scholarly journals Zeeman quantum beats of helium Rydberg states excited by synchrotron radiation

2020 ◽  
Vol 27 (3) ◽  
pp. 675-680 ◽  
Author(s):  
Yasumasa Hikosaka ◽  
Hiroshi Iwayama ◽  
Tatsuo Kaneyasu

Quantum beats in fluorescence decay from Zeeman-split magnetic sublevels have been measured for helium Rydberg states excited by synchrotron radiation. The Zeeman quantum beats observed in this prototypical case were fitted with an equation from a theoretical formulation. It is proposed that Zeeman quantum beat measurement can be a useful way to simply evaluate the polarization characteristics of extreme ultraviolet light.

2019 ◽  
Author(s):  
Ashley Fidler ◽  
Hugo Marroux ◽  
Erika Warrick ◽  
Etienne Bloch ◽  
Wei Cao ◽  
...  

The autoionization dynamics of the (<sup>2</sup>P<sub>1/2</sub>)ns/d Rydberg states in krypton are investigated using wave-mixing signals generated with subfemtosecond XUV pulses and noncollinear, few-cycle NIR pulses. Despite quantum beat oscillations from the XUV-induced coherence, these wave-mixing spectra allow for the simultaneous evaluation of autoionization lifetimes from a series of Rydberg states. Experimentally measured lifetimes for the wave-mixing signals emitting from the (<sup>2</sup>P<sub>1/2</sub>)6d/8s, 7d/9s, and 8d/10s resonances compare favorably with lifetimes for the (<sup>2</sup>P<sub>1/2</sub>)6d, 7d, and 8d Rydberg states determined from spectral linewidths. Analysis of the quantum beats reveals that the enhancement of wave-mixing pathways leads to reporter state-dependent decays in the wave-mixing signals. The results demonstrate the promise of wave-mixing spectroscopies with subfemtosecond XUV pulses to provide valuable insights into processes governed by electronic dynamics.<br>


2019 ◽  
Author(s):  
Ashley Fidler ◽  
Hugo Marroux ◽  
Erika Warrick ◽  
Etienne Bloch ◽  
Wei Cao ◽  
...  

The autoionization dynamics of the (<sup>2</sup>P<sub>1/2</sub>)ns/d Rydberg states in krypton are investigated using wave-mixing signals generated with subfemtosecond XUV pulses and noncollinear, few-cycle NIR pulses. Despite quantum beat oscillations from the XUV-induced coherence, these wave-mixing spectra allow for the simultaneous evaluation of autoionization lifetimes from a series of Rydberg states. Experimentally measured lifetimes for the wave-mixing signals emitting from the (<sup>2</sup>P<sub>1/2</sub>)6d/8s, 7d/9s, and 8d/10s resonances compare favorably with lifetimes for the (<sup>2</sup>P<sub>1/2</sub>)6d, 7d, and 8d Rydberg states determined from spectral linewidths. Analysis of the quantum beats reveals that the enhancement of wave-mixing pathways leads to reporter state-dependent decays in the wave-mixing signals. The results demonstrate the promise of wave-mixing spectroscopies with subfemtosecond XUV pulses to provide valuable insights into processes governed by electronic dynamics.<br>


2017 ◽  
Vol 11 (4) ◽  
pp. 209-210
Author(s):  
Taro Sekikawa ◽  
Kenichi L. Ishikawa

2012 ◽  
Vol 19 (6) ◽  
pp. 063302 ◽  
Author(s):  
Takuya Ozawa ◽  
Shuhei Yamamura ◽  
Nao Tatsumura ◽  
Kazuhiko Horioka ◽  
Tohru Kawamura

Author(s):  
Yun Yuan ◽  
Yan-Yun Ma ◽  
Wenpeng Wang ◽  
Shijia Chen ◽  
Ye Cui ◽  
...  

Abstract In this study, we use the FLASH radiation hydrodynamic code and the FLYCHK atomic code to investigate the energy conversion and spectra associated with laser–Sn target interactions with 1 µm and 2 µm wavelength lasers. We found that the conversion efficiency (CE) reached as much as 3.38% with the 2 µm laser, which is 1.48 percentage points higher than the 1 µm laser (CE = 1.9%). In addition, we analyzed the contribution of dominant ionization states to the emission spectrum for both lasers. We observed that the growths of the out-of-band emission eventually led to a broadening of the spectrum, resulting in a reduction of SP for the 1 µm laser. By contrast, the emission main peaks were all centered near 13.5nm for the 2 µm laser, which is beneficial for efficient emission of light with a 13.5 nm wavelength (relevant for nanolithographic applications).


2018 ◽  
Vol 113 (15) ◽  
pp. 153502 ◽  
Author(s):  
A. G. Shalashov ◽  
A. V. Vodopyanov ◽  
I. S. Abramov ◽  
A. V. Sidorov ◽  
E. D. Gospodchikov ◽  
...  

2020 ◽  
Author(s):  
Oscar Versolato ◽  
Lars Behnke ◽  
Ruben Schupp ◽  
Zoi Bouza ◽  
MUHARREM BAYRAKTAR ◽  
...  

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