Atomic-scale characterization of structural and electronic properties of Hf doped β-Ga2O3

2021 ◽  
Vol 119 (17) ◽  
pp. 172102
Author(s):  
Adrian Chmielewski ◽  
Ziling Deng ◽  
Muad Saleh ◽  
Jani Jesenovec ◽  
Wolfgang Windl ◽  
...  
2021 ◽  
Author(s):  
Qiang Sun ◽  
Luis M. Mateos ◽  
Roberto Robles ◽  
Nicolas Lorente ◽  
Pascal Ruffieux ◽  
...  

<p>Porphyrin nanotapes (Por NTs) have attracted vast interest as potential molecular wires thanks to their exceptional electronic properties. Recently, Por NTs have been synthesized by solution-based methods, demonstrating high versatility and great potential for technological applications. However, their synthesis is tedious and their characterization limited by low solubility and stability. Here, we report the first example of meso-meso triply-fused Por NTs, which are prepared from a readily available Por precursor through a two-step synthesis on Au(111). The structural and electronic properties of individual Por NTs are addressed, both on Au(111) and on a thin insulating NaCl layer, by high-resolution scanning probe microscopy/spectroscopy complemented by density functional theory calculations.<br></p>


2021 ◽  
Author(s):  
Qiang Sun ◽  
Luis M. Mateos ◽  
Roberto Robles ◽  
Nicolas Lorente ◽  
Pascal Ruffieux ◽  
...  

<p>Porphyrin nanotapes (Por NTs) have attracted vast interest as potential molecular wires thanks to their exceptional electronic properties. Recently, Por NTs have been synthesized by solution-based methods, demonstrating high versatility and great potential for technological applications. However, their synthesis is tedious and their characterization limited by low solubility and stability. Here, we report the first example of meso-meso triply-fused Por NTs, which are prepared from a readily available Por precursor through a two-step synthesis on Au(111). The structural and electronic properties of individual Por NTs are addressed, both on Au(111) and on a thin insulating NaCl layer, by high-resolution scanning probe microscopy/spectroscopy complemented by density functional theory calculations.<br></p>


2021 ◽  
Author(s):  
Qiang Sun ◽  
Luis Mateo ◽  
Roberto Robles ◽  
Nicolas Lorente ◽  
Pascal Ruffieux ◽  
...  

Abstract Porphyrin nanotapes (Por NTs) have attracted vast interest as potential molecular wires thanks to their exceptional electronic properties. Recently, Por NTs have been synthesized by solution-based methods, demonstrating high versatility and great potential for technological applications. However, their synthesis is tedious and their characterization limited by low solubility and stability. Here, we report the first example of meso-meso triply-fused Por NTs, which are prepared from a readily available Por precursor through a two-step synthesis on Au(111). The structural and electronic properties of individual Por NTs are addressed, both on Au(111) and on a thin insulating NaCl layer, by high-resolution scanning probe microscopy/spectroscopy complemented by density functional theory calculations. Remarkably, the triply-linked Por NTs carry one unpaired electron at each end, which leads to magnetic end states. Our study provides an alternative and versatile route to the fabrication of Por NTs and the atomic-scale characterizations of their structural and electronic properties.


2021 ◽  
Author(s):  
Qiang Sun ◽  
Luis M. Mateos ◽  
Roberto Robles ◽  
Nicolas Lorente ◽  
Pascal Ruffieux ◽  
...  

<p>Porphyrin nanotapes (Por NTs) have attracted vast interest as potential molecular wires thanks to their exceptional electronic properties. Recently, Por NTs have been synthesized by solution-based methods, demonstrating high versatility and great potential for technological applications. However, their synthesis is tedious and their characterization limited by low solubility and stability. Here, we report the first example of meso-meso triply-fused Por NTs, which are prepared from a readily available Por precursor through a two-step synthesis on Au(111). The structural and electronic properties of individual Por NTs are addressed, both on Au(111) and on a thin insulating NaCl layer, by high-resolution scanning probe microscopy/spectroscopy complemented by density functional theory calculations.<br></p>


2019 ◽  
Vol 25 (S2) ◽  
pp. 576-577 ◽  
Author(s):  
M Conroy ◽  
K Moore ◽  
EN O'Connell ◽  
JPV McConville ◽  
H Lu ◽  
...  

2011 ◽  
Vol 98 (18) ◽  
pp. 181904 ◽  
Author(s):  
Shigetaka Tomiya ◽  
Yuya Kanitani ◽  
Shinji Tanaka ◽  
Tadakatsu Ohkubo ◽  
Kazuhiro Hono

2016 ◽  
Vol 33 (7) ◽  
pp. 419-437 ◽  
Author(s):  
Lidia E. Chinchilla ◽  
Carol Olmos ◽  
Mert Kurttepeli ◽  
Sara Bals ◽  
Gustaaf Van Tendeloo ◽  
...  

2004 ◽  
Vol 10 (S02) ◽  
pp. 452-453
Author(s):  
Hakim Iddir ◽  
Mark Disko ◽  
Nigel D. Browning ◽  
Serdar Ogut

Extended abstract of a paper presented at Microscopy and Microanalysis 2004 in Savannah, Georgia, USA, August 1–5, 2004.


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