Lévy statistics for single molecule spectroscopy in low temperature glass

2001 ◽  
Author(s):  
Eli Barkai
2018 ◽  
Vol 190 ◽  
pp. 04008
Author(s):  
Kamil Karimullin ◽  
Andrei Naumov

Low temperature dynamics (tunneling and vibrational relaxation) in doped polyisobutylene film has been reinvestigated using 2-pulse incoherent photon echo (2IPE) and compared with single-molecule spectroscopy (SMS) data. It has been shown that in a very wide range of low temperatures the 2IPE gives optical dephasing times which correspond to the narrowest zero-phonon lines of single dye molecules.


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