scholarly journals Building better all-solid-state batteries with Li-garnet solid electrolytes and metalloid anodes

2019 ◽  
Vol 7 (37) ◽  
pp. 21299-21308 ◽  
Author(s):  
Semih Afyon ◽  
Kostiantyn V. Kravchyk ◽  
Shutao Wang ◽  
Jan van den Broek ◽  
Christian Hänsel ◽  
...  
Keyword(s):  
Energy Storage ◽  
Solid State ◽  
Solid Electrolytes ◽  
Energy Storage Devices ◽  
Storage Devices ◽  
The Core ◽  
Solid State Batteries ◽  
All Solid State Batteries

All-solid-state batteries provide new opportunities to realize safe, non-flammable, and temperature-tolerant energy storage and display a huge potential to be the core of future energy storage devices.

scholarly journals Cathode–Sulfide Solid Electrolyte Interfacial Instability: Challenges and Solutions

2020 ◽  
Author(s):  
Teerth Brahmbhatt ◽  
◽  
Guang Yang ◽  
Ethan Self ◽  
Jagjit Nanda ◽  
...  
Keyword(s):  
Energy Storage ◽  
Solid State ◽  
Ionic Conductivity ◽  
Energy Density ◽  
Interfacial Instability ◽  
Energy Storage Devices ◽  
Storage Devices ◽  
Solid State Batteries ◽  
All Solid State Batteries ◽  
Solid State Electrolytes

All-solid-state batteries are a candidate for next-generation energy-storage devices due to potential improvements in energy density and safety compared to current battery technologies. Due to their high ionic conductivity and potential scalability through slurry processing routes, sulfide solid-state electrolytes are promising to replace traditional liquid electrolytes and enable All-solid-state batteries, but stability of cathode-sulfide solid-state electrolytes interfaces requires further improvement. Herein we review common issues encountered at cathode-sulfide SE interfaces and strategies to alleviate these issues.

scholarly journals Recycling Strategies for Ceramic All-Solid-State Batteries—Part I: Study on Possible Treatments in Contrast to Li-Ion Battery Recycling

Metals ◽  
2020 ◽  
Vol 10 (11) ◽  
pp. 1523
Author(s):  
Lilian Schwich ◽  
Michael Küpers ◽  
Martin Finsterbusch ◽  
Andrea Schreiber ◽  
Dina Fattakhova-Rohlfing ◽  
...  
Keyword(s):  
Energy Storage ◽  
Solid State ◽  
Energy Density ◽  
Lithium Ion ◽  
High Energy ◽  
High Energy Density ◽  
Future Research ◽  
Energy Storage Devices ◽  
Solid State Batteries ◽  
All Solid State Batteries

In the coming years, the demand for safe electrical energy storage devices with high energy density will increase drastically due to the electrification of the transportation sector and the need for stationary storage for renewable energies. Advanced battery concepts like all-solid-state batteries (ASBs) are considered one of the most promising candidates for future energy storage technologies. They offer several advantages over conventional Lithium-Ion Batteries (LIBs), especially with regard to stability, safety, and energy density. Hardly any recycling studies have been conducted, yet, but such examinations will play an important role when considering raw materials supply, sustainability of battery systems, CO2 footprint, and general strive towards a circular economy. Although different methods for recycling LIBs are already available, the transferability to ASBs is not straightforward due to differences in used materials and fabrication technologies, even if the chemistry does not change (e.g., Li-intercalation cathodes). Challenges in terms of the ceramic nature of the cell components and thus the necessity for specific recycling strategies are investigated here for the first time. As a major result, a recycling route based on inert shredding, a subsequent thermal treatment, and a sorting step is suggested, and transferring the extracted black mass to a dedicated hydrometallurgical recycling process is proposed. The hydrometallurgical approach is split into two scenarios differing in terms of solubility of the ASB-battery components. Hence, developing a full recycling concept is reached by this study, which will be experimentally examined in future research.

Critical role of zeolites as H2S scavengers in argyrodite Li6PS5Cl solid electrolytes for all-solid-state batteries

2021 ◽  
Author(s):  
Donggun Lee ◽  
Kern-Ho Park ◽  
So Yeun Kim ◽  
Jae Yup Jung ◽  
Wonrak Lee ◽  
...  
Keyword(s):  
Energy Storage ◽  
Solid State ◽  
Solid Electrolytes ◽  
Storage Systems ◽  
Critical Role ◽  
High Energy ◽  
Energy Storage Systems ◽  
Solid State Batteries ◽  
All Solid State Batteries

All-solid-state batteries (ASSBs) with inorganic solid electrolytes (SEs) have received much attention as future energy storage systems owing to their high energy densities and excellent safety. Sulfide-based SEs are considered...

Development of Solid Electrolytes for All-Solid-State Batteries

2019 ◽  
Vol 92 (11) ◽  
pp. 430-434
Author(s):  
Akitoshi HAYASHI ◽  
Atsushi SAKUDA ◽  
Masahiro TATSUMISAGO
Keyword(s):  
Solid State ◽  
Solid Electrolytes ◽  
Solid State Batteries ◽  
All Solid State Batteries

Operando Visualization of Morphological Dynamics in All-Solid-State Batteries

2019 ◽  
Author(s):  
Xiaohan Wu ◽  
Juliette Billaud ◽  
Iwan Jerjen ◽  
Federica Marone ◽  
Yuya Ishihara ◽  
...  
Keyword(s):  
Solid State ◽  
Solid Electrolytes ◽  
Rational Design ◽  
Morphological Evolution ◽  
Active Material ◽  
Composite Layer ◽  
Transference Number ◽  
Thermal Stabilities ◽  
Solid State Batteries ◽  
All Solid State Batteries

<div> <div> <div> <p>All-solid-state batteries are considered as attractive options for next-generation energy storage owing to the favourable properties (unit transference number and thermal stabilities) of solid electrolytes. However, there are also serious concerns about mechanical deformation of solid electrolytes leading to the degradation of the battery performance. Therefore, understanding the mechanism underlying the electro-mechanical properties in SSBs are essentially important. Here, we show three-dimensional and time-resolved measurements of an all-solid-state cell using synchrotron radiation x-ray tomographic microscopy. We could clearly observe the gradient of the electrochemical reaction and the morphological evolution in the composite layer. Volume expansion/compression of the active material (Sn) was strongly oriented along the thickness of the electrode. While this results in significant deformation (cracking) in the solid electrolyte region, we also find organized cracking patterns depending on the particle size and their arrangements. This study based on operando visualization therefore opens the door towards rational design of particles and electrode morphology for all-solid-state batteries. </p> </div> </div> </div>

Flexible all-solid-state fiber-shaped Ni–Fe batteries with high electrochemical performance

2019 ◽  
Vol 7 (2) ◽  
pp. 520-530 ◽  
Author(s):  
Qiulong Li ◽  
Qichong Zhang ◽  
Chenglong Liu ◽  
Juan Sun ◽  
Jiabin Guo ◽  
...  
Keyword(s):  
Energy Storage ◽  
Solid State ◽  
Electrochemical Performance ◽  
High Capacity ◽  
Core Shell ◽  
Next Generation ◽  
Energy Storage Devices ◽  
Storage Devices

The fiber-shaped Ni–Fe battery takes advantage of high capacity of hierarchical CoP@Ni(OH)2 NWAs/CNTF core–shell heterostructure and spindle-like α-Fe2O3/CNTF electrodes to yield outstanding electrochemical performance, demonstrating great potential for next-generation portable wearable energy storage devices.

Single crystal Ni-rich layered cathodes enabling superior performance in all-solid-state batteries with PEO-based solid electrolytes

2021 ◽  
Author(s):  
Maoyi Yi ◽  
Li Jie ◽  
Xin-ming Fan ◽  
Maohui Bai ◽  
Zhi Zhang ◽  
...  
Keyword(s):  
Solid State ◽  
Energy Density ◽  
Single Crystal ◽  
Solid Electrolytes ◽  
High Energy ◽  
High Energy Density ◽  
Superior Performance ◽  
Composite Electrolytes ◽  
Solid State Batteries ◽  
All Solid State Batteries

PEO-based composite electrolytes are one of the most practical electrolytes in all-solid batteries (ASSBs). To achieve the perspective of ASSBs with high energy density, PEO based composite electrolytes should match...

Three-dimensional MXene/BCN Microflowers for Wearable All-solid-state microsupercapacitors

2021 ◽  
Author(s):  
Dan Tu ◽  
Wenyao Yang ◽  
Yi Li ◽  
Yujiu Zhou ◽  
LiuWei Shi ◽  
...  
Keyword(s):  
Energy Storage ◽  
Solid State ◽  
Three Dimensional ◽  
Energy Storage Devices ◽  
Flexible Electrode ◽  
Storage Devices

Abstract: Modified MXene (Ti3C2Tx) is attractive as a flexible electrode for wearable energy storage devices. In this work, a convenient and effective method was proposed to change the conventional 2D...

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