scholarly journals Influences of Ga Doping on Crystal Structure and Polarimetric Pattern of SHG in ZnO Nanofilms

Nanomaterials ◽  
2019 ◽  
Vol 9 (6) ◽  
pp. 905 ◽  
Author(s):  
Hua Long ◽  
Ammar Habeeb ◽  
Dickson Kinyua ◽  
Kai Wang ◽  
Bing Wang ◽  
...  
Keyword(s):  
Crystal Structure ◽  
Second Harmonic ◽  
Incident Light ◽  
Light Polarization ◽  
Nonlinear Susceptibility ◽  
Polarization Angle ◽  
Doped Zno ◽  
Non Destructive ◽  
Ga Doping ◽  
Sensitive Method

The second-harmonic generation (SHG) in gallium doped ZnO (GZO) nanofilms was studied. The Ga doping in GZO nanofilms influenced the crystal structure of the films, which affected SHG characteristics of the nanofilms. In our experiments, a strong SHG response was obtained in GZO nanofilms, which was excited by 790 nm femtosecond laser. It was observed that the Ga doping concentrations affected, not only the intensity, but also the polarimetric pattern of SHG in GZO nanofilms. For 5.0% doped GZO films, the SHG intensity increased about 70%. The intensity ratio of SHG between the incident light polarization angle of 90° and 0°changed with the Ga doping concentrations. It showed the most significant increase for 7.3% doped GZO films, with an increased ratio of c/a crystal constants. This result was attributed to the differences of the ratios of d33/d31 (the second-order nonlinear susceptibility components) induced by the crystal distortion. The results are helpful to investigate nanofilms doping levels and crystal distortion by SHG microscopy, which is a non-destructive and sensitive method.

Local Crystal Orientation in Laser Annealed Silicon Using a Raman Microprobe

1983 ◽  
Vol 29 ◽  
Author(s):  
L. A. Farrow ◽  
J.B. Hopkins ◽  
G J Fisanick
Keyword(s):  
Crystal Structure ◽  
Raman Scattering ◽  
Crystal Orientation ◽  
Polarization Angle ◽  
Substrate Plane ◽  
Si Substrate ◽  
Intensity Measurements ◽  
Raman Microprobe ◽  
Destructive Analysis ◽  
Non Destructive

ABSTRACTIn this paper, we discuss the application of polarization selective Raman microprobe spectroscopy to the detailed, non-destructive analysis of the local crystal orientation of a polysilicon sample grown over SiO 2 pads and laser annealed. Intensity measurements taken as a function of input polarization angle are fit to an expression derived from the Raman scattering selection rules to calculate the angles by which the crystal structure is twisted within the original substrate plane, as well as the degree of tipping of the crystal plane away from the plane of the Si substrate. The results give some indication as to the direction of seeding during recrystallization.

scholarly journals Rational Design and Simulation of Two-Dimensional Perovskite Photonic Crystal Absorption Layers Enabling Improved Light Absorption Efficiency for Solar Cells

Energies ◽  
2021 ◽  
Vol 14 (9) ◽  
pp. 2460
Author(s):  
Jian Zou ◽  
Mengnan Liu ◽  
Shuyu Tan ◽  
Zhijie Bi ◽  
Yong Wan ◽  
...  
Keyword(s):  
Crystal Structure ◽  
Solar Cells ◽  
Photonic Crystal ◽  
Incident Light ◽  
Absorption Efficiency ◽  
Utilization Efficiency ◽  
Photonic Crystal Structure ◽  
Two Dimensional ◽  
Photoelectric Conversion ◽  
Absorption Layer

A two-dimensional perovskite photonic crystal structure of Methylamine lead iodide (CH3NH3PbI3, MAPbI3) is rationally designed as the absorption layer for solar cells. The photonic crystal (PC) structure possesses the distinct “slow light” and band gap effect, leading to the increased absorption efficiency of the absorption layer, and thus the increased photoelectric conversion efficiency of the battery. Simulation results indicate that the best absorption efficiency can be achieved when the scattering element of indium arsenide (InAs) cylinder is arranged in the absorption layer in the form of tetragonal lattice with the height of 0.6 μm, the diameter of 0.24 μm, and the lattice constant of 0.4 μm. In the wide wavelength range of 400–1200 nm, the absorption efficiency can be reached up to 82.5%, which is 70.1% higher than that of the absorption layer without the photonic crystal structure. In addition, the absorption layer with photonic crystal structure has good adaptability to the incident light angle, presenting the stable absorption efficiency of 80% in the wide incident range of 0–80°. The results demonstrate that the absorption layer with photonic crystal structure can realize the wide spectrum, wide angle, and high absorption of incident light, resulting in the increased utilization efficiency of solar energy.

scholarly journals Anomalously Strong Second‐Harmonic Generation in GaAs Nanowires via Crystal‐Structure Engineering

2021 ◽  
pp. 2104671
Author(s):  
Bin Zhang ◽  
Jan E. Stehr ◽  
Ping‐Ping Chen ◽  
Xingjun Wang ◽  
Fumitaro Ishikawa ◽  
...  
Keyword(s):  
Crystal Structure ◽  
Second Harmonic Generation ◽  
Harmonic Generation ◽  
Second Harmonic ◽  
Gaas Nanowires ◽  
Structure Engineering

Enhancement of second harmonic generation using a novel asymmetric metal–graphene–insulator–metal plasmonic waveguide

2018 ◽  
Vol 27 (01) ◽  
pp. 1850003 ◽  
Author(s):  
Mohamadreza Soltani
Keyword(s):  
Second Harmonic Generation ◽  
Harmonic Generation ◽  
Nonlinear Optical ◽  
Second Harmonic ◽  
Field Enhancement ◽  
The Other ◽  
Nonlinear Susceptibility ◽  
Optical Process ◽  
Large Enhancement ◽  
Nonlinear Optical Process

Here, we propose a novel plasmonic structure, called asymmetric plasmonic nanocavity grating (APNCG), which is shown to dramatically enhance nonlinear optical process of second harmonic generation (SHG). The proposed structure consists of two different metals on both sides of lithium niobate and a thin layer of graphene. By using two different metals the nonlinear susceptibility of the waveguide would be increased noticeably causing to increase SHG. On the other hand, it consists of two identical gratings on one side. By two identical gratings, the pump beam is coupled to two opposing SPP waves, which interfere with each other and result in SPP standing wave in the region between the two gratings. The distance between two gratings will be optimized to reach the highest SHG. It will be shown that by optimizing the geometry of proposed structure and using different metals, field enhancement in APNCG waveguides can result in large enhancement of SHG.

scholarly journals A Molecular Architectural Approach to Second-Order Nonlinear Optical Materials

1995 ◽  
Vol 392 ◽  
Author(s):  
Xiaoguang Yang ◽  
Duncan McBranch ◽  
Basil Swanson ◽  
Dequan Li
Keyword(s):  
Nonlinear Optical ◽  
Second Harmonic ◽  
Fused Silica ◽  
Second Order ◽  
Nonlinear Susceptibility ◽  
Design And Synthesis ◽  
Fundamental Wavelength ◽  
Assembled Monolayers ◽  
Methylene Groups ◽  
Nlo Chromophores

AbstractThe design and synthesis of a family of calix[4]arene-based nonlinear optical (NLO) chromophores are discussed. The calixarene chromophores are macrocyclic compounds consisting of four simple D-π-A units bridged by methylene groups. These molecules were synthesized such that four D-π-A units of the calix[4]arene were aligned along the same direction with the calixarene in a cone conformation. These nonlinear optical super-chromophores were subsequently fabricated into covalently bound self-assembled monolayers on the surfaces of fused silica and silicon. Spectroscopic second harmonic generation (SHG) measurements were carried out to determine the absolute value of the dominant element of the second-order nonlinear susceptibility, d33, and the average molecular alignment, ψ. We find a value of d33 = 60 pm/V at a fundamental wavelength of 890 nm, and ψ˜ 36° with respect to the surface normal.

scholarly journals Novel Two-Dimensional Layered MoSi2Z4 (Z = P, As): New Promising Optoelectronic Materials

Nanomaterials ◽  
2021 ◽  
Vol 11 (3) ◽  
pp. 559
Author(s):  
Hui Yao ◽  
Chao Zhang ◽  
Qiang Wang ◽  
Jianwei Li ◽  
Yunjin Yu ◽  
...  
Keyword(s):  
Optical Absorption ◽  
Incident Light ◽  
Optoelectronic Devices ◽  
Large Family ◽  
Middle Layer ◽  
Optoelectronic Device ◽  
First Principles Calculation ◽  
Polarization Angle ◽  
Two Dimensional ◽  
Conducting Materials

Very recently, two new two-dimensional (2D) layered semi-conducting materials MoSi2N4 and WSi2N4 were successfully synthesized in experiments, and a large family of these two 2D materials, namely MA2Z4, was also predicted theoretically (Science, 369, 670 (2020)). Motivated by this exciting family, in this work, we systematically investigate the mechanical, electronic and optical properties of monolayer and bilayer MoSi2P4 and MoSi2As4 by using the first-principles calculation method. Numerical results indicate that both monolayer and bilayer MoSi2Z4 (Z = P, As) present good structural stability, isotropic mechanical parameters, moderate bandgap, favorable carrier mobilities, remarkable optical absorption, superior photon responsivity and external quantum efficiency. Especially, due to the wave-functions of band edges dominated by d orbital of the middle-layer Mo atoms are screened effectively, the bandgap and optical absorption hardly depend on the number of layers, providing an added convenience in the experimental fabrication of few-layer MoSi2Z4-based electronic and optoelectronic devices. We also build a monolayer MoSi2Z4-based 2D optoelectronic device, and quantitatively evaluate the photocurrent as a function of energy and polarization angle of the incident light. Our investigation verifies the excellent performance of a few-layer MoSi2Z4 and expands their potential application in nanoscale electronic and optoelectronic devices.

scholarly journals Reflective second harmonic generation near resonance in the epitaxial Al-doped ZnO thin film

2007 ◽  
Vol 15 (17) ◽  
pp. 10666 ◽  
Author(s):  
S. W. Liu ◽  
J. L. Weerasinghe ◽  
J. Liu ◽  
J. Weaver ◽  
C. L. Chen ◽  
...  
Keyword(s):  
Thin Film ◽  
Second Harmonic Generation ◽  
Harmonic Generation ◽  
Second Harmonic ◽  
Zno Thin Film ◽  
Near Resonance ◽  
Doped Zno

scholarly journals L-alaninium perrhenate: crystal structure and non-linear optical properties

2014 ◽  
Vol 12 (10) ◽  
pp. 1016-1022 ◽  
Author(s):  
Vitor Rodrigues ◽  
Maria Costa ◽  
Etelvina Gomes ◽  
Dmitry Isakov ◽  
Michael Belsley
Keyword(s):  
Crystal Structure ◽  
Optical Properties ◽  
Second Harmonic ◽  
Negative Ions ◽  
Damage Threshold ◽  
Linear Optics ◽  
Second Harmonic Generation Efficiency ◽  
Non Linear ◽  
Linear Optical Properties ◽  
Linear Optical

AbstractThe crystal structure and non-linear optical properties of L-alaninium perrhenate, C3H8NO2+ ReO4 −, are reported. The protonated amino acid and the perrhenate anion have their usual geometries. The three-dimensional hydrogen-bonded network can be seen as a stacking of layers parallel to the (100) planes. Each layer is formed by chains of alternating positive and negative ions along the b and c axes. Hydrogen bonding of adjacent layers forms alternating chains along the a axis. A high damage threshold and a second-harmonic generation efficiency three times that of KDP make this new material potentially useful in non-linear optics.

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