scholarly journals Chemistry-climate interactions in the Goddard Institute for Space Studies general circulation model: 1. Tropospheric chemistry model description and evaluation

2001 ◽  
Vol 106 (D8) ◽  
pp. 8047-8075 ◽  
Author(s):  
Drew T. Shindell ◽  
J. Lee Grenfell ◽  
David Rind ◽  
Volker Grewe ◽  
Colin Price
Keyword(s):  
General Circulation Model ◽  
General Circulation ◽  
Circulation Model ◽  
Tropospheric Chemistry ◽  
Model Description ◽  
Climate Interactions ◽  
Goddard Institute

scholarly journals Preindustrial-to-present-day radiative forcing by tropospheric ozone from improved simulations with the GISS chemistry-climate GCM

2003 ◽  
Vol 3 (5) ◽  
pp. 1675-1702 ◽  
Author(s):  
D. T. Shindell ◽  
G. Faluvegi ◽  
N. Bell
Keyword(s):  
Tropospheric Ozone ◽  
Radiative Forcing ◽  
General Circulation ◽  
Climate Model ◽  
Circulation Model ◽  
Tropospheric Chemistry ◽  
True Value ◽  
Tropopause Region ◽  
Dynamics Simulations ◽  
Goddard Institute

Abstract. Improved estimates of the radiative forcing from tropospheric ozone increases since the preindustrial have been calculated with the tropospheric chemistry model used at the Goddard Institute for Space Studies (GISS) within the GISS general circulation model (GCM). The chemistry in this model has been expanded to include simplified representations of peroxyacetylnitrates and non-methane hydrocarbons in addition to background NOx-HOx-Ox-CO-CH4 chemistry. The GCM has improved resolution and physics in the boundary layer, improved resolution near the tropopause, and now contains a full representation of stratospheric dynamics. Simulations of present-day conditions show that this coupled chemistry-climate model is better able to reproduce observed tropospheric ozone, especially in the tropopause region, which is critical to climate forcing. Comparison with preindustrial simulations gives a global annual average radiative forcing due to tropospheric ozone increases of 0.30 W/m2 with standard assumptions for preindustrial emissions. Locally, the forcing reaches more than 0.8 W/m2 in parts of the northern subtropics during spring and summer, and is more than 0.6 W/m2 through nearly all the Northern subtropics and mid-latitudes during summer. An alternative preindustrial simulation with soil NOx emissions reduced by two-thirds and emissions of isoprene, paraffins and alkenes from vegetation increased by 50% gives a forcing of 0.33 W/m2. Given the large uncertainties in preindustrial ozone amounts, the true value may lie well outside this range.

Parameterization of PBL Processes in an Atmospheric General Circulation Model: Description and Preliminary Assessment

2009 ◽  
Vol 137 (3) ◽  
pp. 1061-1082 ◽  
Author(s):  
Celal S. Konor ◽  
Gabriel Cazes Boezio ◽  
Carlos R. Mechoso ◽  
Akio Arakawa
Keyword(s):  
General Circulation Model ◽  
General Circulation ◽  
Atmospheric General Circulation Model ◽  
Potential Temperature ◽  
Circulation Model ◽  
Surface Fluxes ◽  
Shortwave Radiation ◽  
Model Description ◽  
Atmospheric General Circulation ◽  
Seasonal And Diurnal Variations

Abstract This paper presents the basic features of a newly developed planetary boundary layer (PBL) parameterization, and the performance assessment of a version of the University of California, Los Angeles (UCLA), Atmospheric General Circulation Model (AGCM) to which the parameterization is incorporated. The UCLA AGCM traditionally uses a framework in which a sigma-type vertical coordinate for the PBL shares a coordinate surface with the free atmosphere at the PBL top. This framework facilitates an explicit representation of processes concentrated near the PBL top, which is crucially important especially for predicting PBL clouds. In the new framework, multiple layers are introduced between the PBL top and earth’s surface, allowing for predictions of the vertical profiles of potential temperature, total water mixing ratio, and horizontal winds within the PBL. The vertically integrated “bulk” turbulent kinetic energy (TKE) is also predicted for the PBL. The PBL-top mass entrainment is determined through an equation including the effects of TKE and the radiative and evaporative cooling processes concentrated near the PBL top. The surface fluxes are determined from an aerodynamic formula in which the velocity scale depends both on the square root of TKE and the grid-scale PBL velocity at the lowermost model layer. The turbulent fluxes within the PBL are determined through an approach that includes the effects of both large convective and small diffusive eddies. AGCM simulations with the new formulation of PBL are analyzed with a focus on the seasonal and diurnal variations. The simulated seasonal cycle of stratocumulus over the eastern oceans is realistic, as are the diurnal cycles of the PBL depth and precipitation over land. The simulated fluxes of latent heat, momentum, and shortwave radiation at the ocean surface and baroclinic activity in the middle latitudes show significant improvements over the previous versions of the AGCM based on the single-layer PBL.

scholarly journals Development of the global atmospheric chemistry general circulation model BCC-GEOS-Chem v1.0: model description and evaluation

2020 ◽  
Vol 13 (9) ◽  
pp. 3817-3838
Author(s):  
Xiao Lu ◽  
Lin Zhang ◽  
Tongwen Wu ◽  
Michael S. Long ◽  
Jun Wang ◽  
...  
Keyword(s):  
General Circulation Model ◽  
Atmospheric Chemistry ◽  
Tropospheric Ozone ◽  
General Circulation ◽  
Climate Models ◽  
Transport Model ◽  
Stratospheric Ozone ◽  
Circulation Model ◽  
Satellite Observations ◽  
Model Description

Abstract. Chemistry plays an indispensable role in investigations of the atmosphere; however, many climate models either ignore or greatly simplify atmospheric chemistry, limiting both their accuracy and their scope. We present the development and evaluation of the online global atmospheric chemical model BCC-GEOS-Chem v1.0, coupling the GEOS-Chem chemical transport model (CTM) as an atmospheric chemistry component in the Beijing Climate Center atmospheric general circulation model (BCC-AGCM). The GEOS-Chem atmospheric chemistry component includes detailed tropospheric HOx–NOx–volatile organic compounds–ozone–bromine–aerosol chemistry and online dry and wet deposition schemes. We then demonstrate the new capabilities of BCC-GEOS-Chem v1.0 relative to the base BCC-AGCM model through a 3-year (2012–2014) simulation with anthropogenic emissions from the Community Emissions Data System (CEDS) used in the Coupled Model Intercomparison Project Phase 6 (CMIP6). The model captures well the spatial distributions and seasonal variations in tropospheric ozone, with seasonal mean biases of 0.4–2.2 ppbv at 700–400 hPa compared to satellite observations and within 10 ppbv at the surface to 500 hPa compared to global ozonesonde observations. The model has larger high-ozone biases over the tropics which we attribute to an overestimate of ozone chemical production. It underestimates ozone in the upper troposphere which is likely due either to the use of a simplified stratospheric ozone scheme or to biases in estimated stratosphere–troposphere exchange dynamics. The model diagnoses the global tropospheric ozone burden, OH concentration, and methane chemical lifetime to be 336 Tg, 1.16×106 molecule cm−3, and 8.3 years, respectively, which is consistent with recent multimodel assessments. The spatiotemporal distributions of NO2, CO, SO2, CH2O, and aerosol optical depth are generally in agreement with satellite observations. The development of BCC-GEOS-Chem v1.0 represents an important step for the development of fully coupled earth system models (ESMs) in China.

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