Study of Low-Temperature Dynamics of Amorphous Solids with High Spatial and Spectral Resolution: Single Molecule Spectroscopy

Author(s):  
A.V. Naumov ◽  
Yu.G. Vainer ◽  
M. Bauer ◽  
L. Kador
2018 ◽  
Vol 190 ◽  
pp. 04008
Author(s):  
Kamil Karimullin ◽  
Andrei Naumov

Low temperature dynamics (tunneling and vibrational relaxation) in doped polyisobutylene film has been reinvestigated using 2-pulse incoherent photon echo (2IPE) and compared with single-molecule spectroscopy (SMS) data. It has been shown that in a very wide range of low temperatures the 2IPE gives optical dephasing times which correspond to the narrowest zero-phonon lines of single dye molecules.


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