Dehydration of the upper troposphere and lower stratosphere by subvisible cirrus clouds near the tropical tropopause

1996 ◽  
Vol 23 (8) ◽  
pp. 825-828 ◽  
Author(s):  
Eric J. Jensen ◽  
Owen B. Toon ◽  
Leonard Pfister ◽  
Henry B. Selkirk
2005 ◽  
Vol 22 (1) ◽  
pp. 18-29 ◽  
Author(s):  
Ulrich Leiterer ◽  
Horst Dier ◽  
Dagmar Nagel ◽  
Tatjana Naebert ◽  
Dietrich Althausen ◽  
...  

Abstract Routine radiosonde relative humidity (RH) measurements are not reliable as they are presently used in the global upper-air network. The new Lindenberg measuring and evaluation method, which provides RH profile measurements with an accuracy of ±1% RΗ in the temperature range from 35° to −70°C near the tropical tropopause is described. This Standardized Frequencies (FN) method uses a thin-film capacitive polymer sensor of a modified RS90-H Humicap radiosonde. These research humidity reference radiosondes (FN sondes) are used to develop a correction method for operational RS80-A Humicap humidity profiles. All steps of correction and quality control for RS80-A radiosondes are shown: ground-check correction, time-lag and temperature-dependent correction, and the recognition of icing during the ascent. The results of a statistical comparison between FN sondes and RS80-A sondes are presented. Corrected humidity data of operational RS80-A sondes used in Lindenberg (4 times daily) show no bias when compared to FN radiosondes and have an uncertainty of about ±3% RH at the 1 σ or 68% confidence level from 1000 to about 150 hPa. Only a small dry bias of at most −2% RH remains in the lowest part of the boundary layer (up to 500-m height). Finally, some examples of corrected RS80-A RH profiles in cirrus clouds validated by lidar backscattering profiles in a region of the intertropical convergence (Maldive Islands) are demonstrated. The soundings indicate that ice-saturated and ice-supersaturated air above 10-km height were connected with cirrus clouds in all 47 investigated cases, and, second, that the corrected RS80-A RH profiles also provide good quality information on water vapor in the upper troposphere.


2015 ◽  
Vol 15 (11) ◽  
pp. 6467-6486 ◽  
Author(s):  
W. Frey ◽  
R. Schofield ◽  
P. Hoor ◽  
D. Kunkel ◽  
F. Ravegnani ◽  
...  

Abstract. In this study we examine the simulated downward transport and mixing of stratospheric air into the upper tropical troposphere as observed on a research flight during the SCOUT-O3 campaign in connection with a deep convective system. We use the Advanced Research Weather and Research Forecasting (WRF-ARW) model with a horizontal resolution of 333 m to examine this downward transport. The simulation reproduces the deep convective system, its timing and overshooting altitudes reasonably well compared to radar and aircraft observations. Passive tracers initialised at pre-storm times indicate the downward transport of air from the stratosphere to the upper troposphere as well as upward transport from the boundary layer into the cloud anvils and overshooting tops. For example, a passive ozone tracer (i.e. a tracer not undergoing chemical processing) shows an enhancement in the upper troposphere of up to about 30 ppbv locally in the cloud, while the in situ measurements show an increase of 50 ppbv. However, the passive carbon monoxide tracer exhibits an increase, while the observations show a decrease of about 10 ppbv, indicative of an erroneous model representation of the transport processes in the tropical tropopause layer. Furthermore, it could point to insufficient entrainment and detrainment in the model. The simulation shows a general moistening of air in the lower stratosphere, but it also exhibits local dehydration features. Here we use the model to explain the processes causing the transport and also expose areas of inconsistencies between the model and observations.


2014 ◽  
Vol 71 (9) ◽  
pp. 3439-3453 ◽  
Author(s):  
Marta Abalos ◽  
William J. Randel ◽  
Encarna Serrano

Abstract Upwelling across the tropical tropopause exhibits strong subseasonal variability superimposed on the well-known annual cycle, and these variations directly affect temperature and tracers in the tropical lower stratosphere. In this work, the dynamical forcing of tropical upwelling on subseasonal time scales is investigated using the European Centre for Medium-Range Weather Forecasts (ECMWF) Interim Re-Analysis (ERA-Interim) for 1979–2011. Momentum balance diagnostics reveal that transience in lower-stratospheric upwelling is linked to the effects of extratropical wave forcing, with centers of action in the extratropical winter stratosphere and in the subtropical upper troposphere of both hemispheres. The time-dependent forcing in these regions induces a remote coupled response in the zonal mean wind and the meridional circulation (with associated temperature changes), which drives upwelling variability in the tropical stratosphere. This behavior is observed in the reanalysis, consistent with theory. Dynamical patterns reflect distinctive forcing of the shallow versus deep branches of the Brewer–Dobson circulation; the shallow branch is most strongly correlated with wave forcing in the subtropical upper troposphere and lower stratosphere, while the deep branch is mainly influenced by high-latitude planetary waves.


2014 ◽  
Vol 7 (10) ◽  
pp. 10221-10248
Author(s):  
B. C. Kindel ◽  
P. Pilewskie ◽  
K. S. Schmidt ◽  
T. Thornberry ◽  
A. Rollins ◽  
...  

Abstract. Measuring water vapor in the upper troposphere and lower stratosphere is difficult due to the low mixing ratios found there, typically only a few parts per million. Here we examine near infrared spectra acquired with the Solar Spectral Flux Radiometer during the first science phase of the NASA Airborne Tropical Tropopause EXperiment. From the 1400 and 1900 nm absorption bands, we infer water vapor amounts in the tropical tropopause layer and adjacent regions between 14 and 18 km altitude. We compare these measurements to solar transmittance spectra produced with the MODerate resolution atmospheric TRANsmission (MODTRAN) radiative transfer model, using in situ water vapor, temperature, and pressure profiles acquired concurrently with the SSFR spectra. Measured and modeled transmittance values agree within 0.002, with some larger differences in the 1900 nm band (up to 0.004). Integrated water vapor amounts along the absorption path lengths of 3 to 6 km varied from 1.26 × 10−4 to 4.59 × 10−4 g cm−2. A 0.002 difference in absorptance at 1367 nm results in a 3.35 × 10−5 g cm−2 change of integrated water vapor amount, 0.004 absorptance change at 1870 nm results in 5.5 × 10−5 g cm−2 of water vapor. These are 27% (1367 nm) and 44% (1870 nm) differences at the lowest measured value of water vapor (1.26 × 10−4 g cm−2) and 7% (1367 nm) and 12% (1870 nm) differences at the highest measured value of water vapor (4.59 × 10−4 g cm−2). A potential method for extending this type of measurement from aircraft flight altitude to the top of the atmosphere (TOA) is discussed.


2016 ◽  
Vol 73 (2) ◽  
pp. 855-868 ◽  
Author(s):  
Joowan Kim ◽  
William J. Randel ◽  
Thomas Birner ◽  
Marta Abalos

Abstract The zonal wavenumber spectrum of atmospheric wave forcing in the lower stratosphere is examined to understand the annual cycle of upwelling at the tropical tropopause. Tropopause upwelling is derived based on the wave forcing computed from ERA-Interim using the momentum and mass conservation equations in the transformed Eulerian-mean framework. The calculated upwelling agrees well with other upwelling estimates and successfully captures the annual cycle, with a maximum during Northern Hemisphere (NH) winter. The spectrum of wave forcing reveals that the zonal wavenumber-3 component drives a large portion of the annual cycle in upwelling. The wave activity flux (Eliassen–Palm flux) shows that the associated waves originate from the NH extratropics and the Southern Hemisphere tropics during December–February, with both regions contributing significant wavenumber-3 fluxes. These wave fluxes are nearly absent during June–August. Wavenumbers 1 and 2 and synoptic-scale waves have a notable contribution to tropopause upwelling but have little influence on the annual cycle, except the wavenumber-4 component. The quasigeostrophic refractive index suggests that the NH extratropical wavenumber-3 component can enhance tropopause upwelling because these planetary-scale waves are largely trapped in the vertical, while being refracted toward the subtropical upper troposphere and lower stratosphere. Regression analysis based on interannual variability suggests that the wavenumber-3 waves are related to tropical convection and wave breaking along the subtropical jet in the NH extratropics.


2009 ◽  
Vol 9 (4) ◽  
pp. 14645-14681
Author(s):  
A. Butz ◽  
H. Bösch ◽  
C. Camy-Peyret ◽  
M. P. Chipperfield ◽  
M. Dorf ◽  
...  

Abstract. We report upper limits of IO and OIO in the tropical upper troposphere and stratosphere inferred from solar occultation spectra recorded by the LPMA/DOAS (Limb Profile Monitor of the Atmosphere/Differential Optical Absorption Spectroscopy) payload during two stratospheric balloon flights from a station in Northern Brazil (5.1° S, 42.9° W). In the tropical upper troposphere and lower stratosphere, upper limits for both, IO and OIO, are below 0.1 ppt. Photochemical modelling is used to estimate the compatible upper limits for the total gaseous inorganic iodine burden (Iy) amounting to 0.09 to 0.16 (+0.10/−0.04) ppt in the tropical lower stratosphere (21.0 km to 16.5 km) and 0.17 to 0.35 (+0.20/−0.08) ppt in the tropical upper troposphere (16.5 km to 13.5 km). In the middle stratosphere, upper limits increase with altitude as sampling sensitivity decreases. Our findings imply that the amount of gaseous iodine transported into the stratosphere through the tropical tropopause layer is small and that iodine-mediated ozone loss plays only a minor role for stratospheric photochemistry. However, photochemical modelling uncertainties are large and iodine might be transported into the stratosphere in particulate form.


2009 ◽  
Vol 9 (18) ◽  
pp. 7229-7242 ◽  
Author(s):  
A. Butz ◽  
H. Bösch ◽  
C. Camy-Peyret ◽  
M. P. Chipperfield ◽  
M. Dorf ◽  
...  

Abstract. We report upper limits of IO and OIO in the tropical upper troposphere and stratosphere inferred from solar occultation spectra recorded by the LPMA/DOAS (Limb Profile Monitor of the Atmosphere/Differential Optical Absorption Spectroscopy) payload during two stratospheric balloon flights from a station in Northern Brazil (5.1° S, 42.9° W). In the tropical upper troposphere and lower stratosphere, upper limits for both, IO and OIO, are below 0.1 ppt. Photochemical modelling is used to estimate the compatible upper limits for the total gaseous inorganic iodine burden (Iy) amounting to 0.09 to 0.16 (+0.10/−0.04) ppt in the tropical lower stratosphere (21.0 km to 16.5 km) and 0.17 to 0.35 (+0.20/−0.08) ppt in the tropical upper troposphere (16.5 km to 13.5 km). In the middle stratosphere, upper limits increase with altitude as sampling sensitivity decreases. Our findings imply that the amount of gaseous iodine transported into the stratosphere through the tropical tropopause layer is small. Thus, iodine-mediated ozone loss plays a minor role for contemporary stratospheric photochemistry but might become significant in the future if source gas emissions or injection efficiency into the upper atmosphere are enhanced. However, photochemical modelling uncertainties are large and iodine might be transported into the stratosphere in particulate form.


2015 ◽  
Vol 15 (1) ◽  
pp. 1041-1091 ◽  
Author(s):  
W. Frey ◽  
R. Schofield ◽  
P. Hoor ◽  
D. Kunkel ◽  
F. Ravegnani ◽  
...  

Abstract. In this study we examine the simulated downward transport and mixing of stratospheric air into the upper tropical troposphere as observed on a research flight during the SCOUT-O3 campaign in connection to a deep convective system. We use the Advanced Research Weather and Research Forecasting (WRF-ARW) model with a horizontal resolution of 333 m to examine this downward transport. The simulation reproduces the deep convective system, its timing and overshooting altitudes reasonably well compared to radar and aircraft observations. Passive tracers initialised at pre-storm times indicate the downward transport of air from the stratosphere to the upper troposphere as well as upward transport from the boundary layer into the cloud anvils and overshooting tops. For example, a passive ozone tracer (i.e. a tracer not undergoing chemical processing) shows an enhancement in the upper troposphere of up to about 30 ppbv locally in the cloud, while the in situ measurements show an increase of 50 ppbv. However, the passive carbon monoxide tracer exhibits an increase, while the observations show a decrease of about 10 ppbv, indicative of an erroneous model representation of the transport processes in the tropical tropopause layer. Furthermore, it could point to insufficient entrainment and detrainment in the model. The simulation shows a general moistening of air in the lower stratosphere but it also exhibits local dehydration features. Here we use the model to explain the processes causing the transport and also expose areas of inconsistencies between the model and observations.


2011 ◽  
Vol 11 (1) ◽  
pp. 163-192 ◽  
Author(s):  
J. P. Vernier ◽  
J. P. Pommereau ◽  
L. W. Thomason ◽  
J. Pelon ◽  
A. Garnier ◽  
...  

Abstract. The evolution of aerosols in the tropical upper troposphere/lower stratosphere between June 2006 and October 2009 is examined using the observations of the space borne CALIOP lidar aboard the CALIPSO satellite. Superimposed on several volcanic plumes and soot from an extreme biomass-burning event in 2009, the measurements reveal the existence of fast cleansing episodes of the lower stratosphere to altitudes as high as 20 km. The cleansing of the full 14–20 km layer takes place within 1–4 months. Its coincidence with the maximum of convective activity in the southern tropics, suggests that the cleansing is the result of a large number of overshooting towers, injecting aerosol-poor tropospheric air into the lower stratosphere. The enhancements of aerosols at the tropopause level during the NH summer may be due to the same transport process but associated with intense sources of aerosols at the surface. Since, the tropospheric air flux derived from CALIOP observations during North Hemisphere winter is 5–20 times larger than the slow ascent by radiative heating usually assumed, the observations suggest that convective overshooting is a major contributor to troposphere-to-stratosphere transport with concommitant implications to the Tropical Tropopause Layer top height, chemistry and thermal structure.


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