scholarly journals Device Engineering for All-Inorganic Perovskite Light-Emitting Diodes

Nanomaterials ◽  
2019 ◽  
Vol 9 (7) ◽  
pp. 1007 ◽  
Author(s):  
Dongxiang Luo ◽  
Qizan Chen ◽  
Ying Qiu ◽  
Menglong Zhang ◽  
Baiquan Liu

Recently, all-inorganic perovskite light-emitting diodes (PeLEDs) have attracted both academic and industrial interest thanks to their outstanding properties, such as high efficiency, bright luminance, excellent color purity, low cost and potentially good operational stability. Apart from the design and treatment of all-inorganic emitters, the device engineering is another significant factor to guarantee the high performance. In this review, we have summarized the state-of-the-art concepts for device engineering in all-inorganic PeLEDs, where the charge injection, transport, balance and leakage play a critical role in the performance. First, we have described the fundamental concepts of all-inorganic PeLEDs. Then, we have introduced the enhancement of device engineering in all-inorganic PeLEDs. Particularly, we have comprehensively highlighted the emergence of all-inorganic PeLEDs, strategies to improve the hole injection, approaches to enhance the electron injection, schemes to increase the charge balance and methods to decrease the charge leakage. Finally, we have clarified the issues and ways to further enhance the performance of all-inorganic PeLEDs.

2019 ◽  
Vol 33 (24) ◽  
pp. 1950284
Author(s):  
Nan Zhang ◽  
Yang Chen ◽  
Yan-Hui Wang

It has been demonstrated that high efficiency and brightness can be achieved in phosphorescent organic light-emitting diodes (PHOLEDs) by using molybdenum oxide (MoO3)/poly(3,4-ethylenedioxythiophene) poly(styrenesulfonate) (PEDOT:PSS) as dual hole injection layers (HILs) on indium tin oxide (ITO) substrate. The dual HILs were simply fabricated by spin-coating PEDOT:PSS solution on a thin MoO3 layer deposited by vacuum thermal evaporation. This work reveals that PEDOT:PSS coating on MoO3 resulted in a smoother surface, simultaneously MoO3 lamella prevented acid corrosion of PEDOT:PSS on ITO. Meanwhile, with the insertion of PEDOT:PSS and MoO3 as HILs between anode and hole transporting layer (HTL), the energy barrier has been reduced and gave rise to effective hole injection. OLEDs with dual HILs resulted in the maximum current efficiency (CE) of 61.3 cd A[Formula: see text] and maximum luminance of 112200 cd cm[Formula: see text], which showed a superior performance compared to those devices with single HIL of PEDOT:PSS or MoO3. Our results proved the composition of PEDOT:PSS and MoO3 as HILs were beneficial for high performance OLEDs.


2012 ◽  
Vol 13 (5) ◽  
pp. 796-806 ◽  
Author(s):  
Maria Vasilopoulou ◽  
George Papadimitropoulos ◽  
Leonidas C. Palilis ◽  
Dimitra G. Georgiadou ◽  
Panagiotis Argitis ◽  
...  

2019 ◽  
Author(s):  
Baiquan Liu ◽  
Yemliha Altintas ◽  
Lin Wang ◽  
Sushant Shendre ◽  
Manoj Sharma ◽  
...  

<p> Colloidal quantum wells (CQWs) are regarded as a new, highly promising class of optoelectronic materials thanks to their unique excitonic characteristics of high extinction coefficient and ultranarrow emission bandwidth. Although the exploration of CQWs in light-emitting diodes (LEDs) is impressive, the performance of CQW-LEDs lags far behind compared with other types of LEDs (e.g., organic LEDs, colloidal quantum-dot LEDs, and perovskite LEDs). Herein, for the first time, the authors show high-efficiency CQW-LEDs reaching close to the theoretical limit. A key factor for this high performance is the exploitation of hot-injection shell (HIS) growth of CQWs, which enables a near-unity photoluminescence quantum yield (PLQY), reduces nonradiative channels, ensures smooth films and enhances the stability. Remarkably, the PLQY remains 95% in solution and 87% in film despite rigorous cleaning. Through systematically understanding their shape-, composition- and device- engineering, the CQW-LEDs using CdSe/Cd<sub>0.25</sub>Zn<sub>0.75</sub>S core/HIS CQWs exhibit a maximum external quantum efficiency of 19.2%. Additionally, a high luminance of 23,490 cd m<sup>-2</sup>, extremely saturated red color with the Commission Internationale de L’Eclairage coordinates of (0.715, 0.283) and stable emission are obtained. The findings indicate that HIS grown CQWs enable high-performance solution-processed LEDs, which may pave the path for CQW-based display and lighting technologies.</p>


Nanoscale ◽  
2019 ◽  
Vol 11 (11) ◽  
pp. 5021-5029 ◽  
Author(s):  
Qasim Khan ◽  
Alagesan Subramanian ◽  
Guannan Yu ◽  
Khan Maaz ◽  
Delong Li ◽  
...  

Although all-inorganic perovskite light emitting diodes (PeLED) have satisfactory stability under an ambient atmosphere, producing devices with high performance is challenging.


2019 ◽  
Vol 75 (12) ◽  
pp. 1033-1037
Author(s):  
Jae Seung Shin ◽  
Jong Hun Yu ◽  
Su Been Heo ◽  
Seong Jun Kang

2018 ◽  
Vol 6 (40) ◽  
pp. 10793-10803 ◽  
Author(s):  
Shian Ying ◽  
Dezhi Yang ◽  
Xianfeng Qiao ◽  
Yanfeng Dai ◽  
Qian Sun ◽  
...  

High-performance WOLEDs realizing high efficiency and low efficiency roll-off simultaneously were achieved by strategically managing triplet excitons in the emission layer.


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