◽  
Béatrice Josse
Keyword(s):  
Significant Role ◽  
Biomass Burning ◽  
Transport Model ◽  
Chemical Species ◽  
Ozone Production ◽  
In Situ Observation ◽  
Transport Pathway ◽  
Upper Troposphere ◽  
The Impact

&lt;p&gt;The UTLS (Upper Troposphere/Lower Stratosphere) is a key layer of the atmosphere as its chemical composition impacts both the troposphere and the stratosphere, and therefore plays a significant role in the climate system. Ozone at this altitude for instance plays a great role on surface temperature. Unlike in the stratosphere; it can be produced from the photolysis of precursors originating in the troposphere; mainly nitrous oxides (NO&lt;sub&gt;x&lt;/sub&gt;) and carbon monoxide (CO) at this pressure range. Biomass burning emissions in particular are likely to play a significant role in the quantities of these species in the upper troposphere and thus impacting ozone balance. This effect is investigated thanks to the global chemistry transport model MOCAGE. Because of the strong vertical gradients in this layer of the atmosphere, well resolved in-situ observation dataset are valuable for model evaluation. As of measurements used to validate MOCAGE results, IAGOS in-situ measurements from equipped commercial aircraft were chosen for their fine vertical resolution as well as their wide geographical coverage. Using both of these tools, upper tropospheric air composition is studied, with a focus on ozone precursors and production linked to biomass burning emissions.&lt;/p&gt;&lt;p&gt;Firstly is investigated the direct impact of biomass burning emissions on CO concentration in the upper troposphere, as it is both a good tracer of wildfire plumes in the atmosphere and it plays a role in the upper troposphere chemical balance. For this purpose MOCAGE simulations spaning over the year of 2013 where biomass burning emissions were turned on and off are compared to estimate a contribution to upper tropospheric CO. These simulations were validated using all the available data from the IAGOS database. It was found that biomass burning impacted CO levels globally, with the strongest enhancement happening above the most emitting areas (equatorial Africa and the Boreal forests). The importance of a fast vertical transport pathway above the fires was also highlighted with the possible occurrence of pyroconvection in addition to deep convection. Secondly, other chemical species related to ozone production were looked upon. Peroxyacetyl Nitrates (PAN) for instance were found to be impacted by biomass burning as it is a product of NOx oxidation as well as the main &quot;reservoir&quot; specie for NOx in the upper troposphere. Ultimately, ozone production resulting from biomass burning emissions is investigated, both in biomass burning plumes encountered by IAGOS aircraft, and on a more global scale using the MOCAGE simulations.&lt;/p&gt;

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