scholarly journals Identification of surface and volume hot-carrier thermalization mechanisms in ultrathin GaAs layers

2020 ◽  
Vol 128 (19) ◽  
pp. 193102
Author(s):  
Maxime Giteau ◽  
Edouard de Moustier ◽  
Daniel Suchet ◽  
Hamidreza Esmaielpour ◽  
Hassanet Sodabanlu ◽  
...  
1989 ◽  
Vol 32 (12) ◽  
pp. 1863-1867 ◽  
Author(s):  
K. Leo ◽  
W.W. Rühle ◽  
K. Ploog

2019 ◽  
Vol 5 (11) ◽  
pp. eaax9958 ◽  
Author(s):  
Yuzhong Chen ◽  
Yujie Li ◽  
Yida Zhao ◽  
Hongzhi Zhou ◽  
Haiming Zhu

Although the unique hot carrier characteristics in graphene suggest a new paradigm for hot carrier–based energy harvesting, the reported efficiencies with conventional photothermoelectric and photothermionic emission pathways are quite low because of inevitable hot carrier thermalization and cooling loss. Here, we proposed and demonstrated the possibility of efficiently extracting hot electrons from graphene after carrier intraband scattering but before electron-hole interband thermalization, a new regime that has never been reached before. Using various layered semiconductors as model electron-accepting components, we generally observe ultrafast injection of energetic hot electrons from graphene over a very broad photon energy range (visible to mid-infrared). The injection quantum yield reaches as high as ~50%, depending on excitation energy but remarkably, not on fluence, in notable contrast with conventional pathways with nonlinear behavior. Hot electron harvesting in this regime prevails over energy and carrier loss and closely resembles the concept of hot carrier solar cell.


1996 ◽  
pp. 97-99
Author(s):  
A. I. Lobad ◽  
Y. Kostoulas ◽  
G. W. Wicks ◽  
P. M. Fauchet

1981 ◽  
Vol 46 (18) ◽  
pp. 1223-1226 ◽  
Author(s):  
Z. Vardeny ◽  
J. Tauc

RSC Advances ◽  
2016 ◽  
Vol 6 (93) ◽  
pp. 90846-90855 ◽  
Author(s):  
Wenkai Cao ◽  
Zewen Zhang ◽  
Rob Patterson ◽  
Yuan Lin ◽  
Xiaoming Wen ◽  
...  

PbS QDs are studied as attractive candidates to be applied as hot carrier solar cell absorbers.


1981 ◽  
Vol 47 (9) ◽  
pp. 700-700 ◽  
Author(s):  
Z. Vardeny ◽  
J. Tauc

2019 ◽  
Vol 5 (6) ◽  
pp. eaav1493 ◽  
Author(s):  
Yuxuan Lin ◽  
Qiong Ma ◽  
Pin-Chun Shen ◽  
Batyr Ilyas ◽  
Yaqing Bie ◽  
...  

The massless Dirac electron transport in graphene has led to a variety of unique light-matter interaction phenomena, which promise many novel optoelectronic applications. Most of the effects are only accessible by breaking the spatial symmetry, through introducing edges, p-n junctions, or heterogeneous interfaces. The recent development of direct synthesis of lateral heterostructures offers new opportunities to achieve the desired asymmetry. As a proof of concept, we study the photothermoelectric effect in an asymmetric lateral heterojunction between the Dirac semimetallic monolayer graphene and the parabolic semiconducting monolayer MoS2. Very different hot-carrier cooling mechanisms on the graphene and the MoS2 sides allow us to resolve the asymmetric thermalization pathways of photoinduced hot carriers spatially with electrostatic gate tunability. We also demonstrate the potential of graphene-2D semiconductor lateral heterojunctions as broadband infrared photodetectors. The proposed structure shows an extreme in-plane asymmetry and provides a new platform to study light-matter interactions in low-dimensional systems.


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