Advantageous crystalline–amorphous phase boundary for enhanced electrochemical water oxidation

2019 ◽  
Vol 12 (8) ◽  
pp. 2443-2454 ◽  
Author(s):  
HyukSu Han ◽  
Heechae Choi ◽  
Sungwook Mhin ◽  
Yu-Rim Hong ◽  
Kang Min Kim ◽  
...  
Keyword(s):  
Phase Boundary ◽  
Water Splitting ◽  
Amorphous Phase ◽  
Water Oxidation ◽  
High Performance ◽  
Cost Effective ◽  
Effective Strategy

Crystalline–amorphous phase boundary engineering can be an effective strategy to develop cost-effective and high-performance electrocatalysts for water splitting.

Facile construction of self-supported Fe-doped Ni3S2 nanoparticle arrays for ultralow-overpotential oxygen evolution reaction

Nanoscale ◽  
2020 ◽  
Author(s):  
Ning Xie ◽  
Dong-Dong Ma ◽  
Xintao Wu ◽  
Qi-Long Zhu
Keyword(s):  
Water Splitting ◽  
Oxygen Evolution ◽  
Oxygen Evolution Reaction ◽  
Water Oxidation ◽  
High Performance ◽  
Cost Effective ◽  
Nanoparticle Arrays ◽  
Overall Water Splitting ◽  
Construction Of Self ◽  
One Step

Constructing high-performance and cost-effective electrocatalysts for water oxidation, particularly for overall water splitting is extremely needed, whereas still challenging. Herein, based on an economical and facile one-step surface sulfurization strategy,...

Rational design of cobalt–chromium layered double hydroxide as a highly efficient electrocatalyst for water oxidation

2016 ◽  
Vol 4 (29) ◽  
pp. 11292-11298 ◽  
Author(s):  
Chenlong Dong ◽  
Xiaotao Yuan ◽  
Xin Wang ◽  
Xiangye Liu ◽  
Wujie Dong ◽  
...  
Keyword(s):  
Water Splitting ◽  
Oxygen Evolution ◽  
Layered Double Hydroxide ◽  
Water Oxidation ◽  
High Performance ◽  
Rational Design ◽  
Cost Effective ◽  
Cobalt Chromium ◽  
Electrochemical Water Splitting ◽  
Double Hydroxide

The design of a high performance, stable and cost-effective electrocatalyst for oxygen evolution is crucial for H2 production from electrochemical water splitting.

Fe, Ni-codoped W18O49 grown on nickel foam as bifunctional electrocatalyst for boosted water splitting

2021 ◽  
Author(s):  
Guojuan Hai ◽  
Jianfeng Huang ◽  
Liyun Cao ◽  
Koji Kajiyoshi ◽  
Long Wang ◽  
...  
Keyword(s):  
Renewable Energy ◽  
Water Splitting ◽  
High Performance ◽  
Solvothermal Method ◽  
Nickel Foam ◽  
Energy Systems ◽  
Cost Effective ◽  
Bifunctional Catalysts ◽  
Renewable Energy Systems ◽  
Bifunctional Electrocatalyst

Designing cost-effective bifunctional catalysts with high-performance and durability is of great significance for the renewable energy systems. Herein, a typical Fe, Ni-codoped W18O49/NF was prepared via a simple solvothermal method....

scholarly journals A ruthenium-based catalyst on carbon electrodes for electrochemical water splitting

2021 ◽  
Author(s):  
Lin Li ◽  
Biswanath Das ◽  
Ahibur Rahaman ◽  
Andrey Shatskiy ◽  
Fei Ye ◽  
...  
Keyword(s):  
Water Splitting ◽  
Water Oxidation ◽  
State Of The Art ◽  
Cost Effective ◽  
Molecular Catalyst ◽  
Electrolysis Cells ◽  
Multi Walled Carbon Nanotubes ◽  
Energy Economy ◽  
Electrochemical Water Splitting ◽  
Walled Carbon Nanotubes

Electrochemical water splitting constitutes one of the most promising strategies for converting water into hydrogen-based fuels, and this technology is predicted to play a key role in our transition towards a carbon-neutral energy economy. To enable the design of cost-effective electrolysis cells based on this technology, new and more efficient anodes with augmented water splitting activity and stability will be required. Herein, we report an active molecular Ru-based catalyst for electrochemically-driven water oxidation and two simple methods for preparing anodes by attaching this catalyst onto multi-walled carbon nanotubes. The anodes modified with the molecular catalyst were characterized by a broad toolbox of microscopy and spectroscope techniques, and interestingly no RuO2 formation was detected during electrocatalysis over 4 h. These results demonstrate that the herein presented strategy can be used to prepare anodes that rival the performance of state-of-the-art metal oxide anodes.

Large area high-performance bismuth vanadate photoanode for efficient solar water splitting

2020 ◽  
Vol 8 (7) ◽  
pp. 3845-3850 ◽  
Author(s):  
Meirong Huang ◽  
Wenhai Lei ◽  
Min Wang ◽  
Shuji Zhao ◽  
Changli Li ◽  
...  
Keyword(s):  
Water Splitting ◽  
Water Oxidation ◽  
High Performance ◽  
Large Scale ◽  
Photocurrent Density ◽  
Large Area ◽  
Solar Water ◽  
Solar Water Splitting ◽  
Harsh Conditions ◽  
Density Of Water

Large-scale BiVO4 photoanodes were prepared for solar water splitting. A photocurrent density of water oxidation of ∼2.23 mA cm−2 at 1.23 VRHE and ∼0.83% conversion efficiency at 0.65 VRHE were achieved, with <4% decay after 5 h of operation under harsh conditions.

scholarly journals Effective calcium doping at the B-site of BaFeO3−δ perovskite: towards low-cost and high-performance oxygen permeation membranes

2017 ◽  
Vol 5 (17) ◽  
pp. 7999-8009 ◽  
Author(s):  
Yao Lu ◽  
Hailei Zhao ◽  
Kui Li ◽  
Xuefei Du ◽  
Yanhui Ma ◽  
...  
Keyword(s):  
High Performance ◽  
Oxygen Permeability ◽  
Low Cost ◽  
Cost Effective ◽  
Oxygen Permeation ◽  
Effective Strategy ◽  
Highly Efficient ◽  
Cost Effective Strategy ◽  
Calcium Doping

A highly efficient and cost-effective strategy for doping Ca at the B-site of BaFeO3−δ was demonstrated to enhance oxygen permeability.

Cobalt and nitrogen co-doped Ni3S2 nanoflowers on nickel foam as high-efficiency electrocatalysts for overall water splitting in alkaline media

2021 ◽  
Author(s):  
Xiaoqiang Du ◽  
Guangyu Ma ◽  
Xiaoshuang Zhang
Keyword(s):  
Water Splitting ◽  
High Performance ◽  
High Efficiency ◽  
Nickel Foam ◽  
Water Electrolysis ◽  
Cost Effective ◽  
Alkaline Media ◽  
Co Doping ◽  
Production Industry

The development of high-performance and cost-effective bifunctional water splitting catalysts are of enormous significance to the hydrogen production industry from water electrolysis. Herein, an in-situ Co and N co-doping method...

scholarly journals Enhanced stability and ultrahigh activity of amorphous ripple nanostructured Ni-doped Fe oxyhydroxide electrode toward synergetic electrocatalytic water splitting

RSC Advances ◽  
2020 ◽  
Vol 10 (44) ◽  
pp. 26364-26373
Author(s):  
Selvam Mathi ◽  
Jayaraman Jayabharathi
Keyword(s):  
Water Splitting ◽  
Oxygen Evolution ◽  
Oxygen Evolution Reaction ◽  
High Performance ◽  
Cost Effective ◽  
Renewable Electricity ◽  
Fuels And Chemicals ◽  
Enhanced Stability

The development of high-performance catalysts for oxygen-evolution reaction (OER) is paramount for cost-effective conversion of renewable electricity to fuels and chemicals.

scholarly journals Free-base Porphyrin Polymer for Bifunctional Electrochemical Water Splitting

2021 ◽  
Author(s):  
Yulu Ge ◽  
Zhenhua Lyu ◽  
Mariana Marcos Hernandez ◽  
Dino Villagran
Keyword(s):  
Water Splitting ◽  
Water Oxidation ◽  
Precious Metals ◽  
Cost Effective ◽  
Economic Feasibility ◽  
Free Base ◽  
Bifunctional Electrocatalyst ◽  
Energy Demands ◽  
Production Of Hydrogen ◽  
Electrochemical Water Splitting

Projected future global energy demands require sustainable energy sources as alternatives to the current world dependence on hydrocarbon fuels. The production of hydrogen and oxygen gas from water is a promising approach. Currently, water-splitting electrolyzers require precious metals as electrocalysts because they are active and stable. Yet, replacement of these precious metals by cost-effective alternatives is necessary for the economic feasibility of this approach. Here, we describe a molecular based polymeric approach that effectively removes the need to use any metal to electrochemically split water. The incorporation of free-base porphyrin units into a 2D network structure yields a stable and efficient bifunctional electrocatalyst for water oxidation and water reduction that can operate for days at competitive overpotentials comparable to metal based ones. <br><br><br>

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