scholarly journals Interactive chemistry in the Laboratoire de Météorologie Dynamique general circulation model: Description and background tropospheric chemistry evaluation

2004 ◽  
Vol 109 (D4) ◽  
pp. n/a-n/a ◽  
Author(s):  
D. A. Hauglustaine ◽  
F. Hourdin ◽  
L. Jourdain ◽  
M.-A. Filiberti ◽  
S. Walters ◽  
...  
2009 ◽  
Vol 137 (3) ◽  
pp. 1061-1082 ◽  
Author(s):  
Celal S. Konor ◽  
Gabriel Cazes Boezio ◽  
Carlos R. Mechoso ◽  
Akio Arakawa

Abstract This paper presents the basic features of a newly developed planetary boundary layer (PBL) parameterization, and the performance assessment of a version of the University of California, Los Angeles (UCLA), Atmospheric General Circulation Model (AGCM) to which the parameterization is incorporated. The UCLA AGCM traditionally uses a framework in which a sigma-type vertical coordinate for the PBL shares a coordinate surface with the free atmosphere at the PBL top. This framework facilitates an explicit representation of processes concentrated near the PBL top, which is crucially important especially for predicting PBL clouds. In the new framework, multiple layers are introduced between the PBL top and earth’s surface, allowing for predictions of the vertical profiles of potential temperature, total water mixing ratio, and horizontal winds within the PBL. The vertically integrated “bulk” turbulent kinetic energy (TKE) is also predicted for the PBL. The PBL-top mass entrainment is determined through an equation including the effects of TKE and the radiative and evaporative cooling processes concentrated near the PBL top. The surface fluxes are determined from an aerodynamic formula in which the velocity scale depends both on the square root of TKE and the grid-scale PBL velocity at the lowermost model layer. The turbulent fluxes within the PBL are determined through an approach that includes the effects of both large convective and small diffusive eddies. AGCM simulations with the new formulation of PBL are analyzed with a focus on the seasonal and diurnal variations. The simulated seasonal cycle of stratocumulus over the eastern oceans is realistic, as are the diurnal cycles of the PBL depth and precipitation over land. The simulated fluxes of latent heat, momentum, and shortwave radiation at the ocean surface and baroclinic activity in the middle latitudes show significant improvements over the previous versions of the AGCM based on the single-layer PBL.


2020 ◽  
Vol 13 (9) ◽  
pp. 3817-3838
Author(s):  
Xiao Lu ◽  
Lin Zhang ◽  
Tongwen Wu ◽  
Michael S. Long ◽  
Jun Wang ◽  
...  

Abstract. Chemistry plays an indispensable role in investigations of the atmosphere; however, many climate models either ignore or greatly simplify atmospheric chemistry, limiting both their accuracy and their scope. We present the development and evaluation of the online global atmospheric chemical model BCC-GEOS-Chem v1.0, coupling the GEOS-Chem chemical transport model (CTM) as an atmospheric chemistry component in the Beijing Climate Center atmospheric general circulation model (BCC-AGCM). The GEOS-Chem atmospheric chemistry component includes detailed tropospheric HOx–NOx–volatile organic compounds–ozone–bromine–aerosol chemistry and online dry and wet deposition schemes. We then demonstrate the new capabilities of BCC-GEOS-Chem v1.0 relative to the base BCC-AGCM model through a 3-year (2012–2014) simulation with anthropogenic emissions from the Community Emissions Data System (CEDS) used in the Coupled Model Intercomparison Project Phase 6 (CMIP6). The model captures well the spatial distributions and seasonal variations in tropospheric ozone, with seasonal mean biases of 0.4–2.2 ppbv at 700–400 hPa compared to satellite observations and within 10 ppbv at the surface to 500 hPa compared to global ozonesonde observations. The model has larger high-ozone biases over the tropics which we attribute to an overestimate of ozone chemical production. It underestimates ozone in the upper troposphere which is likely due either to the use of a simplified stratospheric ozone scheme or to biases in estimated stratosphere–troposphere exchange dynamics. The model diagnoses the global tropospheric ozone burden, OH concentration, and methane chemical lifetime to be 336 Tg, 1.16×106 molecule cm−3, and 8.3 years, respectively, which is consistent with recent multimodel assessments. The spatiotemporal distributions of NO2, CO, SO2, CH2O, and aerosol optical depth are generally in agreement with satellite observations. The development of BCC-GEOS-Chem v1.0 represents an important step for the development of fully coupled earth system models (ESMs) in China.


2006 ◽  
Vol 6 (4) ◽  
pp. 6957-7050 ◽  
Author(s):  
P. Jöckel ◽  
H. Tost ◽  
A. Pozzer ◽  
C. Brühl ◽  
J. Buchholz ◽  
...  

Abstract. The new Modular Earth Submodel System (MESSy) describes atmospheric chemistry and meteorological processes in a modular framework, following strict coding standards. It has been coupled to the ECHAM5 general circulation model, which has been slightly modified for this purpose. A 90-layer model version up to 0.01 hPa was used at T42 resolution (~2.8 latitude and longitude) to simulate the lower and middle atmosphere. The model meteorology has been tested to check the influence of the changes to ECHAM5 and the radiation interactions with the new representation of atmospheric composition. A Newtonian relaxation technique was applied in the tropospheric part of the domain to weakly nudge the model towards the analysed meteorology during the period 1998–2005. It is shown that the tropospheric wave forcing of the stratosphere in the model suffices to reproduce the Quasi-Biennial Oscillation and major stratospheric warming events leading e.g. to the vortex split over Antarctica in 2002. Characteristic features such as dehydration and denitrification caused by the sedimentation of polar stratospheric cloud particles and ozone depletion during winter and spring are simulated accurately, although ozone loss in the lower polar stratosphere is slightly underestimated. The model realistically simulates stratosphere-troposphere exchange processes as indicated by comparisons with satellite and in situ measurements. The evaluation of tropospheric chemistry presented here focuses on the distributions of ozone, hydroxyl radicals, carbon monoxide and reactive nitrogen compounds. In spite of minor shortcomings, mostly related to the relatively coarse T42 resolution and the neglect of interannual changes in biomass burning emissions, the main characteristics of the trace gas distributions are generally reproduced well. The MESSy submodels and the ECHAM5/MESSy1 model output are available through the internet on request.


2006 ◽  
Vol 6 (12) ◽  
pp. 5067-5104 ◽  
Author(s):  
P. Jöckel ◽  
H. Tost ◽  
A. Pozzer ◽  
C. Brühl ◽  
J. Buchholz ◽  
...  

Abstract. The new Modular Earth Submodel System (MESSy) describes atmospheric chemistry and meteorological processes in a modular framework, following strict coding standards. It has been coupled to the ECHAM5 general circulation model, which has been slightly modified for this purpose. A 90-layer model setup up to 0.01 hPa was used at spectral T42 resolution to simulate the lower and middle atmosphere. With the high vertical resolution the model simulates the Quasi-Biennial Oscillation. The model meteorology has been tested to check the influence of the changes to ECHAM5 and the radiation interactions with the new representation of atmospheric composition. In the simulations presented here a Newtonian relaxation technique was applied in the tropospheric part of the domain to weakly nudge the model towards the analysed meteorology during the period 1998–2005. This allows an efficient and direct evaluation with satellite and in-situ data. It is shown that the tropospheric wave forcing of the stratosphere in the model suffices to reproduce major stratospheric warming events leading e.g. to the vortex split over Antarctica in 2002. Characteristic features such as dehydration and denitrification caused by the sedimentation of polar stratospheric cloud particles and ozone depletion during winter and spring are simulated well, although ozone loss in the lower polar stratosphere is slightly underestimated. The model realistically simulates stratosphere-troposphere exchange processes as indicated by comparisons with satellite and in situ measurements. The evaluation of tropospheric chemistry presented here focuses on the distributions of ozone, hydroxyl radicals, carbon monoxide and reactive nitrogen compounds. In spite of minor shortcomings, mostly related to the relatively coarse T42 resolution and the neglect of inter-annual changes in biomass burning emissions, the main characteristics of the trace gas distributions are generally reproduced well. The MESSy submodels and the ECHAM5/MESSy1 model output are available through the internet on request.


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