Latitudinal distribution of black carbon soot in the upper troposphere and lower stratosphere

1995 ◽  
Vol 100 (D4) ◽  
pp. 7195-7202 ◽  
Author(s):  
David F. Blake ◽  
Katharine Kato
1992 ◽  
Vol 19 (16) ◽  
pp. 1659-1662 ◽  
Author(s):  
R. F. Pusechel ◽  
D. F. Blake ◽  
K. G. Snetsinger ◽  
A. D. A. Hansen ◽  
S. Verma ◽  
...  

2017 ◽  
Vol 2017 ◽  
pp. 1-13 ◽  
Author(s):  
Jiali Luo ◽  
Jiayao Song ◽  
Hongying Tian ◽  
Lei Liu ◽  
Xinlei Liang

We use ERA-Interim reanalysis, MLS observations, and a trajectory model to examine the chemical transport and tracers distribution in the Upper Troposphere and Lower Stratosphere (UTLS) associated with an east-west oscillation case of the anticyclone in 2016. The results show that the spatial distribution of water vapor (H2O) was more consistent with the location of the anticyclone than carbon monoxide (CO) at 100 hPa, and an independent relative high concentration center was only found in H2O field. At 215 hPa, although the anticyclone center also migrated from the Tibetan Mode (TM) to the Iranian Mode (IM), the relative high concentration centers of both tracers were always colocated with regions where upward motion was strong in the UTLS. When the anticyclone migrated from the TM, air within the anticyclone over Tibetan Plateau may transport both westward and eastward but was always within the UTLS. The relative high concentration of tropospheric tracers within the anticyclone in the IM was from the east and transported by the westward propagation of the anticyclone rather than being lifted from surface directly. Air within the relative high geopotential height centers over Western Pacific was partly from the main anticyclone and partly from lower levels.


1997 ◽  
Vol 28 ◽  
pp. S65-S66 ◽  
Author(s):  
F. Arnold ◽  
K.H. Wohlfrom ◽  
J. Schneider ◽  
M. Klemm ◽  
T. Stilp ◽  
...  

2015 ◽  
Vol 15 (13) ◽  
pp. 7667-7684 ◽  
Author(s):  
Fuqing Zhang ◽  
Junhong Wei ◽  
Meng Zhang ◽  
K. P. Bowman ◽  
L. L. Pan ◽  
...  

Abstract. This study analyzes in situ airborne measurements from the 2008 Stratosphere–Troposphere Analyses of Regional Transport (START08) experiment to characterize gravity waves in the extratropical upper troposphere and lower stratosphere (ExUTLS). The focus is on the second research flight (RF02), which took place on 21–22 April 2008. This was the first airborne mission dedicated to probing gravity waves associated with strong upper-tropospheric jet–front systems. Based on spectral and wavelet analyses of the in situ observations, along with a diagnosis of the polarization relationships, clear signals of mesoscale variations with wavelengths ~ 50–500 km are found in almost every segment of the 8 h flight, which took place mostly in the lower stratosphere. The aircraft sampled a wide range of background conditions including the region near the jet core, the jet exit and over the Rocky Mountains with clear evidence of vertically propagating gravity waves of along-track wavelength between 100 and 120 km. The power spectra of the horizontal velocity components and potential temperature for the scale approximately between ~ 8 and ~ 256 km display an approximate −5/3 power law in agreement with past studies on aircraft measurements, while the fluctuations roll over to a −3 power law for the scale approximately between ~ 0.5 and ~ 8 km (except when this part of the spectrum is activated, as recorded clearly by one of the flight segments). However, at least part of the high-frequency signals with sampled periods of ~ 20–~ 60 s and wavelengths of ~ 5–~ 15 km might be due to intrinsic observational errors in the aircraft measurements, even though the possibilities that these fluctuations may be due to other physical phenomena (e.g., nonlinear dynamics, shear instability and/or turbulence) cannot be completely ruled out.


2016 ◽  
Author(s):  
M. Venkat Ratnam ◽  
S. Ravindra Babu ◽  
S. S. Das ◽  
Ghouse Basha ◽  
B. V. Krishnamurthy ◽  
...  

Abstract. Tropical cyclones play an important role in modifying the tropopause structure and dynamics as well as stratosphere-troposphere exchange (STE) process in the Upper Troposphere and Lower Stratosphere (UTLS) region. In the present study, the impact of cyclones that occurred over the North Indian Ocean during 2007–2013 on the STE process is quantified using satellite observations. Tropopause characteristics during cyclones are obtained from the Global Positioning System (GPS) Radio Occultation (RO) measurements and ozone and water vapor concentrations in UTLS region are obtained from Aura-Microwave Limb Sounder (MLS) satellite observations. The effect of cyclones on the tropopause parameters is observed to be more prominent within 500 km from the centre of cyclone. In our earlier study we have observed decrease (increase) in the tropopause altitude (temperature) up to 0.6 km (3 K) and the convective outflow level increased up to 2 km. This change leads to a total increase in the tropical tropopause layer (TTL) thickness of 3 km within the 500 km from the centre of cyclone. Interestingly, an enhancement in the ozone mixing ratio in the upper troposphere is clearly noticed within 500 km from cyclone centre whereas the enhancement in the water vapor in the lower stratosphere is more significant on south-east side extending from 500–1000 km away from the cyclone centre. We estimated the cross-tropopause mass flux for different intensities of cyclones and found that the mean flux from stratosphere to troposphere for cyclonic stroms is 0.05 ± 0.29 × 10−3 kg m−2 and for very severe cyclonic stroms it is 0.5 ± 1.07 × 10−3 kg m−2. More downward flux is noticed in the north-west and south-west side of the cyclone centre. These results indicate that the cyclones have significant impact in effecting the tropopause structure, ozone and water vapour budget and consequentially the STE in the UTLS region.


2013 ◽  
Vol 13 (5) ◽  
pp. 2423-2434 ◽  
Author(s):  
B. H. Samset ◽  
G. Myhre ◽  
M. Schulz ◽  
Y. Balkanski ◽  
S. Bauer ◽  
...  

Abstract. The impact of black carbon (BC) aerosols on the global radiation balance is not well constrained. Here twelve global aerosol models are used to show that at least 20% of the present uncertainty in modeled BC direct radiative forcing (RF) is due to diversity in the simulated vertical profile of BC mass. Results are from phases 1 and 2 of the global aerosol model intercomparison project (AeroCom). Additionally, a significant fraction of the variability is shown to come from high altitudes, as, globally, more than 40% of the total BC RF is exerted above 5 km. BC emission regions and areas with transported BC are found to have differing characteristics. These insights into the importance of the vertical profile of BC lead us to suggest that observational studies are needed to better characterize the global distribution of BC, including in the upper troposphere.


2009 ◽  
Vol 66 (12) ◽  
pp. 3678-3694 ◽  
Author(s):  
Francesco d’Ovidio ◽  
Emily Shuckburgh ◽  
Bernard Legras

Abstract A new diagnostic (the “Lyapunov diffusivity”) is presented that has the ability to quantify isentropic mixing in diffusion units and detects local mixing events by describing latitude–longitude variability. It is a hybrid diagnostic, combining the tracer-based effective diffusivity with the particle-based Lyapunov exponent calculation. Isentropic mixing on the 350-K surface shows that there is significant longitudinal variation to the strength of mixing at the northern subtropical jet, with a strong mixing barrier over Asia and the western Pacific, a weaker mixing barrier over the western Atlantic, and active mixing regions at the jet exits over the eastern Pacific and Atlantic.


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