A Solar Reactor Design for Research on Calcium Oxide-Based Carbon Dioxide Capture

2017 ◽  
Vol 139 (5) ◽  
Author(s):  
Leanne Reich ◽  
Luke Melmoth ◽  
Lindsey Yue ◽  
Roman Bader ◽  
Robert Gresham ◽  
...  

An engineering design for a novel 1-kW solar-driven reactor to capture carbon dioxide via the calcium oxide-based two-step carbonation–calcination cycle has been completed. The reactor consists of a downward-facing cylindrical dual cavity. The inner cavity serves as the radiation receiver, while the outer cavity is the reaction chamber that contains a packed- or fluidized-bed of reacting particles. Several aspects have been incorporated in this reactor design, including high flexibility, mechanical rigidity and simplicity, high-temperature and thermal shock resistance, accommodation of thermal expansion, low convective heat losses, uniform gas distribution inside the reaction chamber, and simple reactor assembly. The final reactor design is presented, and the reactor assembly is illustrated.

Author(s):  
Leanne Reich ◽  
Luke Melmoth ◽  
Robert Gresham ◽  
Terrence Simon ◽  
Wojciech Lipiński

An engineering design for a 1-kW dual-cavity solar-driven reactor to capture carbon dioxide via the calcium oxide based two-step carbonation-calcination cycle is presented. In the low temperature carbonation step, gas containing up to 15% carbon dioxide flows through a gas manifold and plenum into an annular reaction zone filled with calcium oxide particles. The carbon dioxide reacts with the calcium oxide, forming calcium carbonate. Carbon dioxide-depleted gas flows out of the reactor through a second gas manifold. In the high temperature calcination step, concentrated solar radiation enters the beam-up oriented, windowless reactor and is absorbed by the diathermal cavity wall, which transfers heat via conduction to the calcium carbonate particles formed in the previous step. The calcium carbonate dissociates into calcium oxide and carbon dioxide. Additional carbon dioxide is used as a sweep gas to ensure high purity carbon dioxide at the outlet. Mechanical and thermal analyses are conducted to refine an initial reactor design and identify potential design shortcomings. Numerically predicted temperature profiles in the reactor are presented and the final reactor design is established.


2014 ◽  
Vol 3 (1) ◽  
pp. 10-19 ◽  
Author(s):  
Li Zhang ◽  
Bo Zhang ◽  
Zhongqing Yang ◽  
Mingnv Guo

2014 ◽  
Vol 14 (2) ◽  
pp. 500-514 ◽  
Author(s):  
Leanne Reich ◽  
Lindsey Yue ◽  
Roman Bader ◽  
Wojciech Lipiński

2017 ◽  
Vol 5 (8) ◽  
pp. 1514-1514
Author(s):  
Liang Huang ◽  
Yu Zhang ◽  
Wanlin Gao ◽  
Takuya Harada ◽  
Qingqing Qin ◽  
...  

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