Second Harmonic Generation Probe Of Adsorbate Structural Transition And Energy Transfer Dynamics On A Metal Surface

1989 ◽  
Author(s):  
L E. Urbach ◽  
D. Heskett ◽  
J M. Hicks ◽  
K. J. Song ◽  
E W. Plummer ◽  
...  
Keyword(s):  
Energy Transfer ◽  
Second Harmonic Generation ◽  
Metal Surface ◽  
Harmonic Generation ◽  
Structural Transition ◽  
Second Harmonic

Anderson localization effects in the second harmonic generation at a weakly rough metal surface

1992 ◽  
Vol 170 (3) ◽  
pp. 231-234 ◽  
Author(s):  
O.A. Aktsipetrov ◽  
V.N. Golovkina ◽  
O.I. Kapusta ◽  
T.A. Leskova ◽  
N.N. Novikova
Keyword(s):  
Second Harmonic Generation ◽  
Metal Surface ◽  
Harmonic Generation ◽  
Anderson Localization ◽  
Second Harmonic

scholarly journals Enhancing second-harmonic generation with electron spill-out at metallic surfaces

2020 ◽  
Vol 3 (1) ◽  
Author(s):  
Muhammad Khalid ◽  
Cristian Ciracì
Keyword(s):  
Second Harmonic Generation ◽  
Metal Surface ◽  
Harmonic Generation ◽  
Second Harmonic ◽  
Thick Layer ◽  
Metallic Surfaces ◽  
Hydrodynamic Description ◽  
Second Harmonic Generation Efficiency ◽  
Quantum Hydrodynamic ◽  
Quantum Mechanical Effects

AbstractSecond-order nonlinear optical processes do not manifest in the bulk of centrosymmetric materials, but may occur in the angstroms-thick layer at surfaces. At such length scales, quantum mechanical effects come into play which could be crucial for an accurate description of plasmonic systems. In this article, we develop a theoretical model based on the quantum hydrodynamic description to study free-electron nonlinear dynamics in plasmonic systems. Our model predicts strong resonances induced by the spill-out of electron density at the metal surface. We show that these resonances can boost second-harmonic generation efficiency up to four orders of magnitude and can be arbitrarily tuned by controlling the electron spill-out at the metal surface with the aid of thin dielectric layers. These results offer a possibility to artificially increase nonlinear susceptibilities by engineering optical properties at the quantum level.

Dynamical Screening at a Metal Surface Probed by Second-Harmonic Generation

1988 ◽  
Vol 61 (12) ◽  
pp. 1380-1383 ◽  
Author(s):  
K. J. Song ◽  
D. Heskett ◽  
H. L. Dai ◽  
A. Liebsch ◽  
E. W. Plummer
Keyword(s):  
Second Harmonic Generation ◽  
Metal Surface ◽  
Harmonic Generation ◽  
Second Harmonic ◽  
Dynamical Screening

Second-harmonic generation by a reflecting metal surface

1994 ◽  
Author(s):  
N. N. Akhmediev ◽  
Igor V. Mel'nikov ◽  
L. J. Robur
Keyword(s):  
Second Harmonic Generation ◽  
Metal Surface ◽  
Harmonic Generation ◽  
Second Harmonic

Near-field second harmonic generation from a rough metal surface

1997 ◽  
Vol 56 (15) ◽  
pp. 9290-9293 ◽  
Author(s):  
Igor I. Smolyaninov ◽  
Anatoly V. Zayats ◽  
Christopher C. Davis
Keyword(s):  
Second Harmonic Generation ◽  
Metal Surface ◽  
Harmonic Generation ◽  
Second Harmonic ◽  
Near Field
Sign in / Sign up

Export Citation Format

Share Document