scholarly journals Spent fuel performance data: An analysis of data relevant to the NNWSI Project

10.2172/60649 ◽  
1987 ◽  
Author(s):  
V.M. Oversby ◽  
H.F. Shaw
Author(s):  
Edward M. Duchnowski ◽  
Seokbin Seo ◽  
Nicholas R. Brown

Abstract During operation of light water reactors hydrogen from the primary coolant is absorbed within the zirconium cladding and is able to migrate and redistribute within the cladding. The hydrogen in solid solution is able to precipitate, forming zirconium hydrides which results in a decrease of ductility of the cladding and ultimately an increase in likelihood of cladding failure, especially in conditions such as transport or storage of nuclear fuel rods. In collaboration with other universities, industries, and national laboratories the overarching goal of this project is to enhance the development for modeling hydride behavior to be implemented into the BISON fuel performance tool. The University of Tennessee-Knoxville (UTK) has been tasked with quantifying the uncertainty in the models developed within this project as well as quantifying the sensitivity to the most significant parameters of uncertainty. The BISON fuel performance code has been shown to overpredict the total concentration of hydrogen at cold regions of a temperature profile, thus a sensitivity study was performed to quantify the impact that key diffusion parameters have on the local concentration of hydrogen at the cold end of a 1-D model subjected to an asymmetric temperature profile. It is shown within this document that the diffusion activation energy and the pre-exponential factor, values within the diffusion coefficient of hydrogen, have a large impact on the local concentration of hydrogen and their importance increases for an increase in annealing time.


2006 ◽  
Vol 932 ◽  
Author(s):  
Christophe Poinssot ◽  
Cécile Ferry ◽  
Bernd Grambow ◽  
Manfred Kelm ◽  
Kastriot Spahiu ◽  
...  

ABSTRACTEuropean Commission supported a wide research project entitled “Spent Fuel Stability under repository conditions” (SFS) within the 5th FWP, the aim of which was to develop a common understanding of the radionuclides release from spent nuclear fuel in geological disposal and build a RN release model in order to assess the fuel performance. This project achieved by the end of 2004 focuses both on the Instant Release Fraction (IRF) model and the Matrix Alteration Model (MAM).A new IRF model was developed based on the anticipated performances of the various fuel microstructures (gap, rim, grains boundaries) and the potential diffusion of RN before the canister breaching. However, this model lets the choice to the end-user about the degree of conservativeness to consider.In addition, fuel alteration has been demonstrated to be linked to the production of radiolytic oxidants by water radiolysis at the fuel interface, the oxidation of the fuel interface by radiolytic oxidants and the subsequent release of uranium under the influence of aqueous ligands. A large set of experimental data was therefore acquired in order (i) to upgrade the current radiolytic kinetic scheme, (ii) to experimentally correlate the fuel alteration rate and the fuel specific alpha activity by performing experiments on alpha doped samples, (iii) to experimentally test the potential inhibitor effect of hydrogen on fuel dissolution. Based on these results, a new MAM was developed, which was also calibrated using the experiments on inactive UO2 samples. This model was finally applied to representative granitic, salt and clayey environment to predict spent fuel long-term fuel performance.


1994 ◽  
Vol 353 ◽  
Author(s):  
F. B. Neall ◽  
P. Baertschi ◽  
I.G. McKinley ◽  
P. A. Smith ◽  
T. Sumerling ◽  
...  

Integrated performance assessments of proposed repositories for HLW involve multidisciplinary studies which include identification of possible paths of future evolution of the repository system (scenario analysis) and quantification of the consequences of each scenario using deterministic or probabilistic modelling approaches. The results of such studies are commonly presented as estimates of consequence (e.g. dose to a representative individual) against time which extends into the distant future. Individual components of the model chains used can be tested to some extent, but how can the integrated assessment be evaluated to give additional confidence in the overall results? In order to address this issue, the Kristallin-l performance assessmentI has been compared with other HLW/spent fuel performance assessments. This technical comparison forms the basis of this paper which summarises the results from a more extensive comparison of a number of HLW/spent fuel disposal concepts, safety assessment methodologies and models2. It is part of a wider study which attempted to put the results of the Kristallin-I performance assessment into perspective by use of both this technical comparison with other performance assessments and by consideration of other information (e.g. natural analogue studies, environmental radiation data and risk assessments for radiological and non-radiological hazards) which allows the reasonableness of the results and significance of the predicted doses to be illustrated. Due to limitations of space, this aspect of the study has not been included here and the reader is referred to the “Kristallin-I: Results in Perspective” report2 for more details.


Sign in / Sign up

Export Citation Format

Share Document