Quantifying the rate of heterogeneous processing in the Arctic polar vortex with in situ observations of OH

2002 ◽  
Vol 107 (D20) ◽  
Author(s):  
T. F. Hanisco
Keyword(s):  
Polar Vortex ◽  
The Arctic ◽  
Heterogeneous Processing ◽  
In Situ Observations

scholarly journals International Arctic Systems for Observing the Atmosphere: An International Polar Year Legacy Consortium

2016 ◽  
Vol 97 (6) ◽  
pp. 1033-1056 ◽  
Author(s):  
Taneil Uttal ◽  
Sandra Starkweather ◽  
James R. Drummond ◽  
Timo Vihma ◽  
Alexander P. Makshtas ◽  
...  
Keyword(s):  
United States ◽  
The United States ◽  
Satellite Observations ◽  
The Arctic ◽  
International Polar Year ◽  
Network Measurements ◽  
International Polar ◽  
In Situ Observations ◽  
Arctic Atmosphere

Abstract International Arctic Systems for Observing the Atmosphere (IASOA) activities and partnerships were initiated as a part of the 2007–09 International Polar Year (IPY) and are expected to continue for many decades as a legacy program. The IASOA focus is on coordinating intensive measurements of the Arctic atmosphere collected in the United States, Canada, Russia, Norway, Finland, and Greenland to create synthesis science that leads to an understanding of why and not just how the Arctic atmosphere is evolving. The IASOA premise is that there are limitations with Arctic modeling and satellite observations that can only be addressed with boots-on-the-ground, in situ observations and that the potential of combining individual station and network measurements into an integrated observing system is tremendous. The IASOA vision is that by further integrating with other network observing programs focusing on hydrology, glaciology, oceanography, terrestrial, and biological systems it will be possible to understand the mechanisms of the entire Arctic system, perhaps well enough for humans to mitigate undesirable variations and adapt to inevitable change.

The prevalence of meteoric-sulphuric particles within the stratospheric aerosol layer

2021 ◽  
Author(s):  
Graham Mann ◽  
James Brooke ◽  
Kamalika Sengupta ◽  
Lauren Marshall ◽  
Sandip Dhomse ◽  
...  
Keyword(s):  
High Latitude ◽  
Climate Model ◽  
Polar Vortex ◽  
Stratospheric Aerosol ◽  
Light Extinction ◽  
The Arctic ◽  
Aerosol Layer ◽  
Aerosol Composition ◽  
Particle Layer

<p>The widespread presence of meteoric smoke particles (MSPs) within a distinct class of stratospheric aerosol particles has become clear from in-situ measurements in the Arctic, Antarctic and at mid-latitudes.<br> <br>We apply an adapted version of the interactive stratosphere aerosol configuration of the composition-climate model UM-UKCA, to predict the global distribution of meteoric-sulphuric particles nucleated heterogeneously on MSP cores. We compare the UM-UKCA results to new MSP-sulphuric simulations with the European stratosphere-troposphere chemistry-aerosol modelling system IFS-CB05-BASCOE-GLOMAP.</p><p><br>The simulations show a strong seasonal cycle in meteoric-sulphuric particle abundance results from the winter-time source of MSPs transported down into the stratosphere in the polar vortex. Coagulation during downward transport sees high latitude MSP concentrations reduce from ~500 per cm3 at 40km to ~20 per cm3 at 25km, the uppermost extent of the stratospheric aerosol particle layer (the Junge layer).<br> <br>Once within the Junge layer's supersaturated environment, meteoric-sulphuric particles form readily on the MSP cores, growing to 50-70nm dry-diameter (Dp) at 20-25km. Further inter-particle coagulation between these non-volatile particles reduces their number to 1-5 per cc at 15-20km, particle sizes there larger, at Dp ~100nm.</p><p><br>The model predicts meteoric-sulphurics in high-latitude winter comprise >90% of Dp>10nm particles above 25km, reducing to ~40% at 20km, and ~10% at 15km.<br> <br>These non-volatile particle fractions are slightly less than measured from high-altitude aircraft in the lowermost Arctic stratosphere (Curtius et al., 2005; Weigel et al., 2014), and consistent with mid-latitude aircraft measurements of lower stratospheric aerosol composition (Murphy et al., 1998), total particle concentrations  also matching in-situ balloon measurements from Wyoming (Campbell and Deshler, 2014).<br> <br>The MSP-sulphuric interactions also improve agreement with SAGE-II observed stratospheric aerosol extinction in the quiescent 1998-2002 period. <br> <br>Simulations with a factor-8-elevated MSP input form more Dp>10nm meteoric-sulphurics, but the increased number sees fewer growing to Dp ~100nm, the increased MSPs reducing the stratospheric aerosol layer’s light extinction.</p>

scholarly journals Evidence for long-lived polar vortex air in the mid-latitude summer stratosphere from in situ laser diode CH<sub>4</sub> and H<sub>2</sub>O measurements

2005 ◽  
Vol 5 (6) ◽  
pp. 1467-1472 ◽  
Author(s):  
G. Durry ◽  
A. Hauchecorne
Keyword(s):  
High Resolution ◽  
Laser Diode ◽  
Polar Vortex ◽  
The Arctic ◽  
Concentration Profiles ◽  
Spatial Structures ◽  
Laser Spectrometer ◽  
Southern France ◽  
Diode Laser Spectrometer

Abstract. A balloon borne diode laser spectrometer was launched in southern France in June 2000 to yield in situ stratospheric CH4 and H2O measurements. In the altitude region ranging from 20km to 25km, striking large spatial structures were observed in the vertical concentration profiles of both species. We suggest these patterns are due to the presence of long-lived remnants of the wintertime polar vortex in the mid-latitude summer stratosphere. To support this interpretation, a high resolution advection model for potential vorticity is used to investigate the evolution of the Arctic vortex after its breakdown phase in spring 2000.

scholarly journals Investigation of Arctic middle-atmospheric dynamics using 3 years of H<sub>2</sub>O and O<sub>3</sub> measurements from microwave radiometers at Ny-Ålesund

2019 ◽  
Author(s):  
Franziska Schranz ◽  
Brigitte Tschanz ◽  
Rolf Rüfenacht ◽  
Klemens Hocke ◽  
Mathias Palm ◽  
...  
Keyword(s):  
Water Vapour ◽  
Middle Atmosphere ◽  
Microwave Radiometer ◽  
Polar Vortex ◽  
The Arctic ◽  
High Time Resolution ◽  
Middle Atmospheric Dynamics ◽  
Wind Profiles ◽  
Microwave Radiometers

Abstract. We use 3 years of water vapour and ozone measurements to analyse dynamical events in the polar middle atmosphere such as sudden stratospheric warmings (SSW), polar vortex shifts, water vapour descent rates and periodicities. The measurements were performed with the two ground-based microwave radiometers MIAWARA-C and GROMOS-C which are co-located at the AWIPEV research base at Ny-Ålesund, Svalbard (79° N, 12° E) since September 2015. The almost continuous datasets of water vapour and ozone are characterised by a high time resolution in the order of hours. A thorough intercomparison of these datasets with models and measurements from satellite, ground-based and in-situ instruments was performed. In the upper stratosphere and lower mesosphere the MIAWARA-C profiles agree within 5 % with SD-WACCM simulations and ACE-FTS measurements whereas AuraMLS measurements show an average offset of 10–15 % depending on altitude but constant in time. Stratospheric GROMOS-C profiles are within 5 % of the satellite instruments AuraMLS and ACE-FTS and the ground-based microwave radiometer OZORAM which is also located at Ny-Ålesund. During these first three years of the measurement campaign typical phenomena of the Arctic middle atmosphere took place and we analysed their signatures in the water vapour and ozone datasets. Inside of the polar vortex in autumn we found the descent rate of mesospheric water vapour to be 435 m/day on average. In early 2017 distinct increases in mesospheric water vapour of about 2 ppm were observed when the polar vortex was displaced and midlatitude air was brought to Ny-Ålesund. Two major sudden stratospheric warmings took place in March 2016 and February 2018 where ozone enhancements of up to 4 ppm were observed. The zonal wind reversals accompanying a major SSW were captured in the GROMOS-C wind profiles which are retrieved from the ozone spectra. After the SSW in February 2018 the polar vortex re-established and the water vapour descent rate in the mesosphere was 355 m/day. In the water vapour and ozone time series signatures of atmospheric waves with periods close to 2, 5, 10 and 16 days were found.

scholarly journals Integrative and comprehensive Understanding on Polar Environments (iCUPE): the concept and initial results

2020 ◽  
Author(s):  
Tuukka Petäjä ◽  
Ella-Maria Duplissy ◽  
Ksenia Tabakova ◽  
Julia Schmale ◽  
Barbara Altstädter ◽  
...  
Keyword(s):  
Remote Sensing ◽  
Natural Resources ◽  
Satellite Remote Sensing ◽  
Integrated Approach ◽  
The Arctic ◽  
Polar Regions ◽  
Comprehensive Understanding ◽  
In Situ Observations ◽  
Initial Results

Abstract. The role of polar regions increases in terms of megatrends such as globalization, new transport routes, demography and use of natural resources consequent effects of regional and transported pollutant concentrations. We set up the ERA-PLANET Strand 4 project iCUPE – integrative and Comprehensive Understanding on Polar Environments to provide novel insights and observational data on global grand challenges with an Arctic focus. We utilize an integrated approach combining in situ observations, satellite remote sensing Earth Observations (EO) and multi-scale modeling to synthesize data from comprehensive long-term measurements, intensive campaigns and satellites to deliver data products, metrics and indicators to the stakeholders concerning the environmental status, availability and extraction of natural resources in the polar areas. The iCUPE work consists of thematic state-of-the-art research and provision of novel data in atmospheric pollution, local sources and transboundary transport, characterization of arctic surfaces and their changes, assessment of concentrations and impacts of heavy metals and persistent organic pollutants and their cycling, quantification of emissions from natural resource extraction and validation and optimization of satellite Earth Observation (EO) data streams. In this paper we introduce the iCUPE project and summarize initial results arising out of integration of comprehensive in situ observations, satellite remote sensing and multiscale modeling in the Arctic context.

scholarly journals Middle atmospheric water vapour and dynamics in the vicinity of the polar vortex during the Hygrosonde-2 campaign

2009 ◽  
Vol 9 (13) ◽  
pp. 4407-4417 ◽  
Author(s):  
S. Lossow ◽  
M. Khaplanov ◽  
J. Gumbel ◽  
J. Stegman ◽  
G. Witt ◽  
...  
Keyword(s):  
Water Vapour ◽  
Middle Atmosphere ◽  
Polar Vortex ◽  
The Arctic ◽  
Small Scale ◽  
Air Masses ◽  
Mixing Ratios ◽  
Water Vapour Concentration ◽  
Wind Shears

Abstract. The Hygrosonde-2 campaign took place on 16 December 2001 at Esrange/Sweden (68° N, 21° E) with the aim to investigate the small scale distribution of water vapour in the middle atmosphere in the vicinity of the Arctic polar vortex. In situ balloon and rocket-borne measurements of water vapour were performed by means of OH fluorescence hygrometry. The combined measurements yielded a high resolution water vapour profile up to an altitude of 75 km. Using the characteristic of water vapour being a dynamical tracer it was possible to directly relate the water vapour data to the location of the polar vortex edge, which separates air masses of different character inside and outside the polar vortex. The measurements probed extra-vortex air in the altitude range between 45 km and 60 km and vortex air elsewhere. Transitions between vortex and extra-vortex usually coincided with wind shears caused by gravity waves which advect air masses with different water vapour volume mixing ratios. From the combination of the results from the Hygrosonde-2 campaign and the first flight of the optical hygrometer in 1994 (Hygrosonde-1) a clear picture of the characteristic water vapour distribution inside and outside the polar vortex can be drawn. Systematic differences in the water vapour concentration between the inside and outside of the polar vortex can be observed all the way up into the mesosphere. It is also evident that in situ measurements with high spatial resolution are needed to fully account for the small-scale exchange processes in the polar winter middle atmosphere.

scholarly journals The Energy Budget of the Polar Atmosphere in MERRA

2012 ◽  
Vol 25 (1) ◽  
pp. 5-24 ◽  
Author(s):  
Richard I. Cullather ◽  
Michael G. Bosilovich
Keyword(s):  
Energy Budget ◽  
The Arctic ◽  
Polar Regions ◽  
Polar Cap ◽  
The South ◽  
Atmospheric Energy ◽  
In Situ Observations ◽  
Energy Convergence ◽  
South Polar

Abstract Components of the atmospheric energy budget from the Modern-Era Retrospective Analysis for Research and Applications (MERRA) are evaluated in polar regions for the period 1979–2005 and compared with previous estimates, in situ observations, and contemporary reanalyses. Closure of the budget is reflected by the analysis increments term, which indicates an energy surplus of 11 W m−2 over the North Polar cap (70°–90°N) and 22 W m−2 over the South Polar cap (70°–90°S). Total atmospheric energy convergence from MERRA compares favorably with previous studies for northern high latitudes but exceeds the available previous estimate for the South Polar cap by 46%. Discrepancies with the Southern Hemisphere energy transport are largest in autumn and may be related to differences in topography with earlier reanalyses. For the Arctic, differences between MERRA and other sources in top of atmosphere (TOA) and surface radiative fluxes are largest in May. These differences are concurrent with the largest discrepancies between MERRA parameterized and observed surface albedo. For May, in situ observations of the upwelling shortwave flux in the Arctic are 80 W m−2 larger than MERRA, while the MERRA downwelling longwave flux is underestimated by 12 W m−2 throughout the year. Over grounded ice sheets, the annual mean net surface energy flux in MERRA is erroneously nonzero. Contemporary reanalyses from the Climate Forecast Center (CFSR) and the Interim Re-Analyses of the European Centre for Medium-Range Weather Forecasts (ERA-I) are found to have better surface parameterizations; however, these reanalyses also disagree with observed surface and TOA energy fluxes. Discrepancies among available reanalyses underscore the challenge of reproducing credible estimates of the atmospheric energy budget in polar regions.

scholarly journals Validation of first chemistry mode retrieval results from new limb-<i>imaging</i> FTS GLORIA with correlative MIPAS-STR observations

2014 ◽  
Vol 7 (12) ◽  
pp. 12691-12717 ◽  
Author(s):  
W. Woiwode ◽  
O. Suminska-Ebersoldt ◽  
H. Oelhaf ◽  
M. Höpfner ◽  
G. V. Belyaev ◽  
...  
Keyword(s):  
Polar Vortex ◽  
Ongoing Work ◽  
First Results ◽  
Research Aircraft ◽  
Order Of Magnitude ◽  
In Situ Observations ◽  
Field Deployment ◽  
Cross Track ◽  
Stratospheric Clouds

Abstract. We report first chemistry mode retrieval results from the new airborne limb-imaging infrared FTS (Fourier transform spectrometer) GLORIA and comparisons with observations by the conventional airborne limb-scanning infrared FTS MIPAS-STR. For GLORIA, the flights aboard the high-altitude research aircraft M55 Geophysica during the ESSenCe campaign (ESa Sounder Campaign 2011) were the very first in field deployment after several years of development. The simultaneous observations of GLORIA and MIPAS-STR during the flight on 16 December 2011 inside the polar vortex and under the conditions of optically partially transparent polar stratospheric clouds (PSCs) provided us the unique opportunity to compare the observations by two different infrared FTS generations directly. The retrieval results of temperature, HNO3, O3, H2O, CFC-11 and CFC-12 show reasonable agreement of GLORIA with MIPAS-STR and collocated in-situ observations. For the horizontally binned hyperspectral limb-images, the GLORIA sampling outnumbered the horizontal cross-track sampling of MIPAS-STR by up to one order of magnitude. Depending on the target parameter, typical vertical resolutions of 0.5 to 2.0 km were obtained for GLORIA and are typically by factors of 2 to 4 better compared to MIPAS-STR. While the improvement of the performance, characterisation and data processing of GLORIA are subject of ongoing work, the presented first results already demonstrate the considerable gain in sampling and vertical resolution achieved with GLORIA.

Gelatinous zooplankton of the Arctic Ocean: in situ observations under the ice

Polar Biology ◽  
2004 ◽  
Vol 28 (3) ◽  
pp. 207-217 ◽  
Author(s):  
K. A. Raskoff ◽  
J. E. Purcell ◽  
R. R. Hopcroft
Keyword(s):  
Arctic Ocean ◽  
Gelatinous Zooplankton ◽  
The Arctic ◽  
The Arctic Ocean ◽  
In Situ Observations
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