Hot-Carrier Thermalization in Amorphous Silicon

1981 ◽  
Vol 47 (9) ◽  
pp. 700-700 ◽  
Author(s):  
Z. Vardeny ◽  
J. Tauc
1981 ◽  
Vol 46 (18) ◽  
pp. 1223-1226 ◽  
Author(s):  
Z. Vardeny ◽  
J. Tauc

1992 ◽  
Vol 258 ◽  
Author(s):  
J. Fan ◽  
J. Kakalios

ABSTRACTThe room temperature non-radiative efficiency, defined as the ratio of the heat released per absorbed photon for doped and undoped hydrogenated amorphous silicon (a-Si:H) has been measured using photo-pyroelectric spectroscopy (PPES) for photon energies ranging from 2.5 to 1.6 eV. There is a fairly sharp minimum in the non-radiative efficiency when the a-Si:H is illuminated with near bandgap photons. We describe a model wherein this minimum arises from the variation in the amount of heat generated by free carrier thermalization as the incident photon energy is varied, and report measurements of the excitation kinetics of the non-radiative efficiency which support this proposal.


1989 ◽  
Vol 32 (12) ◽  
pp. 1863-1867 ◽  
Author(s):  
K. Leo ◽  
W.W. Rühle ◽  
K. Ploog

2019 ◽  
Vol 5 (11) ◽  
pp. eaax9958 ◽  
Author(s):  
Yuzhong Chen ◽  
Yujie Li ◽  
Yida Zhao ◽  
Hongzhi Zhou ◽  
Haiming Zhu

Although the unique hot carrier characteristics in graphene suggest a new paradigm for hot carrier–based energy harvesting, the reported efficiencies with conventional photothermoelectric and photothermionic emission pathways are quite low because of inevitable hot carrier thermalization and cooling loss. Here, we proposed and demonstrated the possibility of efficiently extracting hot electrons from graphene after carrier intraband scattering but before electron-hole interband thermalization, a new regime that has never been reached before. Using various layered semiconductors as model electron-accepting components, we generally observe ultrafast injection of energetic hot electrons from graphene over a very broad photon energy range (visible to mid-infrared). The injection quantum yield reaches as high as ~50%, depending on excitation energy but remarkably, not on fluence, in notable contrast with conventional pathways with nonlinear behavior. Hot electron harvesting in this regime prevails over energy and carrier loss and closely resembles the concept of hot carrier solar cell.


1996 ◽  
pp. 97-99
Author(s):  
A. I. Lobad ◽  
Y. Kostoulas ◽  
G. W. Wicks ◽  
P. M. Fauchet

1998 ◽  
Vol 84 (9) ◽  
pp. 4984-4991 ◽  
Author(s):  
J. O. White ◽  
S. Cuzeau ◽  
D. Hulin ◽  
R. Vanderhaghen

2017 ◽  
Vol 12 (9) ◽  
pp. 871-876 ◽  
Author(s):  
Bolin Liao ◽  
Ebrahim Najafi ◽  
Heng Li ◽  
Austin J. Minnich ◽  
Ahmed H. Zewail

2020 ◽  
Vol 128 (19) ◽  
pp. 193102
Author(s):  
Maxime Giteau ◽  
Edouard de Moustier ◽  
Daniel Suchet ◽  
Hamidreza Esmaielpour ◽  
Hassanet Sodabanlu ◽  
...  

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