Rayleigh–Brillouin Scattering in Compressed H2, D2, and HD. II

1972 ◽  
Vol 50 (12) ◽  
pp. 1227-1229 ◽  
Author(s):  
E. H. Hara ◽  
A. D. May

The observations presented by Hara et al. for the Brillouin spectrum of H2, D2, and HD are compared with the thermo-hydrodynamic theory of Bhatia and Tong. It is noted that although this theory is qualitatively correct it fails to describe accurately the spectrum at low to medium densities. It is suggested that the introduction of a relaxing thermal conduction might account for the discrepancy observed.

1971 ◽  
Vol 49 (4) ◽  
pp. 420-431 ◽  
Author(s):  
E. H. Hara ◽  
A. D. May ◽  
H. F. P. Knaap

The Rayleigh–Brillouin spectrum of light scattered from H2, D2, and HD has been measured at densities ranging from 1/2 to 104 amagat, all at room temperature. The apparatus consisted of a 20 mW He–Ne laser, a high pressure cell for 90° scattering, a pressure scanned Fabry–Perot interferometer, and photon counting electronics. A discrepancy is noted between the observed spectra and various theoretical spectra. It is suggested that the discrepancy arises from an omission in the theories of coupling between relaxation of the rotational states and thermal conduction.


1977 ◽  
Vol 55 (1) ◽  
pp. 23-26 ◽  
Author(s):  
M. Hubert ◽  
A. D. May

This paper reports on a comparison between the observed Rayleigh–Brillouin spectra of compressed hydrogen and those computed according to the translational hydrodynamic theory of Desai and Kapral. Reasonable agreement is found in the range of densities from 19 to 61 amagat units. It is suggested that small residual discrepancies may be due to the neglect of part of the coupling between the energy and momentum fluctuations arising from relaxation of the rotational states, i.e. due to the neglect of the 1ν1 terms.


1978 ◽  
Vol 56 (9) ◽  
pp. 1168-1174 ◽  
Author(s):  
A. D. May ◽  
M. Hubert ◽  
V. Ghaem-Maghami

The Rayleigh–Brillouin spectrum of light scattered from hydrogen at high densities is reported. The observations are compared with translational hydrodynamic theory and ultrasonic experiments. The range of densities includes the relaxation region and we find evidence for multiple relaxation. A mean relaxation time for normal hydrogen at 24 °C of (1.41 ± 0.06) × 10−8 s is found, in agreement with theoretical calculations.


1992 ◽  
Vol 2 (12) ◽  
pp. 2081-2088 ◽  
Author(s):  
Francesco Mallamace ◽  
Norberto Micali ◽  
Cirino Vasi ◽  
Rama Bansil ◽  
Sinisa Pajevic ◽  
...  
Keyword(s):  

1981 ◽  
Vol 42 (C6) ◽  
pp. C6-804-C6-806
Author(s):  
V. Bortolani ◽  
F. Nizzoli ◽  
G. Santoro ◽  
A. Marvin

1984 ◽  
Vol 45 (C5) ◽  
pp. C5-103-C5-107
Author(s):  
D. R. Tilley ◽  
E. L. Albuquerque ◽  
M. C. Oliveros

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