Thermal Vibration Correlation Function Formalism for Molecular Excited State Decay Rates

2020 ◽  
Vol 38 (11) ◽  
pp. 1223-1232 ◽  
Author(s):  
Zhigang Shuai
Keyword(s):  
Correlation Function ◽  
Excited State ◽  
Decay Rates ◽  
Thermal Vibration ◽  
State Decay ◽  
Function Formalism ◽  
Molecular Excited State

scholarly journals Size and shape dependent photoluminescence and excited state decay rates of diamondoids

2014 ◽  
Vol 16 (7) ◽  
pp. 3070-3076 ◽  
Author(s):  
Robert Richter ◽  
David Wolter ◽  
Tobias Zimmermann ◽  
Lasse Landt ◽  
Andre Knecht ◽  
...  
Keyword(s):  
Excited State ◽  
Decay Rates ◽  
Size And Shape ◽  
State Decay

scholarly journals Correction: Size and shape dependent photoluminescence and excited state decay rates of diamondoids

2015 ◽  
Vol 17 (48) ◽  
pp. 32574-32575
Author(s):  
Robert Richter ◽  
David Wolter ◽  
Tobias Zimmermann ◽  
Lasse Landt ◽  
Andre Knecht ◽  
...  
Keyword(s):  
Excited State ◽  
Chem Phys ◽  
Decay Rates ◽  
Size And Shape ◽  
State Decay ◽  
Phys Chem Chem Phys

Correction for ‘Size and shape dependent photoluminescence and excited state decay rates of diamondoids’ by Robert Richter et al., Phys. Chem. Chem. Phys., 2014, 16, 3070–3076.

On the optimality of optical pumping for a closed Λ-system with large decay rates of the intermediate excited state

2021 ◽  
Author(s):  
Dionisis Stefanatos ◽  
Emmanuel Paspalakis
Keyword(s):  
Optimal Control ◽  
Excited State ◽  
Decay Rate ◽  
Optimal Control Theory ◽  
Optical Pumping ◽  
Quantum Information Processing ◽  
Decay Rates ◽  
Population Transfer ◽  
Initial State ◽  
Weakly Coupled

Abstract We use optimal control theory to show that for a closed Λ-system where the excited intermediate level decays to the lower levels with a common large rate, the optimal scheme for population transfer between the lower levels is actually optical pumping. In order to obtain this result we exploit the large decay rate to eliminate adiabatically the weakly coupled excited state, then perform a transformation to the basis comprised of the dark and bright states, and finally apply optimal control to this transformed system. Subsequently, we confirm the optimality of the optical pumping scheme for the original closed Λ-system using numerical optimal control. We also demonstrate numerically that optical pumping remains optimal when the decay rate to the target state is larger than that to the initial state or the two rates are not very different from each other. The present work is expected to find application in various tasks of quantum information processing, where such systems are encountered

Modulating the Excited-State Decay Pathways of Cu(I) 4H-Imidazolate Complexes by Excitation Wavelength and Ligand Backbone

2021 ◽  
Author(s):  
Bianca Seidler ◽  
Maria Sittig ◽  
Clara Zens ◽  
Jens H. Tran ◽  
Carolin Müller ◽  
...  
Keyword(s):  
Excited State ◽  
Excitation Wavelength ◽  
State Decay

Excited State Decay Dynamics in 3‐Formyl‐4‐hydroxy Benzoic Acid: Understanding the Global Picture of an ESIPT‐Driven Multiple‐Emissive Species

2019 ◽  
Vol 4 (22) ◽  
pp. 6702-6712
Author(s):  
Mostofa Ataur Rohman ◽  
Dipankar Sutradhar ◽  
Prakriti Ranjan Bangal ◽  
Asit K. Chandra ◽  
Sivaprasad Mitra
Keyword(s):  
Excited State ◽  
Benzoic Acid ◽  
State Decay
Sign in / Sign up

Export Citation Format

Share Document