scholarly journals Oxy-Fuel Combustion Characteristics of Pulverized Coal under O2/Recirculated Flue Gas Atmospheres

2020 ◽  
Vol 10 (4) ◽  
pp. 1362
Author(s):  
Shuhn-Shyurng Hou ◽  
Chiao-Yu Chiang ◽  
Ta-Hui Lin

Oxy-fuel combustion is an effective technology for carbon capture and storage (CCS). Oxy-combustion for coal-fired power stations is a promising technology by which to diminish CO2 emissions. Unfortunately, little attention has been paid to the oxy-combustion characteristics affected by the combustion atmosphere. This paper is aimed at investigating the oxy-fuel combustion characteristics of Australian coal in a 0.3 MWth furnace. In particular, the influences of various oxygen flow rates and recirculated flue gas (RFG) on heating performance and pollutant emissions are examined in O2/RFG environments. The results show that with increases in the secondary RFG flow rate, the temperatures in the radiative and convective sections decrease and increase, respectively. At a lower oxygen flow rate, burning Australian coal emits lower residual oxygen and NO concentrations. In the flue gas, a high CO2 concentration of up to 94.8% can be achieved. Compared to air combustion, NO emissions are dramatically reduced up to 74% for Australian coal under oxy-combustion. Note that the high CO2 concentrations in the flue gas under oxy-coal combustions suggest great potential for reducing CO2 emissions through carbon capture and storage.

Author(s):  
Tamilselvi Dananjayan Rushendra Revathy ◽  
Andimuthu Ramachandran ◽  
Kandasamy Palanivelu

Materials ◽  
2019 ◽  
Vol 12 (13) ◽  
pp. 2088 ◽  
Author(s):  
Elizabeth Rodriguez Acevedo ◽  
Farid B. Cortés ◽  
Camilo A. Franco ◽  
Francisco Carrasco-Marín ◽  
Agustín F. Pérez-Cadenas ◽  
...  

The implementation of carbon capture and storage process (CCS) has been unsuccessful to date, mainly due to the technical issues and high costs associated with two main stages: (1) CO2 separation from flue gas and (2) CO2 injection in deep geological deposits, more than 300 m, where CO2 is in supercritical conditions. This study proposes, for the first time, an enhanced CCS process (e-CCS), in which the stage of CO2 separation is removed and the flue gas is injected directly in shallow reservoirs located at less than 300 m, where the adsorptive phenomena control CO2 storage. Nitrogen-rich carbon nanospheres were used as modifying agents of the reservoir porous texture to improve both the CO2 adsorption capacity and selectivity. For this purpose, sandstone was impregnated with a nanofluid and CO2 adsorption was evaluated at different pressures (atmospheric pressure and from 3 × 10−3 MPa to 3.0 MPa) and temperatures (0, 25, and 50 °C). As a main result, a mass fraction of only 20% of nanomaterials increased both the surface area and the molecular interactions, so that the increase of adsorption capacity at shallow reservoir conditions (50 °C and 3.0 MPa) was more than 677 times (from 0.00125 to 0.9 mmol g−1).


2011 ◽  
Vol 347-353 ◽  
pp. 1479-1482 ◽  
Author(s):  
Pu Peng ◽  
Yi Zhuang

The CO2 capturing technologies as applied to FCC flue gas in order to reduce GHG (green house gases) were evaluated and compared in this review. Although the CCS (carbon capture and storage) idea has been proposed for more than 30 years, there has been little commercial success of CCS projects. The largest issue is where to store the massive amount of captured pure CO2 every year. Therefore, the review will focus on the efficient use of power or heat to reduce CO2 emission and how to recycle the use of produced CO2 before it is emitted to the atmosphere rather than being captured and stored. The scenarios with oxyfiring, microalgae-cofiring or biogas burning to treat FCC flue gas are introduced and discussed.


2006 ◽  
Vol 46 (1) ◽  
pp. 435
Author(s):  
B. Hooper ◽  
B. Koppe ◽  
L. Murray

The Latrobe Valley in Victoria’s Gippsland Basin is the location of one of Australia’s most important energy resources—extremely thick, shallow brown coal seams constituting total useable reserves of more than 50,000 million tonnes. Brown coal has a higher moisture content than black coal and generates more CO2 emissions per unit of useful energy when combusted. Consequently, while the Latrobe Valley’s power stations provide Australia’s lowest- cost bulk electricity, they are also responsible for over 60 million tonnes of CO2 emissions per year—over half of the Victorian total. In an increasingly carbon constrained world the ongoing development of the Latrobe Valley brown coal resource is likely to require a drastic reduction in the CO2 emissions from new coal use projects—and carbon capture and storage (CCS) has the potential to meet such deep cuts. The offshore Gippsland Basin, the site of major producing oil and gas fields, has the essential geological characteristics to provide a high-volume, low-cost site for CCS. The importance of this potential to assist the continuing use of the nation’s lowest-cost energy source prompted the Australian Government to fund the Latrobe Valley CO2 Storage Assessment (LVCSA).The LVCSA proposal was initiated by Monash Energy (formerly APEL, and now a 100% subsidiary of Anglo American)—the proponent of a major brown coal-to-liquids plant in the Latrobe Valley. Monash Energy’s plans for the 60,000 BBL per day plant include CCS to store about 13 million tonnes of CO2 per year. The LVCSA, undertaken for Monash Energy by the Cooperative Research Centre for Greenhouse Gas Technologies (CO2CRC), provides a medium to high-level technical and economic characterisation of the volume and cost potential for secure geosequestration of CO2 produced by the use of Latrobe Valley brown coal (Hooper et al, 2005a). The assessment’s scope includes consideration of the interaction between CO2 injection and oil and gas production, and its findings have been publicly released for use by CCS proponents, oil and gas producers and all other interested parties as an executive summary, (Hooper et al, 2005b), a fact sheet (Hooper et al, 2005c) and a presentation (Hooper et al, 2005d)).The LVCSA identifies the key issues and challenges for implementing CCS in the Latrobe Valley and provides a reference framework for the engagement of stakeholders. In effect the LVCSA constitutes a pre-feasibility study for the implementation of geosequestration in support of the continuing development of Victoria’s brown coal resources.The LVCSA findings indicate that the Gippsland Basin has sufficient capacity to safely and securely store large volumes of CO2 and may provide a viable means of substantially reducing greenhouse gas emissions from coal-fired power plants and other projects using brown coal in the Latrobe Valley. The assessment also indicates that CO2 injection could well be designed to avoid any adverse impact on adjacent oil and gas production, so that CO2 injection can begin near fields that have not yet come to the end of their productive lives. However, CCS proposals involving adjacent injection and production will require more detailed risk management strategies and continuing cooperation between prospective injectors and existing producers.


2020 ◽  
pp. 100608
Author(s):  
Congbin Xu ◽  
Jingjing Yang ◽  
Li He ◽  
Wenxia Wei ◽  
Yong Yang ◽  
...  

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