scholarly journals Size and shape dependent photoluminescence and excited state decay rates of diamondoids

2014 ◽  
Vol 16 (7) ◽  
pp. 3070-3076 ◽  
Author(s):  
Robert Richter ◽  
David Wolter ◽  
Tobias Zimmermann ◽  
Lasse Landt ◽  
Andre Knecht ◽  
...  
2015 ◽  
Vol 17 (48) ◽  
pp. 32574-32575
Author(s):  
Robert Richter ◽  
David Wolter ◽  
Tobias Zimmermann ◽  
Lasse Landt ◽  
Andre Knecht ◽  
...  

Correction for ‘Size and shape dependent photoluminescence and excited state decay rates of diamondoids’ by Robert Richter et al., Phys. Chem. Chem. Phys., 2014, 16, 3070–3076.


Author(s):  
Dionisis Stefanatos ◽  
Emmanuel Paspalakis

Abstract We use optimal control theory to show that for a closed Λ-system where the excited intermediate level decays to the lower levels with a common large rate, the optimal scheme for population transfer between the lower levels is actually optical pumping. In order to obtain this result we exploit the large decay rate to eliminate adiabatically the weakly coupled excited state, then perform a transformation to the basis comprised of the dark and bright states, and finally apply optimal control to this transformed system. Subsequently, we confirm the optimality of the optical pumping scheme for the original closed Λ-system using numerical optimal control. We also demonstrate numerically that optical pumping remains optimal when the decay rate to the target state is larger than that to the initial state or the two rates are not very different from each other. The present work is expected to find application in various tasks of quantum information processing, where such systems are encountered


Author(s):  
Bianca Seidler ◽  
Maria Sittig ◽  
Clara Zens ◽  
Jens H. Tran ◽  
Carolin Müller ◽  
...  

2019 ◽  
Vol 4 (22) ◽  
pp. 6702-6712
Author(s):  
Mostofa Ataur Rohman ◽  
Dipankar Sutradhar ◽  
Prakriti Ranjan Bangal ◽  
Asit K. Chandra ◽  
Sivaprasad Mitra

RSC Advances ◽  
2020 ◽  
Vol 10 (23) ◽  
pp. 13442-13450
Author(s):  
Aimin Duan ◽  
Suosuo An ◽  
Jiadan Xue ◽  
Xuming Zheng ◽  
Yanying Zhao

The excited state decay process of N-heterocyclic compounds is attracting increasing attention due to their fundamental applications in pharmaceutical and biological sciences.


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