Synergistic effects of lanthanide surface adhesion and photon-upconversion for enhanced near-infrared responsive photodegradation of organic contaminants in wastewater

2020 ◽  
Vol 7 (11) ◽  
pp. 3333-3342
Author(s):  
Jiaying Wang ◽  
Haiying Wang ◽  
Sijin Zuo ◽  
Xuming Jin ◽  
Bingzhu Zheng ◽  
...  
Keyword(s):  
Rhodamine B ◽  
Organic Contaminants ◽  
Near Infrared ◽  
Synergistic Effects ◽  
Light Irradiation ◽  
Ring Cleavage ◽  
Carboxyl Groups ◽  
Surface Adhesion ◽  
Nir Light

Upconversion nanoparticle-TiO2 catalyst with Gd3+-rich surface shows stronger binding coefficiency to the carboxyl groups, resulting in faster ring cleavage and higher mineralization efficiency of rhodamine B under NIR light irradiation.

Near-infrared-activated NaYF4:Yb3+, Er3+/Au/CdS for H2 production via photoreforming of bio-ethanol: plasmonic Au as light nanoantenna, energy relay, electron sink and co-catalyst

2017 ◽  
Vol 5 (21) ◽  
pp. 10311-10320 ◽  
Author(s):  
Wenhui Feng ◽  
Lulu Zhang ◽  
Yan Zhang ◽  
Yu Yang ◽  
Zhibin Fang ◽  
...  
Keyword(s):  
Near Infrared ◽  
H2 Production ◽  
Light Irradiation ◽  
Low Density ◽  
Co Catalyst ◽  
Ethanol Reforming ◽  
Nir Light ◽  
Electron Sink

A sandwich-structured NaYF4:Yb3+, Er3+/Au/CdS architecture delivers enhanced photocatalytic bio-ethanol reforming activity under low-density NIR light irradiation.

Constructing two-dimensional CuFeSe2@Au heterostructured nanosheets with an amorphous core and a crystalline shell for enhanced near-infrared light water oxidation

Nanoscale ◽  
2018 ◽  
Vol 10 (5) ◽  
pp. 2380-2387 ◽  
Author(s):  
Huang Wen ◽  
Hua Li ◽  
Suisui He ◽  
Fengjuan Chen ◽  
Erli Ding ◽  
...  
Keyword(s):  
Photocatalytic Activity ◽  
Water Oxidation ◽  
Near Infrared ◽  
Light Irradiation ◽  
Infrared Light ◽  
Core Shell ◽  
Two Dimensional ◽  
Near Infrared Light ◽  
Light Water ◽  
Nir Light

The reversed growth of 2D core–shell CuFeSe2@Au heterostructured nanosheets with a crystalline shell and an amorphous core were first prepared and show enhanced photocatalytic activity for water oxidation under NIR light irradiation.

scholarly journals Extended Near-Infrared Photoactivity of Bi6Fe1.9Co0.1Ti3O18 by Upconversion Nanoparticles

Nanomaterials ◽  
2018 ◽  
Vol 8 (7) ◽  
pp. 534 ◽  
Author(s):  
Wen Ge ◽  
Zhiang Li ◽  
Tong Chen ◽  
Min Liu ◽  
Yalin Lu
Keyword(s):  
Photocatalytic Activity ◽  
Rhodamine B ◽  
Near Infrared ◽  
Hydrothermal Process ◽  
Upconversion Nanoparticles ◽  
Ferromagnetic Properties ◽  
Optimal Ratio ◽  
Nir Light

Bi6Fe1.9Co0.1Ti3O18 (BFCTO)/NaGdF4:Yb3+, Er3+ (NGF) nanohybrids were successively synthesized by the hydrothermal process followed by anassembly method, and BFCTO-1.0/NGF nanosheets, BFCTO-1.5/NGF nanoplates and BFCTO-2.0/NGF truncated tetragonal bipyramids were obtained when 1.0, 1.5 and 2.0 M NaOH were adopted, respectively. Under the irradiation of 980 nm light, all the BFCTO samples exhibited no activity in degrading Rhodamine B (RhB). In contrast, with the loading of NGF upconversion nanoparticles, all the BFCTO/NGF samples exhibited extended near-infrared photoactivity, with BFCTO-1.5/NGF showing the best photocatalytic activity, which could be attributed to the effect of {001} and {117} crystal facets with the optimal ratio. In addition, the ferromagnetic properties of the BFCTO/NGF samples indicated their potential as novel, recyclable and efficient near-infrared (NIR) light-driven photocatalysts.

scholarly journals Enhanced Delivery of Thermoresponsive Polymer-Based Medicine into Tumors by Using Heat Produced from Gold Nanorods Irradiated with Near-Infrared Light

Cancers ◽  
2021 ◽  
Vol 13 (19) ◽  
pp. 5005
Author(s):  
Kohei Sano ◽  
Yumi Ishida ◽  
Toshie Tanaka ◽  
Tatsuya Mizukami ◽  
Tomono Nagayama ◽  
...  
Keyword(s):  
Gold Nanorods ◽  
Near Infrared ◽  
Drug Carrier ◽  
Light Irradiation ◽  
Infrared Light ◽  
Solution Temperature ◽  
Dependent Manner ◽  
Thermoresponsive Polymer ◽  
Tumor Bearing ◽  
Nir Light

The aim of this study was to establish a drug delivery system (DDS) for marked therapy of tumors using a thermoresponsive polymer, polyoxazoline (POZ). The effectiveness of the following was investigated: (i) the delivery of gold nanorods (GNRs) to tumor tissues, (ii) heat production of GNR upon irradiation with near-infrared (NIR) light, and (iii) high accumulation of an intravenously injected radiolabeled POZ as a drug carrier in tumors by sensing heat produced by GNRs. When the GNR solution was irradiated with NIR light (808 nm), the solution temperature was increased both in a GNR-concentration-dependent manner and in a light-dose-dependent manner. POZ, with a lower critical solution temperature of 38 °C, was aggregated depending on the heat produced by the GNR irradiated by NIR light. When it was intratumorally pre-injected into colon26-tumor-bearing mice, followed by NIR light irradiation (GNR+/Light+ group), the tumor surface temperature increased to approximately 42 °C within 5 min. Fifteen minutes after irradiation with NIR light, indium-111 (111In)-labeled POZ was intravenously injected into tumor-bearing mice, and the radioactivity distribution was evaluated. The accumulation of POZ in the tumor was significantly (approximately 4-fold) higher than that in the control groups (GNR+/without NIR light irradiation (Light–), without injection of GNR (GNR–)/Light+, and GNR–/Light– groups). Furthermore, an in vivo confocal fluorescence microscopy study, using fluorescence-labeled POZ, revealed that uptake of POZ by the tumor could be attributed to the heat produced by GNR. In conclusion, we successfully established a novel DDS in which POZ could be efficiently delivered into tumors by using the heat produced by GNR irradiated with NIR light.

A perylene diimide zwitterionic polymer for photoacoustic imaging guided photothermal/photodynamic synergistic therapy with single near-infrared irradiation

2018 ◽  
Vol 6 (20) ◽  
pp. 3395-3403 ◽  
Author(s):  
Pengfei Sun ◽  
Xiaoxiao Wang ◽  
Gaina Wang ◽  
Weixing Deng ◽  
Qingming Shen ◽  
...  
Keyword(s):  
Near Infrared ◽  
Photoacoustic Imaging ◽  
Perylene Diimide ◽  
Light Irradiation ◽  
Infrared Irradiation ◽  
Nir Light ◽  
Zwitterionic Polymer

A biocompatible zwitterionic polymer (PDS-PDI) was designed for PAI guided synergistic PDT and PTT with single NIR light irradiation.

Enhancement of ultralow-intensity NIR light-triggered photodynamic therapy based on exo- and endogenous synergistic effects through combined glutathione-depletion chemotherapy

Nanoscale ◽  
2019 ◽  
Vol 11 (27) ◽  
pp. 13078-13088 ◽  
Author(s):  
Jun-hui Shi ◽  
Tian-ran Wang ◽  
Yong-qiang You ◽  
Muhammad Luqman Akhtar ◽  
Zong-jun Liu ◽  
...  
Keyword(s):  
Photodynamic Therapy ◽  
Near Infrared ◽  
Synergistic Effects ◽  
Glutathione Depletion ◽  
Infrared Light ◽  
Near Infrared Light ◽  
Nir Light

An ultralow-intensity (0.30 W cm−2) near-infrared light-triggered PDT was developed and enhanced through combination of GSH-depletion chemotherapy based on both exo- and endogenous synergistic effects.

scholarly journals Nanomaterials for the Photothermal Killing of Bacteria

Nanomaterials ◽  
2020 ◽  
Vol 10 (6) ◽  
pp. 1123 ◽  
Author(s):  
Sibidou Yougbaré ◽  
Chinmaya Mutalik ◽  
Dyah Ika Krisnawati ◽  
Heny Kristanto ◽  
Achmad Jazidie ◽  
...  
Keyword(s):  
Human Health ◽  
Structural Properties ◽  
Near Infrared ◽  
Antibacterial Activities ◽  
Multidrug Resistant ◽  
Clinical Applications ◽  
Light Irradiation ◽  
Nir Light ◽  
Current Trends ◽  
Bactericidal Effects

An upsurge in the multidrug-resistant (MDR) bacterial pestilence is a global cause for concern in terms of human health. Lately, nanomaterials with photothermal effects have assisted in the efficient killing of MDR bacteria, attributable to their uncommon plasmonic, photocatalytic, and structural properties. Examinations of substantial amounts of photothermally enabled nanomaterials have shown bactericidal effects in an optimized time under near-infrared (NIR) light irradiation. In this review, we have compiled recent advances in photothermally enabled nanomaterials for antibacterial activities and their mechanisms. Photothermally enabled nanomaterials are classified into three groups, including metal-, carbon-, and polymer-based nanomaterials. Based on substantial accomplishments with photothermally enabled nanomaterials, we have inferred current trends and their prospective clinical applications.

Catalyst Halogenation Enables Rapid and Efficient Polymerizations with Visible to Near-Infrared Light

2020 ◽  
Author(s):  
Alex Stafford ◽  
Dowon Ahn ◽  
Emily Raulerson ◽  
Kun-You Chung ◽  
Kaihong Sun ◽  
...  
Keyword(s):  
Near Infrared ◽  
Transient Absorption ◽  
Reaction Times ◽  
Infrared Light ◽  
Structure Property ◽  
Light Emitting ◽  
Structure Property Relationships ◽  
Nir Light ◽  
Light Intensities ◽  
Emission Quenching

Driving rapid polymerizations with visible to near-infrared (NIR) light will enable nascent technologies in the emerging fields of bio- and composite-printing. However, current photopolymerization strategies are limited by long reaction times, high light intensities, and/or large catalyst loadings. Improving efficiency remains elusive without a comprehensive, mechanistic evaluation of photocatalysis to better understand how composition relates to polymerization metrics. With this objective in mind, a series of methine- and aza-bridged boron dipyrromethene (BODIPY) derivatives were synthesized and systematically characterized to elucidate key structure-property relationships that facilitate efficient photopolymerization driven by visible to NIR light. For both BODIPY scaffolds, halogenation was shown as a general method to increase polymerization rate, quantitatively characterized using a custom real-time infrared spectroscopy setup. Furthermore, a combination of steady-state emission quenching experiments, electronic structure calculations, and ultrafast transient absorption revealed that efficient intersystem crossing to the lowest excited triplet state upon halogenation was a key mechanistic step to achieving rapid photopolymerization reactions. Unprecedented polymerization rates were achieved with extremely low light intensities (< 1 mW/cm<sup>2</sup>) and catalyst loadings (< 50 μM), exemplified by reaction completion within 60 seconds of irradiation using green, red, and NIR light-emitting diodes.

Bi19S27I3 nanorods: a new candidate for photothermal therapy in the first and second biological near-infrared windows

Nanoscale ◽  
2021 ◽  
Author(s):  
Jinsong Xiong ◽  
Qinghuan Bian ◽  
Shuijin Lei ◽  
Yatian Deng ◽  
Kehan Zhao ◽  
...  
Keyword(s):  
Cancer Therapy ◽  
Photothermal Therapy ◽  
Near Infrared ◽  
Research Interest ◽  
The Past ◽  
Nir Light ◽  
Considerable Research ◽  
Key Factor

Near-infrared (NIR) light induced photothermal cancer therapy using nanomaterials as photothermal agents has attracted considerable research interest over the past few years. As the key factor in the photothermal therapy...

scholarly journals Near-Infrared-Triggered Upconverting Nanoparticles for Biomedicine Applications

Biomedicines ◽  
2021 ◽  
Vol 9 (7) ◽  
pp. 756
Author(s):  
Manoj Kumar Mahata ◽  
Ranjit De ◽  
Kang Taek Lee
Keyword(s):  
Drug Delivery ◽  
Photothermal Therapy ◽  
Near Infrared ◽  
Cutting Edge ◽  
Clinical Translation ◽  
Basic Knowledge ◽  
Nanotechnology Research ◽  
Nir Light

Due to the unique properties of lanthanide-doped upconverting nanoparticles (UCNP) under near-infrared (NIR) light, the last decade has shown a sharp progress in their biomedicine applications. Advances in the techniques for polymer, dye, and bio-molecule conjugation on the surface of the nanoparticles has further expanded their dynamic opportunities for optogenetics, oncotherapy and bioimaging. In this account, considering the primary benefits such as the absence of photobleaching, photoblinking, and autofluorescence of UCNPs not only facilitate the construction of accurate, sensitive and multifunctional nanoprobes, but also improve therapeutic and diagnostic results. We introduce, with the basic knowledge of upconversion, unique properties of UCNPs and the mechanisms involved in photon upconversion and discuss how UCNPs can be implemented in biological practices. In this focused review, we categorize the applications of UCNP-based various strategies into the following domains: neuromodulation, immunotherapy, drug delivery, photodynamic and photothermal therapy, bioimaging and biosensing. Herein, we also discuss the current emerging bioapplications with cutting edge nano-/biointerfacing of UCNPs. Finally, this review provides concluding remarks on future opportunities and challenges on clinical translation of UCNPs-based nanotechnology research.

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