scholarly journals In-situ measurement of the heat transport in defect- engineered free-standing single-layer graphene

2016 ◽  
Vol 6 (1) ◽  
Author(s):  
Haidong Wang ◽  
Kosaku Kurata ◽  
Takanobu Fukunaga ◽  
Hiroshi Takamatsu ◽  
Xing Zhang ◽  
...  
2021 ◽  
Vol 7 (9) ◽  
pp. eabf0116
Author(s):  
Shiqi Huang ◽  
Shaoxian Li ◽  
Luis Francisco Villalobos ◽  
Mostapha Dakhchoune ◽  
Marina Micari ◽  
...  

Etching single-layer graphene to incorporate a high pore density with sub-angstrom precision in molecular differentiation is critical to realize the promising high-flux separation of similar-sized gas molecules, e.g., CO2 from N2. However, rapid etching kinetics needed to achieve the high pore density is challenging to control for such precision. Here, we report a millisecond carbon gasification chemistry incorporating high density (>1012 cm−2) of functional oxygen clusters that then evolve in CO2-sieving vacancy defects under controlled and predictable gasification conditions. A statistical distribution of nanopore lattice isomers is observed, in good agreement with the theoretical solution to the isomer cataloging problem. The gasification technique is scalable, and a centimeter-scale membrane is demonstrated. Last, molecular cutoff could be adjusted by 0.1 Å by in situ expansion of the vacancy defects in an O2 atmosphere. Large CO2 and O2 permeances (>10,000 and 1000 GPU, respectively) are demonstrated accompanying attractive CO2/N2 and O2/N2 selectivities.


2017 ◽  
Vol 19 (12) ◽  
pp. 8496-8503 ◽  
Author(s):  
Nicolas Boulanger ◽  
Victor Yu ◽  
Michael Hilke ◽  
Michael F. Toney ◽  
David R. Barbero

In situ X-ray diffraction analysis of P3HT films during cooling down on both Si and G.


2013 ◽  
Vol 88 (7) ◽  
Author(s):  
P. Wachsmuth ◽  
R. Hambach ◽  
M. K. Kinyanjui ◽  
M. Guzzo ◽  
G. Benner ◽  
...  

2018 ◽  
Vol 9 (1) ◽  
Author(s):  
Anna V. Prydatko ◽  
Liubov A. Belyaeva ◽  
Lin Jiang ◽  
Lia M. C. Lima ◽  
Grégory F. Schneider

2017 ◽  
Vol 111 (9) ◽  
pp. 093103 ◽  
Author(s):  
Masahiro Narasaki ◽  
Haidong Wang ◽  
Takashi Nishiyama ◽  
Tatsuya Ikuta ◽  
Koji Takahashi

2019 ◽  
Vol 236 ◽  
pp. 324-328 ◽  
Author(s):  
Mee-Ree Kim ◽  
Imbok Lee ◽  
Keun Soo Kim ◽  
Ki-Chul Kim

Carbon ◽  
2016 ◽  
Vol 99 ◽  
pp. 564-570 ◽  
Author(s):  
Haidong Wang ◽  
Kosaku Kurata ◽  
Takanobu Fukunaga ◽  
Hiroshi Takamatsu ◽  
Xing Zhang ◽  
...  

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