scholarly journals Seasonal and interannual variations in the propagation of photosynthetically available radiation through the Arctic atmosphere

Elem Sci Anth ◽  
2021 ◽  
Vol 9 (1) ◽  
Author(s):  
J. Laliberté ◽  
S. Bélanger ◽  
M. Babin
Keyword(s):  
Large Data ◽  
The Arctic ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
The Sun ◽  
Photosynthetically Available Radiation ◽  
Data Set ◽  
Melt Ponds ◽  
Arctic Atmosphere ◽  
Marine Productivity

The Arctic atmosphere–surface system transmits visible light from the Sun to the ocean, determining the annual cycle of light available to microalgae. This light is referred to as photosynthetically available radiation (PAR). A known consequence of Arctic warming is the change at the atmosphere–ocean interface (longer ice-free season, younger ice), implying an increase in the percentage of PAR being transferred to the water. However, much less is known about the recent changes in how much PAR is being transferred by the overlaying atmosphere. We studied the transfer of PAR through the atmosphere between May 21 and July 23 at a pan-Arctic scale for the period ranging from 2000 to 2016. By combining a large data set of atmospheric and surface conditions into a radiative transfer model, we computed the percentage of PAR transferred to the surface. We found that typical Arctic atmospheres convey between 60% and 70% of the incident PAR received from the Sun, meaning the Arctic atmosphere typically transmits more light than most sea ice surfaces, with the exception of mature melt ponds. We also found that the transfer of PAR through the atmosphere decreased at a rate of 2.3% per decade over the studied period, due to the increase in cloudiness and the weaker radiative interaction between the atmosphere and the surface. Further investigation is required to address how, in the warmer Arctic climate, this negative trend would compensate for the increased surface transmittance and its consequences on marine productivity.

scholarly journals A synthetic data set of high-spectral resolution infrared spectra for the Arctic atmosphere

2016 ◽  
Author(s):  
C. J. Cox ◽  
P. M. Rowe ◽  
S. P. Neshyba ◽  
V. P. Walden
Keyword(s):  
Remote Sensing ◽  
Radiative Transfer ◽  
Infrared Spectra ◽  
Spectral Resolution ◽  
High Spectral Resolution ◽  
The Arctic ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Data Set ◽  
Atmospheric State

Abstract. Retrievals of cloud microphysical and macrophysical properties from ground-based and satellite-based infrared remote sensing instruments are critical for understanding clouds. However, retrieval uncertainties are difficult to quantify without a standard for comparison. This is particularly true over the polar regions where surface-based data for a cloud climatology are sparse, yet clouds represent a major source of uncertainty in weather and climate models. We describe a synthetic high-spectral resolution infrared data set that is designed to facilitate validation and development of cloud retrieval algorithms for surface- and satellite-based remote sensing instruments. Since the data set is calculated using pre-defined cloudy atmospheres, the properties of the cloud and atmospheric state are known a priori. The atmospheric state used for the simulations is drawn from radiosonde measurements made at the North Slope of Alaska (NSA) Atmospheric Radiation Measurement (ARM) site at Barrow, Alaska (71.325° N, 156.615° W), a location that is generally representative of the western Arctic. The cloud properties for each simulation are selected from statistical distributions derived from past field measurements. Upwelling (at 60 km) and downwelling (at the surface) infrared spectra are simulated for 222 cloudy cases from 50–3000 cm−1 (3.3 to 200 μm) at monochromatic (line-by-line) resolution at a spacing of ~ 0.01 cm−1 using the Line-by-line Radiative Transfer Model (LBLRTM) and the discrete-ordinate-method radiative transfer code (DISORT). These spectra are freely available for interested researchers from the ACADIS data repository (doi:10.5065/D61J97TT).

scholarly journals A synthetic data set of high-spectral-resolution infrared spectra for the Arctic atmosphere

2016 ◽  
Vol 8 (1) ◽  
pp. 199-211 ◽  
Author(s):  
Christopher J. Cox ◽  
Penny M. Rowe ◽  
Steven P. Neshyba ◽  
Von P. Walden
Keyword(s):  
Remote Sensing ◽  
Radiative Transfer ◽  
Infrared Spectra ◽  
Spectral Resolution ◽  
High Spectral Resolution ◽  
The Arctic ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Data Set ◽  
Atmospheric State

Abstract. Cloud microphysical and macrophysical properties are critical for understanding the role of clouds in climate. These properties are commonly retrieved from ground-based and satellite-based infrared remote sensing instruments. However, retrieval uncertainties are difficult to quantify without a standard for comparison. This is particularly true over the polar regions, where surface-based data for a cloud climatology are sparse, yet clouds represent a major source of uncertainty in weather and climate models. We describe a synthetic high-spectral-resolution infrared data set that is designed to facilitate validation and development of cloud retrieval algorithms for surface- and satellite-based remote sensing instruments. Since the data set is calculated using pre-defined cloudy atmospheres, the properties of the cloud and atmospheric state are known a priori. The atmospheric state used for the simulations is drawn from radiosonde measurements made at the North Slope of Alaska (NSA) Atmospheric Radiation Measurement (ARM) site at Barrow, Alaska (71.325° N, 156.615° W), a location that is generally representative of the western Arctic. The cloud properties for each simulation are selected from statistical distributions derived from past field measurements. Upwelling (at 60 km) and downwelling (at the surface) infrared spectra are simulated for 260 cloudy cases from 50 to 3000 cm−1 (3.3 to 200 µm) at monochromatic (line-by-line) resolution at a spacing of  ∼  0.01 cm−1 using the Line-by-line Radiative Transfer Model (LBLRTM) and the discrete-ordinate-method radiative transfer code (DISORT). These spectra are freely available for interested researchers from the NSF Arctic Data Center data repository (doi:10.5065/D61J97TT).

scholarly journals Observation of HClO3 and HClO4 in the Arctic atmosphere

2020 ◽  
Author(s):  
Yee Jun Tham ◽  
Nina Sarnela ◽  
Carlos A. Cuevas ◽  
Iyer Siddharth ◽  
Lisa Beck ◽  
...  
Keyword(s):  
Gas Phase ◽  
Ozone Depletion ◽  
Surface Ozone ◽  
Negative Ion ◽  
The Arctic ◽  
Research Station ◽  
Visible Absorption ◽  
Data Set ◽  
Near Surface ◽  
Arctic Atmosphere

<p>Atmospheric halogens chemistry like the catalytic reaction of bromine and chlorine radicals with ozone (O<sub>3</sub>) has been known to cause the springtime surface-ozone destruction in the polar region. Although the initial atmospheric reactions of chlorine with ozone are well understood, the final oxidation steps leading to the formation of chlorate (ClO<sub>3</sub><sup>-</sup>) and perchlorate (ClO<sub>4</sub><sup>-</sup>) remain unclear due to the lack of direct evidence of their presence and fate in the atmosphere. In this study, we present the first high-resolution ambient data set of gas-phase HClO<sub>3</sub> (chloric acid) and HClO<sub>4</sub> (perchlorate acid) obtained from the field measurement at the Villum Research Station, Station Nord, in high arctic North Greenland (81°36’ N, 16°40’ W) during the spring of 2015. A state-of-the-art chemical ionization atmospheric pressure interface time-of-flight mass spectrometer (CI-APi-TOF) was used in negative ion mode with nitrate ion as the reagent ion to detect the gas-phase HClO<sub>3</sub> and HClO<sub>4</sub>. We measured significant level of HClO<sub>3</sub> and HClO<sub>4</sub> only during the springtime ozone depletion events in the Greenland, with concentration up to 9x10<sup>5</sup> molecule cm<sup>-3</sup>. Air mass trajectory analysis shows that the air during the ozone depletion event was confined to near-surface, indicating that the O<sub>3</sub> and surface of sea-ice/snowpack may play important roles in the formation of HClO<sub>3</sub> and HClO<sub>4</sub>. We used high-level quantum-chemical methods to calculate the ultraviolet-visible absorption spectra and cross-section of HClO<sub>3</sub> and HClO<sub>4</sub> in the gas-phase to assess their fates in the atmosphere. Overall, our results reveal the presence of HClO<sub>3</sub> and HClO<sub>4</sub> during ozone depletion events, which could affect the chlorine chemistry in the Arctic atmosphere.</p>

scholarly journals PHIPS-HALO: the airborne Particle Habit Imaging and Polar Scattering probe – Part 3: Single-particle phase discrimination and particle size distribution based on the angular-scattering function

2021 ◽  
Vol 14 (4) ◽  
pp. 3049-3070
Author(s):  
Fritz Waitz ◽  
Martin Schnaiter ◽  
Thomas Leisner ◽  
Emma Järvinen
Keyword(s):  
Particle Size ◽  
Single Particle ◽  
Large Data ◽  
The Arctic ◽  
Scattering Data ◽  
Scattering Function ◽  
Data Set ◽  
Phase Discrimination ◽  
Angular Scattering

Abstract. A major challenge for in situ observations in mixed-phase clouds remains the phase discrimination and sizing of cloud hydrometeors. In this work, we present a new method for determining the phase of individual cloud hydrometeors based on their angular-light-scattering behavior employed by the PHIPS (Particle Habit Imaging and Polar Scattering) airborne cloud probe. The phase discrimination algorithm is based on the difference of distinct features in the angular-scattering function of spherical and aspherical particles. The algorithm is calibrated and evaluated using a large data set gathered during two in situ aircraft campaigns in the Arctic and Southern Ocean. Comparison of the algorithm with manually classified particles showed that we can confidently discriminate between spherical and aspherical particles with a 98 % accuracy. Furthermore, we present a method for deriving particle size distributions based on single-particle angular-scattering data for particles in a size range from 100 µm ≤ D ≤ 700 µm and 20 µm ≤ D ≤ 700 µm for droplets and ice particles, respectively. The functionality of these methods is demonstrated in three representative case studies.

Radiative forcing over the Arctic of aerosols from the August 2017 Canadian and Greenlandic wildfires

2021 ◽  
Author(s):  
Filippo Calì Quaglia ◽  
Daniela Meloni ◽  
Alcide Giorgio di Sarra ◽  
Tatiana Di Iorio ◽  
Virginia Ciardini ◽  
...  
Keyword(s):  
Radiative Transfer ◽  
Radiative Forcing ◽  
Solar Zenith Angle ◽  
Surface Albedo ◽  
High Arctic ◽  
The Arctic ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Aerosol Layer ◽  
Radiative Effect

<p>Extended and intense wildfires occurred in Northern Canada and, unexpectedly, on the Greenlandic West coast during summer 2017. The thick smoke plume emitted into the atmosphere was transported to the high Arctic, producing one of the largest impacts ever observed in the region. Evidence of Canadian and Greenlandic wildfires was recorded at the Thule High Arctic Atmospheric Observatory (THAAO, 76.5°N, 68.8°W, www.thuleatmos-it.it) by a suite of instruments managed by ENEA, INGV, Univ. of Florence, and NCAR. Ground-based observations of the radiation budget have allowed quantification of the surface radiative forcing at THAAO. </p><p>Excess biomass burning chemical tracers such as CO, HCN, H2CO, C2H6, and NH3 were  measured in the air column above Thule starting from August 19 until August 23. The aerosol optical depth (AOD) reached a peak value of about 0.9 on August 21, while an enhancement of wildfire compounds was  detected in PM10. The measured shortwave radiative forcing was -36.7 W/m2 at 78° solar zenith angle (SZA) for AOD=0.626.</p><p>MODTRAN6.0 radiative transfer model (Berk et al., 2014) was used to estimate the aerosol radiative effect and the heating rate profiles at 78° SZA. Measured temperature profiles, integrated water vapour, surface albedo, spectral AOD and aerosol extinction profiles from CALIOP onboard CALIPSO were used as model input. The peak  aerosol heating rate (+0.5 K/day) was  reached within the aerosol layer between 8 and 12 km, while the maximum radiative effect (-45.4 W/m2) is found at 3 km, below the largest aerosol layer.</p><p>The regional impact of the event that occurred on August 21 was investigated using a combination of atmospheric radiative transfer modelling with measurements of AOD and ground surface albedo from MODIS. The aerosol properties used in the radiative transfer model were constrained by in situ measurements from THAAO. Albedo data over the ocean have been obtained from Jin et al. (2004). Backward trajectories produced through HYSPLIT simulations (Stein et al., 2015) were also employed to trace biomass burning plumes.</p><p>The radiative forcing efficiency (RFE) over land and ocean was derived, finding values spanning from -3 W/m2 to -132 W/m2, depending on surface albedo and solar zenith angle. The fire plume covered a vast portion of the Arctic, with large values of the daily shortwave RF (< -50 W/m2) lasting for a few days. This large amount of aerosol is expected to influence cloud properties in the Arctic, producing significant indirect radiative effects.</p>

Exploring the representation of clouds and humidity in the Arctic with cloud-resolving simulations using ICON-LEM

2021 ◽  
Author(s):  
Theresa Kiszler ◽  
Giovanni Chellini ◽  
Kerstin Ebell ◽  
Stefan Kneifel ◽  
Vera Schemann
Keyword(s):  
Microwave Radiometer ◽  
Remote Sensing Data ◽  
Large Data ◽  
Research Unit ◽  
Rain Gauge ◽  
The Arctic ◽  
Arctic Amplification ◽  
Data Set ◽  
Microphysical Processes ◽  
Mixed Phase Clouds

<p>The discussions around Arctic Amplification have led to extensive research, as done in the transregional collaboration (AC)³. One focus are the feedback mechanisms that are strengthening or weakening the warming. Several of these feedbacks involve moisture in the atmosphere in all phases. To understand these better we have been running and analysing daily cloud-resolving simulations. We performed these simulations for a region more strongly affected by the warming around Ny-Ålesund (Svalbard), which is challenging due to its diverse surface properties and mountainous surrounding. We have created an outstandingly large data set of several months of these simulations with 600 m resolution, using the Icosahedral non-hydrostatic model in the large-eddy mode (ICON-LEM).</p> <p>To gain some understanding of how well the model can represent such a complex location, we evaluated the performance of the model. For this, we used a range of observations from the measurement super-site located at Ny-Ålesund. This included radiosondes [1], a rain gauge, a microwave radiometer and further processed remote sensing data. Combining the measurements and simulations enables us to provide thorough statistics for different variables connected to clouds and to establish an understanding of how well they are represented.</p> <p>We show that the model is capable of simulating the two distinct flow regimes in the boundary layer and the free troposphere. Further, we found a tendency in the model to misrepresent liquid and mixed-phase clouds as purely ice clouds. Though the water vapour is well captured, we found further steps in the chain towards precipitation formation are insufficiently represented. Through the use of forward simulations and expanded model output, we can continue to get a better picture of possibilities to understand and improve the microphysical processes.</p> <p><em>This work was supported by the</em><em> DFG funded Transregio-project TR 172 “Arctic Amplification </em>(AC)3<em>“.</em></p> <p><strong>References</strong></p> <p>[1] M. Maturilli, High resolution radiosonde measurements from station Ny-Ålesund (2017-04 et seq). <em>Alfred</em> <em>Wegener Institute - Research Unit Potsdam, PANGAEA</em>, https://doi.org/10.1594/PANGAEA.914973 (2020)</p>

scholarly journals The color of melt ponds on Arctic sea ice

2018 ◽  
Vol 12 (4) ◽  
pp. 1331-1345 ◽  
Author(s):  
Peng Lu ◽  
Matti Leppäranta ◽  
Bin Cheng ◽  
Zhijun Li ◽  
Larysa Istomina ◽  
...  
Keyword(s):  
Radiative Transfer ◽  
Sea Ice ◽  
Arctic Sea Ice ◽  
Radiative Transfer Model ◽  
Ice Thickness ◽  
Transfer Model ◽  
Blue Color ◽  
Validation Data ◽  
Melt Ponds ◽  
Arctic Sea

Abstract. Pond color, which creates the visual appearance of melt ponds on Arctic sea ice in summer, is quantitatively investigated using a two-stream radiative transfer model for ponded sea ice. The upwelling irradiance from the pond surface is determined and then its spectrum is transformed into RGB (red, green, blue) color space using a colorimetric method. The dependence of pond color on various factors such as water and ice properties and incident solar radiation is investigated. The results reveal that increasing underlying ice thickness Hi enhances both the green and blue intensities of pond color, whereas the red intensity is mostly sensitive to Hi for thin ice (Hi  <  1.5 m) and to pond depth Hp for thick ice (Hi  >  1.5 m), similar to the behavior of melt-pond albedo. The distribution of the incident solar spectrum F0 with wavelength affects the pond color rather than its intensity. The pond color changes from dark blue to brighter blue with increasing scattering in ice, and the influence of absorption in ice on pond color is limited. The pond color reproduced by the model agrees with field observations for Arctic sea ice in summer, which supports the validity of this study. More importantly, the pond color has been confirmed to contain information about meltwater and underlying ice, and therefore it can be used as an index to retrieve Hi and Hp. Retrievals of Hi for thin ice (Hi  <  1 m) agree better with field measurements than retrievals for thick ice, but those of Hp are not good. The analysis of pond color is a new potential method to obtain thin ice thickness in summer, although more validation data and improvements to the radiative transfer model will be needed in future.

scholarly journals Climatological and radiative properties of midlatitude cirrus clouds derived by automatic evaluation of lidar measurements

2016 ◽  
Vol 16 (12) ◽  
pp. 7605-7621 ◽  
Author(s):  
Erika Kienast-Sjögren ◽  
Christian Rolf ◽  
Patric Seifert ◽  
Ulrich K. Krieger ◽  
Bei P. Luo ◽  
...  
Keyword(s):  
Radiative Forcing ◽  
Cirrus Clouds ◽  
Radiative Properties ◽  
Radiation Budget ◽  
Shortwave Radiation ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Data Set ◽  
Detection Scheme ◽  
Lidar Measurements

Abstract. Cirrus, i.e., high, thin clouds that are fully glaciated, play an important role in the Earth's radiation budget as they interact with both long- and shortwave radiation and affect the water vapor budget of the upper troposphere and stratosphere. Here, we present a climatology of midlatitude cirrus clouds measured with the same type of ground-based lidar at three midlatitude research stations: at the Swiss high alpine Jungfraujoch station (3580 m a.s.l.), in Zürich (Switzerland, 510 m a.s.l.), and in Jülich (Germany, 100 m a.s.l.). The analysis is based on 13 000 h of measurements from 2010 to 2014. To automatically evaluate this extensive data set, we have developed the Fast LIdar Cirrus Algorithm (FLICA), which combines a pixel-based cloud-detection scheme with the classic lidar evaluation techniques. We find mean cirrus optical depths of 0.12 on Jungfraujoch and of 0.14 and 0.17 in Zürich and Jülich, respectively. Above Jungfraujoch, subvisible cirrus clouds (τ < 0.03) have been observed during 6 % of the observation time, whereas above Zürich and Jülich fewer clouds of that type were observed. Cirrus have been observed up to altitudes of 14.4 km a.s.l. above Jungfraujoch, whereas they have only been observed to about 1 km lower at the other stations. These features highlight the advantage of the high-altitude station Jungfraujoch, which is often in the free troposphere above the polluted boundary layer, thus enabling lidar measurements of thinner and higher clouds. In addition, the measurements suggest a change in cloud morphology at Jungfraujoch above ∼ 13 km, possibly because high particle number densities form in the observed cirrus clouds, when many ice crystals nucleate in the high supersaturations following rapid uplifts in lee waves above mountainous terrain. The retrieved optical properties are used as input for a radiative transfer model to estimate the net cloud radiative forcing, CRFNET, for the analyzed cirrus clouds. All cirrus detected here have a positive CRFNET. This confirms that these thin, high cirrus have a warming effect on the Earth's climate, whereas cooling clouds typically have cloud edges too low in altitude to satisfy the FLICA criterion of temperatures below −38 °C. We find CRFNET = 0.9 W m−2 for Jungfraujoch and 1.0 W m−2 (1.7 W m−2) for Zürich (Jülich). Further, we calculate that subvisible cirrus (τ < 0.03) contribute about 5 %, thin cirrus (0.03 < τ < 0.3) about 45 %, and opaque cirrus (0.3 < τ) about 50 % of the total cirrus radiative forcing.

scholarly journals Aerosol absorption retrieval at ultraviolet wavelengths in a complex environment

2016 ◽  
Author(s):  
Stelios Kazadzis ◽  
Panagiotis Ι. Raptis ◽  
Natalia Kouremeti ◽  
Vassilis Amiridis ◽  
Antti Arola ◽  
...  
Keyword(s):  
Wavelength Dependence ◽  
Single Scattering ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Aerosol Composition ◽  
Data Set ◽  
Aerosol Absorption ◽  
Uv Irradiance ◽  
Band Radiometer ◽  
Uv Range

Abstract. We have used total and diffuse UV irradiance measurements with a multi-filter rotating shadow-band radiometer (UVMFR), in order to calculate aerosol absorption properties (Single Scattering Albedo – SSA) in the UV range, for a 5 years period in Athens, Greece. Τhis data set was used as input to a radiative transfer model and the SSA for 368 nm and 332 nm has been calculated. Retrievals from a collocated CIMEL sun-photometer were used to validate the products and study absorption spectral behavior SSA values at these wavelengths. UVMFR SSA together with synchronous,CIMEL-derived, retrievals at 440 nm, show a mean of 0.90, 0.87 and 0.83, with lowest values (higher absorption) towards lower wavelengths. In addition, noticeable diurnal variations of the SSA in all wavelengths are revealed, with amplitudes in up to 0.05. High SSA wavelength dependence is found for cases of low Ångström exponents and also an SSA decrease with decreasing extinction optical depth, suggesting an effect of the different aerosol composition. Dust and Brown Carbon UV absorbing properties were investigated to understand seasonal variability of the results.

scholarly journals Accounting for the effect of horizontal gradients in limb measurements of scattered sunlight

2007 ◽  
Vol 7 (6) ◽  
pp. 16155-16183 ◽  
Author(s):  
J. Puķīte ◽  
S. Kühl ◽  
T. Deutschmann ◽  
U. Platt ◽  
T. Wagner
Keyword(s):  
Monte Carlo ◽  
Radiative Transfer ◽  
Scattered Light ◽  
Trace Gases ◽  
The Arctic ◽  
Radiative Transfer Model ◽  
Boreal Winter ◽  
Transfer Model ◽  
Measurement Sensitivity ◽  
Horizontal Gradients

Abstract. Limb measurements provided by the SCanning Imaging Absorption spectrometer for Atmospheric CHartographY (SCIAMACHY) on the ENVISAT satellite allow retrieving stratospheric profiles of various trace gases on a global scale, among them BrO for the first time. For limb observations in the UV/VIS spectral region the instrument measures scattered light with a complex distribution of light paths: the light is measured at different elevation angles and can be scattered or absorbed in the atmosphere or reflected by the ground. By means of spectroscopy and radiative transfer modelling the measurements can be inverted to retrieve the vertical distribution of stratospheric trace gases. A full spherical 3-D Monte Carlo radiative transfer model "Tracy-II" is applied in this study. The Monte Carlo method benefits from conceptual simplicity and allows realizing the concept of full spherical geometry of the atmosphere and also its 3-D properties, which is important for a realistic description of the limb geometry. Furthermore it allows accounting for horizontal gradients in the distribution of trace gases. In this study the effect ofhorizontal inhomogeneous distributions of trace gases on the retrieval of profiles from limb measurements of scattered UV/VIS light is investigated. We introduce a method to correct for this effect by combining consecutive limb scanning sequences and utilizing the overlap in their measurement sensitivity regions. It is found that if horizontal inhomogenity is not properly accounted for, typical errors of 20% for NO2 and up to 50% for OClO around the altitude of the profile peak can arise for measurements close to the Arctic polar vortex boundary in boreal winter.

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