Iodine-mediated a new avenue to sulfonylation employing N-hydroxy aryl sulfonamide as a sulfonylating agent

2021 ◽  
Author(s):  
Dushyant Singh Raghuvanshi ◽  
Narsingh Verma
Keyword(s):  
Acetylenic Acid ◽  
Highly Efficient ◽  
First Time

A novel and highly efficient I2/K2CO3 mediated regioselective sulfonylation of thiophenols, aryl acetylenic acid, and aromatic alkynes with N-hydroxy sulfonamide has been developed. N-hydroxy sulfonamide has been realized first time...

Pt NPs@GO as a highly efficient and reusable catalyst for one-pot synthesis of acridinedione derivatives

RSC Advances ◽  
2015 ◽  
Vol 5 (61) ◽  
pp. 49295-49300 ◽  
Author(s):  
Handan Pamuk ◽  
Burak Aday ◽  
Fatih Şen ◽  
Muharrem Kaya
Keyword(s):  
Aromatic Aldehydes ◽  
Reusable Catalyst ◽  
One Pot ◽  
Highly Efficient ◽  
One Pot Synthesis ◽  
First Time

Pt NPs@GO has been used for the first time for synthesizing acridinedione from dimedone, aromatic aldehydes and various amines as a catalyst.

scholarly journals 3D Graphene Nanosheets from Plastic Waste for Highly Efficient HTM free Perovskite Solar Cells

2021 ◽  
Author(s):  
Sandeep Pandey ◽  
Amit Kumar ◽  
Manoj Karakoti ◽  
Kuldeep K. Garg ◽  
Aniket Rana ◽  
...  
Keyword(s):  
Solar Cells ◽  
Graphene Nanosheets ◽  
Perovskite Solar Cells ◽  
Hole Transport ◽  
Plastic Waste ◽  
Waste Plastic ◽  
3D Graphene ◽  
Highly Efficient ◽  
First Time

Herein, we report the first time application of waste plastic derived 3D graphene nanosheets (GNs) for hole transport material (HTM) free perovskite solar cells (PSCs), where 3D GNs has been...

Surface activated carbon nitride nanosheets with optimized electro-optical properties for highly efficient photocatalytic hydrogen production

2016 ◽  
Vol 4 (7) ◽  
pp. 2445-2452 ◽  
Author(s):  
Mohammad Ziaur Rahman ◽  
Jingrun Ran ◽  
Youhong Tang ◽  
Mietek Jaroniec ◽  
Shi Zhang Qiao
Keyword(s):  
Optical Properties ◽  
Activated Carbon ◽  
Hydrogen Production ◽  
Carbon Nitride ◽  
Surface Activation ◽  
Step Method ◽  
Highly Efficient ◽  
Thin Carbon ◽  
Carbon Nitride Nanosheets ◽  
First Time

We introduce a three-step method (co-polymerization, surface activation and exfoliation) for the first time to synthesize sub-nanometer-thin carbon nitride nanosheets as highly efficient hydrogen evolution photocatalysts.

Efficient Modulation of Catalytic Performance of Electrocatalytic Nitrogen Reduction with Transition Metal Anchored N/O-codoped Graphene by Coordination Engineering

2021 ◽  
Author(s):  
Xiaolin Wang ◽  
Li-Ming Yang
Keyword(s):  
Nitrogen Fixation ◽  
Transition Metal ◽  
High Throughput ◽  
First Principles ◽  
High Throughput Screening ◽  
Catalytic Performance ◽  
Nitrogen Reduction ◽  
Highly Efficient ◽  
First Time

We for the first time report the discovery of a series of highly efficient electrocatalysts, i.e., transition metal anchored N/O-codoped graphene, for nitrogen fixation via high-throughput screening combined with first-principles...

scholarly journals Efficient Nonrecursive Bit-Parallel Karatsuba Multiplier for a Special Class of Trinomials

VLSI Design ◽  
2018 ◽  
Vol 2018 ◽  
pp. 1-7 ◽  
Author(s):  
Yin Li ◽  
Yu Zhang ◽  
Xiaoli Guo
Keyword(s):  
Time Delay ◽  
Special Class ◽  
Time Complexity ◽  
Space Complexity ◽  
Polynomial Basis ◽  
Gate Delay ◽  
Complexity Bound ◽  
Parallel Multiplier ◽  
Highly Efficient ◽  
First Time

Recently, we present a novel Mastrovito form of nonrecursive Karatsuba multiplier for all trinomials. Specifically, we found that related Mastrovito matrix is very simple for equally spaced trinomial (EST) combined with classic Karatsuba algorithm (KA), which leads to a highly efficient Karatsuba multiplier. In this paper, we consider a new special class of irreducible trinomial, namely, xm+xm/3+1. Based on a three-term KA and shifted polynomial basis (SPB), a novel bit-parallel multiplier is derived with better space and time complexity. As a main contribution, the proposed multiplier costs about 2/3 circuit gates of the fastest multipliers, while its time delay matches our former result. To the best of our knowledge, this is the first time that the space complexity bound is reached without increasing the gate delay.

Immobilizing AgPd alloy on Vulcan XC-72 carbon: a novel catalyst for highly efficient hydrogen generation from formaldehyde aqueous solution

RSC Advances ◽  
2016 ◽  
Vol 6 (107) ◽  
pp. 105638-105643 ◽  
Author(s):  
Shutao Gao ◽  
Tao Feng ◽  
Qiuhua Wu ◽  
Cheng Feng ◽  
Ningzhao Shang ◽  
...  
Keyword(s):  
Aqueous Solution ◽  
Room Temperature ◽  
Hydrogen Generation ◽  
Bimetallic Catalyst ◽  
Highly Efficient ◽  
Novel Catalyst ◽  
First Time

A novel bimetallic catalyst, AgPd nanoalloy supported on Vulcan XC-72 carbon (AgPd@C-72), has been successfully fabricated and used for catalyzing H2 generation from formaldehyde aqueous solution at room temperature for the first time.

Brønsted acidic ionic liquid-catalyzed dehydrative formation of isosorbide from sorbitol: introduction of a continuous process

2017 ◽  
Vol 7 (10) ◽  
pp. 2065-2073 ◽  
Author(s):  
Jie Deng ◽  
Bao-Hua Xu ◽  
Yao-Feng Wang ◽  
Xian-En Mo ◽  
Rui Zhang ◽  
...  
Keyword(s):  
Ionic Liquid ◽  
Ionic Liquids ◽  
Continuous Process ◽  
Efficient Synthesis ◽  
Acidic Ionic Liquid ◽  
Highly Efficient ◽  
Brønsted Acidic Ionic Liquid ◽  
Acidic Ionic Liquids ◽  
First Time

A highly efficient synthesis of isosorbide from sorbitol was developed using Brønsted acidic ionic liquids (BILs) as the catalyst for the first time.

Azo-Compound-Mediated Cyanoalkylation of Alkenes by Copper Catalysis: General Access to Cyano-Substituted Oxindoles

Synthesis ◽  
2015 ◽  
Vol 47 (11) ◽  
pp. 1567-1580 ◽  
Author(s):  
Shi Tang ◽  
Dong Zhou ◽  
Zhi-Hao Li ◽  
Mei-Jun Fu ◽  
Li Jie ◽  
...  
Keyword(s):  
Radical Addition ◽  
Copper Catalysis ◽  
Azo Compound ◽  
Highly Efficient ◽  
First Time ◽  
General Synthesis

A practical and highly efficient azo-compound-mediated/ promoted radical cyanoalkylation of activated alkenes by copper catalysis was developed, which allowed for general synthesis of oxindoles bearing various nitrile moieties, especially the rarely reported 3° nitrile moiety via cascade radical addition/C(sp2)–H cyclization. This protocol demonstrates that DIAD served for a new promoter instead of usual Ag salts or bases in the C(sp3)–H functionalization of acetonitrile for the first time. The use of readily available AIBN and beyond as the radical sources, and inexpensive copper as the catalyst, as well as the simplicity of operation and handling, make this protocol an attractive access to therapeutically important cyano-substituted oxindoles.

Palladium-catalyzed asymmetric formal [3+2] cycloaddition of α-N-heterocyclic acrylates with vinyl epoxides for construction of isonucleoside analogs

2019 ◽  
Vol 55 (90) ◽  
pp. 13550-13553 ◽  
Author(s):  
Ke-Xin Huang ◽  
Ming-Sheng Xie ◽  
Dong-Chao Wang ◽  
Ji-Wei Sang ◽  
Gui-Rong Qu ◽  
...  
Keyword(s):  
Highly Efficient ◽  
Palladium Catalyzed ◽  
First Time

A highly efficient Pd-catalyzed asymmetric formal [3+2] cycloaddition of α-N-heterocyclic acrylates with vinyl epoxides has been developed for the first time.

Laser synthesis of oxygen vacancy-modified CoOOH for highly efficient oxygen evolution

2019 ◽  
Vol 55 (20) ◽  
pp. 2904-2907 ◽  
Author(s):  
Chao Meng ◽  
Mengchang Lin ◽  
Xuechun Sun ◽  
Xiaodong Chen ◽  
Xuemin Chen ◽  
...  
Keyword(s):  
Laser Ablation ◽  
Oxygen Vacancy ◽  
Oxygen Evolution ◽  
Water Oxidation ◽  
Laser Synthesis ◽  
Highly Efficient ◽  
Laser Ablation In Liquids ◽  
First Time

Laser ablation in liquids has been, for the first time, employed to produce oxygen vacancy-modified CoOOH nanosheets for efficient water oxidation.

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