scholarly journals Impact of high-resolution <i>a priori</i> profiles on satellite-based formaldehyde retrievals

2017 ◽  
Author(s):  
Si-Wan Kim ◽  
Vijay Natraj ◽  
Seoyoung Lee ◽  
Hyeong-Ahn Kwon ◽  
Rokjin Park ◽  
...  
Keyword(s):  
Los Angeles ◽  
Urban Area ◽  
Temporal Resolution ◽  
A Priori ◽  
Measurement Data ◽  
Tropospheric Chemistry ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Los Angeles Basin ◽  
Model Calculations

Abstract. Formaldehyde (HCHO) is either directly emitted from sources or produced during the oxidation of volatile organic compounds in the troposphere. It is possible to infer atmospheric HCHO concentrations using space-based observations, which may be useful for studying emissions and tropospheric chemistry at urban to global scales depending on the quality of the retrievals. In the near future, an unprecedented volume of satellite-based HCHO measurement data will be available from both geostationary and polar-orbiting platforms. Therefore, it is essential to develop retrieval methods appropriate for the next-generation satellites that measure at higher spatial and temporal resolution than the current ones. In this study, we examine the importance of fine spatial and temporal resolution a priori profile information on the retrieval by conducting approximately 45 000 radiative transfer model calculations in the Los Angeles Basin megacity. Our analyses suggest that an air mass factor (AMF, ratio of slant columns to vertical columns) based on fine spatial and temporal resolution a priori profiles can better capture the spatial distributions of the enhanced HCHO plumes in an urban area than the nearly constant AMFs used for current operational products. For this urban area, the AMF values are inversely proportional to the magnitude of the HCHO mixing ratios in the boundary layer. Using our optimized model HCHO results in the Los Angeles Basin that mimic the HCHO retrievals from future geostationary satellites, we illustrate the effectiveness of HCHO data from geostationary measurements for understanding and predicting tropospheric ozone and its precursors.

scholarly journals Impact of high-resolution a priori profiles on satellite-based formaldehyde retrievals

2018 ◽  
Vol 18 (10) ◽  
pp. 7639-7655 ◽  
Author(s):  
Si-Wan Kim ◽  
Vijay Natraj ◽  
Seoyoung Lee ◽  
Hyeong-Ahn Kwon ◽  
Rokjin Park ◽  
...  
Keyword(s):  
Los Angeles ◽  
Urban Area ◽  
Temporal Resolution ◽  
A Priori ◽  
Measurement Data ◽  
Tropospheric Chemistry ◽  
Los Angeles Basin ◽  
Model Calculations ◽  
Mixing Ratios ◽  
Optimized Model

Abstract. Formaldehyde (HCHO) is either directly emitted from sources or produced during the oxidation of volatile organic compounds (VOCs) in the troposphere. It is possible to infer atmospheric HCHO concentrations using space-based observations, which may be useful for studying emissions and tropospheric chemistry at urban to global scales depending on the quality of the retrievals. In the near future, an unprecedented volume of satellite-based HCHO measurement data will be available from both geostationary and polar-orbiting platforms. Therefore, it is essential to develop retrieval methods appropriate for the next-generation satellites that measure at higher spatial and temporal resolution than the current ones. In this study, we examine the importance of fine spatial and temporal resolution a priori profile information on the retrieval by conducting approximately 45 000 radiative transfer (RT) model calculations in the Los Angeles Basin (LA Basin) megacity. Our analyses suggest that an air mass factor (AMF, a factor converting observed slant columns to vertical columns) based on fine spatial and temporal resolution a priori profiles can better capture the spatial distributions of the enhanced HCHO plumes in an urban area than the nearly constant AMFs used for current operational products by increasing the columns by ∼ 50 % in the domain average and up to 100 % at a finer scale. For this urban area, the AMF values are inversely proportional to the magnitude of the HCHO mixing ratios in the boundary layer. Using our optimized model HCHO results in the Los Angeles Basin that mimic the HCHO retrievals from future geostationary satellites, we illustrate the effectiveness of HCHO data from geostationary measurements for understanding and predicting tropospheric ozone and its precursors.

scholarly journals The inter-comparison of major satellite aerosol retrieval algorithms using simulated intensity and polarization characteristics of reflected light

2010 ◽  
Vol 3 (4) ◽  
pp. 909-932 ◽  
Author(s):  
A. A. Kokhanovsky ◽  
J. L. Deuzé ◽  
D. J. Diner ◽  
O. Dubovik ◽  
F. Ducos ◽  
...  
Keyword(s):  
A Priori ◽  
Light Polarization ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Retrieval Process ◽  
Retrieval Task ◽  
Major Satellite ◽  
Single View ◽  
Intensity Measurements ◽  
Priori Information

Abstract. Remote sensing of aerosol from space is a challenging and typically underdetermined retrieval task, requiring many assumptions to be made with respect to the aerosol and surface models. Therefore, the quality of a priori information plays a central role in any retrieval process (apart from the cloud screening procedure and the forward radiative transfer model, which to be most accurate should include the treatment of light polarization and molecular-aerosol coupling). In this paper the performance of various algorithms with respect to the of spectral aerosol optical thickness determination from optical spaceborne measurements is studied. The algorithms are based on various types of measurements (spectral, angular, polarization, or some combination of these). It is confirmed that multiangular spectropolarimetric measurements provide more powerful constraints compared to spectral intensity measurements alone, particularly those acquired at a single view angle and which rely on a priori assumptions regarding the particle phase function in the retrieval process.

scholarly journals HAMP – the microwave package on the High Altitude and LOng range research aircraft HALO

2014 ◽  
Vol 7 (5) ◽  
pp. 4623-4657
Author(s):  
M. Mech ◽  
E. Orlandi ◽  
S. Crewell ◽  
F. Ament ◽  
L. Hirsch ◽  
...  
Keyword(s):  
High Altitude ◽  
Long Range ◽  
Microwave Remote Sensing ◽  
Passive Microwave ◽  
Lower Atmosphere ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Model Calculations ◽  
Cloud Radar ◽  
Research Aircraft

Abstract. An advanced package of microwave remote sensing instrumentation has been developed for the operation on the new German High Altitude LOng range research aircraft (HALO). The HALO Microwave Package, HAMP, consists of two nadir looking instruments: a cloud radar at 36 GHz and a suite of passive microwave radiometers with 26 frequencies in different bands between 22.24 and 183.31 ± 12.5 GHz. We present a description of HAMP's instrumentation together with an illustration of its potential. To demonstrate this potential synthetic measurements for the implemented passive microwave frequencies and the cloud radar based on cloud resolving and radiative transfer model calculations were performed. These illustrate the advantage of HAMP's chosen frequency coverage, which allows for improved detection of hydrometeors both via the emission and scattering of radiation. Regression algorithms compare HAMP retrieval with standard satellite instruments from polar orbiters and show its advantages particularly for the lower atmosphere with a reduced root mean square error by 5 and 15% for temperature and humidity, respectively. HAMP's main advantage is the high spatial resolution of about 1 km which is illustrated by first measurements from test flights. Together these qualities make it an exciting tool for gaining better understanding of cloud processes, testing retrieval algorithms, defining future satellite instrument specifications, and validating platforms after they have been placed in orbit.

scholarly journals Ozone Monitoring Instrument spectral UV irradiance products: comparison with ground based measurements at an urban environment

2008 ◽  
Vol 8 (5) ◽  
pp. 17467-17493 ◽  
Author(s):  
S. Kazadzis ◽  
A. Bais ◽  
A. Arola ◽  
N. Krotkov ◽  
N. Kouremeti ◽  
...  
Keyword(s):  
Global Scale ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Ozone Monitoring Instrument ◽  
Model Calculations ◽  
Aerosol Absorption ◽  
Theoretical Approaches ◽  
Uv Irradiance ◽  
Ozone Monitoring ◽  
Comparison Period

Abstract. We have compared spectral ultraviolet overpass irradiances from the Ozone Monitoring Instruments (OMI) against ground-based Brewer measurements at Thessaloniki, Greece from September 2004 to December 2007. It is demonstrated that OMI overestimates UV irradiances by 30%, 17% and 13% for 305 nm, 324 nm, and 380 nm respectively and 20% for erythemally weighted irradiance. The bias between OMI and Brewer increases with increasing aerosol absorption optical thickness. We present methodologies that can be applied for correcting this bias based on experimental results derived from the comparison period and also theoretical approaches using radiative transfer model calculations. All correction approaches minimize the bias and the standard deviation of the ratio OMI versus Brewer ratio. According to the results, the best correction approach suggests that the OMI UV product has to be multiplied by a correction factor CA(λ) are in the order of 0.8, 0.88 and 0.9 for 305 nm, 324 nm and 380 nm respectively. Limitations and possibilities for applying such methodologies in a global scale are also discussed.

scholarly journals Temporal variations of microwave brightness temperatures over Antarctica

1994 ◽  
Vol 20 ◽  
pp. 19-25 ◽  
Author(s):  
I. Sherjal ◽  
M. Fily
Keyword(s):  
Satellite Data ◽  
A Priori ◽  
Temporal Variations ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Brightness Temperatures ◽  
Surface Temperatures ◽  
Air Temperatures ◽  
Microwave Imager ◽  
Snow Temperature

Passive microwave brightness temperatures from the Special Sensor Microwave Imager (SSMI) are studied together with surface air temperatures from two Automatic Weather Stations (AWS) for the year 1989. One station is located on the East Antarctic plateau (Dome C) and the other on the Ross lee Shelf (Lettau).The satellite data for frequencies 19, 22 and 37 GHz with vertical polarization,centered on the two AWS stations, are studied. A simple thermodynamic model and asimple radiative-transfer model, that takes into account the snow temperature profile and assumes a constant annual emissivity, are proposed. The combination of these two models enables us to compute extinction coefficients, penetration depths and toretrieve the measured brightness temperature variations from the AWS surface temperatures. Afterwards, this model is reversed in order to retrieve the snow-surface temperatures from the satellite data. Results are promising but strong approximationsand a priori knowledge of the extinction coefficient are still needed at this point.

Process-Based Decomposition of the Decadal Climate Difference between 2002–13 and 1984–95

2017 ◽  
Vol 30 (12) ◽  
pp. 4373-4393 ◽  
Author(s):  
Xiaoming Hu ◽  
Yana Li ◽  
Song Yang ◽  
Yi Deng ◽  
Ming Cai
Keyword(s):  
Radiative Transfer ◽  
Heat Storage ◽  
Decomposition Analysis ◽  
Arctic Region ◽  
The Arctic ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Model Calculations ◽  
Surface Warming ◽  
Decadal Climate

This study examines at the process level the climate difference between 2002–13 and 1984–95 in ERA-Interim. A linearized radiative transfer model is used to calculate the temperature change such that its thermal radiative cooling would balance the energy flux perturbation associated with the change of an individual process, without regard to what causes the change of the process in the first place. The global mean error of the offline radiative transfer model calculations is 0.09 K, which corresponds to the upper limit of the uncertainties from a single term in the decomposition analysis. The process-based decomposition indicates that the direct effect of the increase of CO2 (0.15 K) is the largest contributor to the global warming between the two periods (about 0.27 K). The second and third largest contributors are the cloud feedback (0.14 K) and the combined effect of the oceanic heat storage and evaporation terms (0.11 K), respectively. The largest warming associated with the oceanic heat storage term is found in the tropical Pacific and Indian Oceans, with relatively weaker warming over the tropical Atlantic Ocean. The increase in atmospheric moisture adds another 0.1 K to the global surface warming, but the enhancement in tropical convections acts to reduce the surface warming by 0.17 K. The ice-albedo and atmospheric dynamical feedbacks are the two leading factors responsible for the Arctic polar warming amplification (PWA). The increase of atmospheric water vapor over the Arctic region also contributes substantially to the Arctic PWA pattern.

scholarly journals Aerosol forcing efficiency in the UVA region from spectral solar irradiance measurements at an urban environment

2009 ◽  
Vol 27 (6) ◽  
pp. 2515-2522 ◽  
Author(s):  
S. Kazadzis ◽  
N. Kouremeti ◽  
A. Bais ◽  
A. Kazantzidis ◽  
C. Meleti
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Model Calculations ◽  
Aerosol Forcing ◽  
Aerosol Absorption ◽  
Absorbing Aerosols ◽  
Spectral Solar Irradiance ◽  
The City

Abstract. Spectral Ultraviolet (UV) measurements using a Brewer MKIII double spectroradiometer were used for the determination of the aerosol forcing efficiency (RFE) under cloud free conditions at Thessaloniki, Greece for the period 1998–2006. Using measured spectral UVA irradiance in combination with synchronous aerosol optical depth (AOD) measurements at 340 nm, we calculated the seasonal and the percent RFE changes with the help of radiative transfer model calculations used for cloud and aerosol free conditions reference. The calculated RFE for the 325–340 nm wavelength integral was found to be −0.71±0.30 W m−2/τs340 nm and corresponds to a mean calculated RFE% value of −15.2%±3.8% (2 σ) per unit of τs340 nm, for the whole period. This indicates a mean reduction of 15.2% of the 325–340 nm irradiance for a unit of aerosol optical depth slant column increase. Lower RFE% was found during summertime, which is a possible indication of lower absorbing aerosols. Mean AOD slant at 340 nm for the city of Thessaloniki were processed in combination with RFE% and a mean monthly UVA attenuation of ~10% for the whole period was revealed. The nine years' analysis results showed a reduction in RFE%, which provides a possible indication of the changes in the optical properties over the city area. If such changes are only due to changes in the aerosol absorbing properties, the above finding suggests a 2% per decade increase in UVA due to changes in the aerosol absorption properties, in addition to the calculated increase by 4.2%, which is attributed only to AOD decrease at Thessaloniki area over the 1998–2006 period.

scholarly journals Ozone Monitoring Instrument spectral UV irradiance products: comparison with ground based measurements at an urban environment

2009 ◽  
Vol 9 (2) ◽  
pp. 585-594 ◽  
Author(s):  
S. Kazadzis ◽  
A. Bais ◽  
A. Arola ◽  
N. Krotkov ◽  
N. Kouremeti ◽  
...  
Keyword(s):  
Global Scale ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Ozone Monitoring Instrument ◽  
Model Calculations ◽  
Aerosol Absorption ◽  
Theoretical Approaches ◽  
Uv Irradiance ◽  
Ozone Monitoring ◽  
Comparison Period

Abstract. We have compared spectral ultraviolet overpass irradiances from the Ozone Monitoring Instruments (OMI) against ground-based Brewer measurements at Thessaloniki, Greece from September 2004 to December 2007. It is demonstrated that OMI overestimates UV irradiances by 30%, 17% and 13% for 305 nm, 324 nm, and 380 nm respectively and 20% for erythemally weighted irradiance. The bias between OMI and Brewer increases with increasing aerosol absorption optical thickness. We present methodologies that can be applied for correcting this bias based on experimental results derived from the comparison period and also theoretical approaches using radiative transfer model calculations. All correction approaches minimize the bias and the standard deviation of the ratio OMI versus Brewer ratio. According to the results, the best correction approach suggests that the OMI UV product has to be multiplied by a correction factor CA(λ) of the order of 0.8, 0.88 and 0.9 for 305 nm, 324 nm and 380 nm respectively. Limitations and possibilities for applying such methodologies in a global scale are also discussed.

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