Near-field second harmonic generation from a rough metal surface

1997 ◽  
Vol 56 (15) ◽  
pp. 9290-9293 ◽  
Author(s):  
Igor I. Smolyaninov ◽  
Anatoly V. Zayats ◽  
Christopher C. Davis
1992 ◽  
Vol 170 (3) ◽  
pp. 231-234 ◽  
Author(s):  
O.A. Aktsipetrov ◽  
V.N. Golovkina ◽  
O.I. Kapusta ◽  
T.A. Leskova ◽  
N.N. Novikova

2020 ◽  
Vol 3 (1) ◽  
Author(s):  
Muhammad Khalid ◽  
Cristian Ciracì

AbstractSecond-order nonlinear optical processes do not manifest in the bulk of centrosymmetric materials, but may occur in the angstroms-thick layer at surfaces. At such length scales, quantum mechanical effects come into play which could be crucial for an accurate description of plasmonic systems. In this article, we develop a theoretical model based on the quantum hydrodynamic description to study free-electron nonlinear dynamics in plasmonic systems. Our model predicts strong resonances induced by the spill-out of electron density at the metal surface. We show that these resonances can boost second-harmonic generation efficiency up to four orders of magnitude and can be arbitrarily tuned by controlling the electron spill-out at the metal surface with the aid of thin dielectric layers. These results offer a possibility to artificially increase nonlinear susceptibilities by engineering optical properties at the quantum level.


1999 ◽  
Author(s):  
Anatoly V. Zayats ◽  
Igor I. Smolyaninov ◽  
Christopher C. Davis

2002 ◽  
Vol 81 (18) ◽  
pp. 3461-3463 ◽  
Author(s):  
Inna Barsegova ◽  
Aaron Lewis ◽  
Artium Khatchatouriants ◽  
Alexandra Manevitch ◽  
Andrei Ignatov ◽  
...  

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