A graphene oxide-mediated polyelectrolyte with high ion-conductivity for highly stretchable and self-healing all-solid-state supercapacitors

2018 ◽  
Vol 6 (40) ◽  
pp. 19463-19469 ◽  
Author(s):  
Xuting Jin ◽  
Guoqiang Sun ◽  
Hongsheng Yang ◽  
Guofeng Zhang ◽  
Yukun Xiao ◽  
...  

New polyelectrolytes based on polyacrylic acid cross-linked by methacrylated graphene oxide enable the fabrication of self-healing supercapacitors and stretchable supercapacitors.

2019 ◽  
Vol 7 (43) ◽  
pp. 24814-24829 ◽  
Author(s):  
Yitian Wang ◽  
Qiang Chang ◽  
Rixing Zhan ◽  
Kaige Xu ◽  
Ying Wang ◽  
...  

A versatile hydrogel with extraordinary mechanical strength and self-healing efficiency was developed by integrating physically crosslinked graphene oxide into a chemically crosslinked polyacrylic acid network.


Author(s):  
Cheng Wang ◽  
RuiJing Li ◽  
Peng Chen ◽  
Yongsheng Fu ◽  
XinYan Ma ◽  
...  

A highly stretchable (extensibility > 4000% and stress > 130 kPa), adhesive (weight loading > 200 g), non-flammable and notch-insensitive intrinsic self-healing solid-state polymer electrolyte is designed for stable and safe flexible batteries.


RSC Advances ◽  
2021 ◽  
Vol 11 (45) ◽  
pp. 27801-27811
Author(s):  
M. Vandana ◽  
Y. S. Nagaraju ◽  
H. Ganesh ◽  
S. Veeresh ◽  
H. Vijeth ◽  
...  

Representation of the synthesis steps of SnO2QDs/GO/PPY ternary composites and SnO2QDs/GO/PPY//GO/charcoal asymmetric supercapacitor device.


2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Yuyan Wang ◽  
Xin Huang ◽  
Xinxing Zhang

AbstractSelf-healing materials integrated with excellent mechanical strength and simultaneously high healing efficiency would be of great use in many fields, however their fabrication has been proven extremely challenging. Here, inspired by biological cartilage, we present an ultrarobust self-healing material by incorporating high density noncovalent bonds at the interfaces between the dentritic tannic acid-modified tungsten disulfide nanosheets and polyurethane matrix to collectively produce a strong interfacial interaction. The resultant nanocomposite material with interwoven network shows excellent tensile strength (52.3 MPa), high toughness (282.7 MJ m‒3, which is 1.6 times higher than spider silk and 9.4 times higher than metallic aluminum), high stretchability (1020.8%) and excellent healing efficiency (80–100%), which overturns the previous understanding of traditional noncovalent bonding self-healing materials where high mechanical robustness and healing ability are mutually exclusive. Moreover, the interfacical supramolecular crosslinking structure enables the functional-healing ability of the resultant flexible smart actuation devices. This work opens an avenue toward the development of ultrarobust self-healing materials for various flexible functional devices.


Materials ◽  
2021 ◽  
Vol 14 (14) ◽  
pp. 3790
Author(s):  
Yongzheng Ji ◽  
Tsuyoshi Honma ◽  
Takayuki Komatsu

Sodium super ionic conductor (NASICON)-type Na3Zr2Si2PO12 (NZSP) with the advantages of the high ionic conductivity, stability and safety is one of the most famous solid-state electrolytes. NZSP, however, requires the high sintering temperature about 1200 °C and long sintering time in the conventional solid-state reaction (SSR) method. In this study, the liquid-phase sintering (LPS) method was applied to synthesize NZSP with the use of NaPO3 glass with a low glass transition temperature of 292 °C. The formation of NZSP was confirmed by X-ray diffraction analyses in the samples obtained by the LPS method for the mixture of Na2ZrSi2O7, ZrO2, and NaPO3 glass. The sample sintered at 1000 °C for 10 h exhibited a higher Na+ ion conductivity of 1.81 mS/cm at 100 °C and a lower activation energy of 0.18 eV compared with the samples prepared by the SSR method. It is proposed that a new LPE method is effective for the synthesis of NZSP and the NaPO3 glass has a great contribution to the Na+ diffusion at the grain boundaries.


2021 ◽  
Vol 13 (7) ◽  
pp. 9043-9052
Author(s):  
Peiyao Qu ◽  
Chi Lv ◽  
Yuhao Qi ◽  
Lu Bai ◽  
Junping Zheng

2019 ◽  
Vol 129 ◽  
pp. 285-291 ◽  
Author(s):  
Jing Li ◽  
Zhenwei Li ◽  
Qingkang Feng ◽  
Hanxun Qiu ◽  
Guangzhi Yang ◽  
...  

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