scholarly journals Hybrid bilayer plasmonic metasurface efficiently manipulates visible light

2016 ◽  
Vol 2 (1) ◽  
pp. e1501168 ◽  
Author(s):  
Fei Qin ◽  
Lu Ding ◽  
Lei Zhang ◽  
Francesco Monticone ◽  
Chan Choy Chum ◽  
...  

Metasurfaces operating in the cross-polarization scheme have shown an interesting degree of control over the wavefront of transmitted light. Nevertheless, their inherently low efficiency in visible light raises certain concerns for practical applications. Without sacrificing the ultrathin flat design, we propose a bilayer plasmonic metasurface operating at visible frequencies, obtained by coupling a nanoantenna-based metasurface with its complementary Babinet-inverted copy. By breaking the radiation symmetry because of the finite, yet small, thickness of the proposed structure and benefitting from properly tailored intra- and interlayer couplings, such coupled bilayer metasurface experimentally yields a conversion efficiency of 17%, significantly larger than that of earlier single-layer designs, as well as an extinction ratio larger than 0 dB, meaning that anomalous refraction dominates the transmission response. Our finding shows that metallic metasurface can counterintuitively manipulate the visible light as efficiently as dielectric metasurface (~20% in conversion efficiency in Lin et al.’s study), although the metal’s ohmic loss is much higher than dielectrics. Our hybrid bilayer design, still being ultrathin (~λ/6), is found to obey generalized Snell’s law even in the presence of strong couplings. It is capable of efficiently manipulating visible light over a broad bandwidth and can be realized with a facile one-step nanofabrication process.

Author(s):  
Aufandra Cakra Wardhana ◽  
Sou Yasuhara ◽  
Min Wen Yu ◽  
Akira Yamaguchi ◽  
Tadaaki Nagao ◽  
...  

Efficient visible-light-active photocatalysts are of great interest for practical applications. First-row transition metal oxide nanoclusters have been loaded onto ultraviolet (UV)-driven semiconductors for several photocatalytic reactions under visible-light illumination. However,...


2015 ◽  
Vol 29 (13) ◽  
pp. 1550057 ◽  
Author(s):  
Bo Wang ◽  
Hongtao Li ◽  
Wenhao Shu ◽  
Li Chen ◽  
Liang Lei ◽  
...  

The high efficiency and the wideband properties are not easy to be obtained by the conventional binary grating-based polarizer. Although the grating polarizer was demonstrated in experiments, the performance should be improved further to meet the practical applications. A novel sandwiched two-layer grating polarizer is presented to improve the efficiency and the bandwidth. Such a polarizer can have advantages of high efficiency of the sandwiched grating and wide bandwidth of the two-layer grating. The grating depths of two layers are optimized for the special duty cycle of 0.3 and the given period. The diffraction efficiency and the incident bandwidth of the novel grating polarizer are improved greatly compared with the conventional simple grating and the sandwiched single-layer grating. Moreover, high extinction ratio can be shown in both two orders and the moderate fabrication tolerance should be good guideline for practical applications.


Nanomaterials ◽  
2018 ◽  
Vol 8 (9) ◽  
pp. 697 ◽  
Author(s):  
Jun Yang ◽  
Taiping Xie ◽  
Chenglun Liu ◽  
Longjun Xu

Dy-doped BiOCl powder photocatalyst was synthesized A one–step coprecipitation method. The incorporation of Dy3+ replaced partial Bi3+ in BiOCl crystal lattice system. For Rhodamine B (RhB) under visible light irradiation, 2% Dy doped BiOCl possessed highly efficient photocatalytic activity and photodegradation efficiency. The photodegradation ratio of RhB could reach 97.3% after only 30 min of photocatalytic reaction; this was more than relative investigations have reported in the last two years. The main reason was that the 4f electron shell of Dy in the BiOCl crystal lattice system can generate a special electronic shell structure that facilitated the transfer of electron from valance band to conduction band and separation of the photoinduced charge carrier. Apart from material preparation, this research is expected to provide important references for RhB photodegradation in practical applications.


Processes ◽  
2021 ◽  
Vol 9 (1) ◽  
pp. 99
Author(s):  
Sun-Woo Yi ◽  
In-Keun Yu ◽  
Woon-Jung Kim ◽  
Seong-Ho Choi

In this study, we coated the surface of glass slides with nanoprotrusion, nanoparticles, and nanofilm structures by one-step plasma deposition of three vinyl monomers. Three functional vinyl monomers with symmetrical polarity sites were used: methyl methacrylate (MMA), trifluoro methylmethacrylate (TFMA), and trimethylsilyl methyl methacrylate (TSMA). The TSMA/MMA (80/20, mol-%) nanoprotrusion-coated surface of slide glass was superhydrophobic, with a 153° contact angle. We also evaluated the transmittance (%) of the slide glass with nanoprotrusions in the infrared (IR) (940 nm), ultraviolet (365 nm) and visible light (380–700 nm) regions. The obtained nanoprotrusion structure surface of slide glass created by plasma deposition transmits more than 90% of visible light.


Author(s):  
Chao Zhang ◽  
Baoquan Liu ◽  
Weiping Li ◽  
Xiangxue Liu ◽  
Ke Wang ◽  
...  

Well-designed honeycomb Co3O4@CdS (H-Co3O4@CdS) was fabricated via a one-step strategy for efficient water splitting. During the decoration of CdS, honeycomb Co3O4 (H-Co3O4) with macropore was formed simultaneously. H-Co3O4 could enhance...


Catalysts ◽  
2021 ◽  
Vol 11 (7) ◽  
pp. 848
Author(s):  
Jong-Wook Hong

Visible-light-driven hydrogen production through photocatalysis has attracted enormous interest owing to its great potential to address energy and environmental issues. However, photocatalysis possesses several limitations to overcome for practical applications, such as low light absorption efficiency, rapid charge recombination, and poor stability of photocatalysts. Here, the preparation of efficient noble metal–semiconductor hybrid photocatalysts for photocatalytic hydrogen production is presented. The prepared ternary Rh–TiO2–CeO2 hybrid photocatalysts exhibited excellent photocatalytic performance toward the hydrogen production reaction compared with their counterparts, ascribed to the synergistic combination of Rh, TiO2, and CeO2.


2020 ◽  
Vol 276 ◽  
pp. 128213 ◽  
Author(s):  
Jie Chen ◽  
Xiaojun Xu ◽  
Li Feng ◽  
Aijiang He ◽  
Lixiu Liu ◽  
...  

Nanoscale ◽  
2019 ◽  
Vol 11 (6) ◽  
pp. 2871-2877 ◽  
Author(s):  
Ting Zhang ◽  
Feng Wang ◽  
Peng Zhang ◽  
Yafei Wang ◽  
Hao Chen ◽  
...  

The flexible perovskite photodetector, fabricated by a modified one-step method, showed a broadband spectrum response from blind ultraviolet to visible light, and exhibited excellent mechanical flexibility and improved environmental stability.


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