scholarly journals Radiative effects of absorbing aerosols and the impact of water vapor

2000 ◽  
Vol 105 (D10) ◽  
pp. 12221-12234 ◽  
Author(s):  
Merlinde J. Kay ◽  
Michael Box
2019 ◽  
Author(s):  
Lucia T. Deaconu ◽  
Nicolas Ferlay ◽  
Fabien Waquet ◽  
Fanny Peers ◽  
François Thieuleux ◽  
...  

Abstract. Aerosols have a direct effect on the Earth's radiative budget and can also affect the cloud development and lifetime. The aerosols above clouds (AAC) are particularly associated with high uncertainties in global climate models. Therefore, it is prerequisite to improve the description and understanding of these situations. During the austral winter, large loadings of biomass burning aerosols originating from fires in the southern African subcontinent are lifted and transported long distances westwards, across the Southeast Atlantic Ocean. The negligible wet scavenging of these absorbing aerosols leads to a near-persistent smoke layer above one of the largest stratocumulus cloud deck on the planet. Therefore, the Southeast Atlantic region is a very important area for studying the impact of above cloud absorbing aerosols, their radiative forcing and their possible effects on clouds. In this study we aim to analyse and quantify the effect of smoke loadings on cloud properties using a synergy of different remote sensing technics from A-Train retrievals (methods based on the passive instruments POLDER and MODIS and the operational method of the spaceborne lidar CALIOP), collocated with ERA-Interim re-analysis meteorological profiles. To analyse the possible mechanisms of AACs effects on cloud properties, we developed a high and low aerosol loading approach, that consists in evaluating the change in radiative quantities (i.e. cloud top cooling, heating rate vertical profiles) and cloud properties with the smoke loading. During this analysis, we account for the variation in the meteorological conditions over our sample area. The results show that the region we focus on is primarily under the energetic influence of absorbing aerosols, leading to a significant positive shortwave direct effect at the top of the atmosphere. For larger loads of AACs, clouds are optically thicker, with an increase in liquid water path of 20 g m−2 and lower cloud top altitudes by 100 m. These results do not contradict the semi-direct effect of above cloud aerosols, explored in previous studies. Furthermore, we observe a strong correlation between the aerosol and the water vapor loadings, which has to be accounted for. A detailed analysis of the heating rates shows that the absorbing aerosols are 90 % responsible for warming the ambient air where they reside, with approximately + 5.7 K/day, while the accompanying water vapour above clouds has a longwave effect of + 4.7 K/day (equivalent to 7 % decrease) on the cloud top cooling. We infer that this decreased cloud top cooling in particular, in addition with the higher humidity above the clouds, might modify the cloud top entrainment rate and its effect, leading to thicker clouds. Therefore, smoke (the combination of aerosol and water vapor) events would have the potential to modify and probably reinforce the underlaying cloud cover.


Nanomaterials ◽  
2019 ◽  
Vol 9 (1) ◽  
pp. 64 ◽  
Author(s):  
Qin Wang ◽  
Hui Xie ◽  
Zhiming Hu ◽  
Chao Liu

In this study, molecular dynamics simulations were carried out to study the coupling effect of electric field strength and surface wettability on the condensation process of water vapor. Our results show that an electric field can rotate water molecules upward and restrict condensation. Formed clusters are stretched to become columns above the threshold strength of the field, causing the condensation rate to drop quickly. The enhancement of surface attraction force boosts the rearrangement of water molecules adjacent to the surface and exaggerates the threshold value for shape transformation. In addition, the contact area between clusters and the surface increases with increasing amounts of surface attraction force, which raises the condensation efficiency. Thus, the condensation rate of water vapor on a surface under an electric field is determined by competition between intermolecular forces from the electric field and the surface.


Atmosphere ◽  
2021 ◽  
Vol 12 (3) ◽  
pp. 291
Author(s):  
Jinpeng Lu ◽  
Fei Xie ◽  
Hongying Tian ◽  
Jiali Luo

Stratospheric water vapor (SWV) changes play an important role in regulating global climate change, and its variations are controlled by tropopause temperature. This study estimates the impacts of tropopause layer ozone changes on tropopause temperature by radiative process and further influences on lower stratospheric water vapor (LSWV) using the Whole Atmosphere Community Climate Model (WACCM4). It is found that a 10% depletion in global (mid-low and polar latitudes) tropopause layer ozone causes a significant cooling of the tropical cold-point tropopause with a maximum cooling of 0.3 K, and a corresponding reduction in LSWV with a maximum value of 0.06 ppmv. The depletion of tropopause layer ozone at mid-low latitudes results in cooling of the tropical cold-point tropopause by radiative processes and a corresponding LSWV reduction. However, the effect of polar tropopause layer ozone depletion on tropical cold-point tropopause temperature and LSWV is opposite to and weaker than the effect of tropopause layer ozone depletion at mid-low latitudes. Finally, the joint effect of tropopause layer ozone depletion (at mid-low and polar latitudes) causes a negative cold-point tropopause temperature and a decreased tropical LSWV. Conversely, the impact of a 10% increase in global tropopause layer ozone on LSWV is exactly the opposite of the impact of ozone depletion. After 2000, tropopause layer ozone decreased at mid-low latitudes and increased at high latitudes. These tropopause layer ozone changes at different latitudes cause joint cooling in the tropical cold-point tropopause and a reduction in LSWV. Clarifying the impacts of tropopause layer ozone changes on LSWV clearly is important for understanding and predicting SWV changes in the context of future global ozone recovery.


1990 ◽  
Vol 118 (12) ◽  
pp. 2513-2542 ◽  
Author(s):  
Ross N. Hoffman ◽  
Christopher Grassotti ◽  
Ronald G. Isaacs ◽  
Jean-Francois Louis ◽  
Thomas Nehrkorn ◽  
...  

2021 ◽  
Author(s):  
Tomasz Hadas ◽  
Grzegorz Marut ◽  
Jan Kapłon ◽  
Witold Rohm

<p>The dynamics of water vapor distribution in the troposphere, measured with Global Navigation Satellite Systems (GNSS), is a subject of weather research and climate studies. With GNSS, remote sensing of the troposphere in Europe is performed continuously and operationally under the E-GVAP (http://egvap.dmi.dk/) program with more than 2000 permanent stations. These data are one of the assimilation system component of mesoscale weather prediction models (10 km scale) for many nations across Europe. However, advancing precise local forecasts for severe weather requires high resolution models and observing system.   Further densification of the tracking network, e.g. in urban or mountain areas, will be costly when considering geodetic-grade equipment. However, the rapid development of GNSS-based applications results in a dynamic release of mass-market GNSS receivers. It has been demonstrated that post-processing of GPS-data from a dual-frequency low-cost receiver allows retrieving ZTD with high accuracy. Although low-cost receivers are a promising solution to the problem of densifying GNSS networks for water vapor monitoring, there are still some technological limitations and they require further development and calibration.</p><p>We have developed a low-cost GNSS station, dedicated to real-time GNSS meteorology, which provides GPS, GLONASS and Galileo dual-frequency observations either in RINEX v3.04 format or via RTCM v3.3 stream, with either Ethernet or GSM data transmission. The first two units are deployed in a close vicinity of permanent station WROC, which belongs to the International GNSS Service (IGS) network. Therefore, we compare results from real-time and near real-time processing of GNSS observations from a low-cost unit with IGS Final products. We also investigate the impact of replacing a standard patch antenna with an inexpensive survey-grade antenna. Finally, we deploy a local network of low-cost receivers in and around the city of Wroclaw, Poland, in order to analyze the dynamics of troposphere delay at a very high spatial resolution.</p><p>As a measure of accuracy, we use the standard deviation of ZTD differences between estimated ZTD and IGS Final product. For the near real-time mode, that accuracy is 5 mm and 6 mm, for single- (L1) and dual-frequency (L1/L5,E5b) solution, respectively. Lower accuracy of the dual-frequency relative solution we justify by the missing antenna phase center correction model for L5 and E5b frequencies. With the real-time Precise Point Positioning technique, we estimate ZTD with the accuracy of 7.5 – 8.6 mm. After antenna replacement, the accuracy is improved almost by a factor of 2 (to 4.1 mm), which is close to the 3.1 mm accuracy which we obtain in real-time using data from the WROC station.</p>


Author(s):  
Christoforus Bayu Risanto ◽  
Christopher L. Castro ◽  
Avelino F. Arellano ◽  
James M. Moker ◽  
David K. Adams

AbstractWe assess the impact of GPS precipitable water vapor (GPS-PWV) data assimilation (DA) on short-range North American monsoon (NAM) precipitation forecasts, across 38 days with weak synoptic forcing, during the NAM GPS Hydrometeorological Network field campaign in 2017 over northwest Mexico. Utilizing an ensemble-based data assimilation technique, the GPS-PWV data retrieved from 18 observation sites are assimilated every hour for 12 hours into a 30-member ensemble convective-permitting (2.5 km) Advanced Research version of the Weather Research and Forecasting (WRF-ARW) model. As the assimilation of the GPS-PWV improves the initial condition of WRF by reducing the root mean square error and bias of PWV across 1200-1800 UTC, this also leads to an improvement in capturing nocturnal convection of mesoscale convective systems (MCSs; after 0300 UTC) and to an increase by 0.1 mm h-1 in subsequent precipitation during the 0300-0600 UTC period relative to no assimilation of the GPS-PWV (NODA) over the area with relatively more observation sites. This response is consistent with observed precipitation from the Integrated Multi-satellitE Retrievals for Global Precipitation Measurement Final Precipitation product. Moreover, compared to the NODA, we find that the GPS-PWV DA decreases cloud top temperature, increases most unstable convective available energy and surface dewpoint temperature, and thus creates a more favorable condition for convective organization in the region.


2021 ◽  
Author(s):  
Diego G. Miralles ◽  
Dominik L. Schumacher ◽  
Jessica Keune ◽  
Paul A. Dirmeyer

<p>The predicted increase in drought occurrence and intensity will pose serious threats to global future water and food security. This was hinted by several historically unprecedented droughts over the last two decades, taking place in Europe, Australia, Amazonia or the USA. It has been hypothesised that the strength of these events responded to self-reinforcement processes related to land–atmospheric feedbacks: as rainfall deficits dry out soil and vegetation, the evaporation of land water is reduced, then the local air becomes too dry to yield rainfall, which further enhances drought conditions. Despite the 'local' nature of these feedbacks, their consequences can be remote, as downwind regions may rely on evaporated water transported by winds from drought-affected locations. Following this rationale, droughts may not only self-reinforce locally, due to land atmospheric feedbacks, but <em>self-propagate</em> in the downwind direction, always conditioned on atmospheric circulation. This propagation is not only meteorological but relies on soil moisture drought, and may lead to a downwind cascading of impacts on water resources. However, a global capacity to observe these processes is lacking, and thus our knowledge of how droughts start and evolve, and how this may change as climate changes, remains limited. Furthermore, climate and forecast models are still immature when it comes to representing the influences of land on rainfall.</p><p>Here, the largest global drought events are studied to unravel the role of land–atmosphere feedbacks during the spatiotemporal propagation of these events. We based our study on satellite and reanalysis records of soil moisture, evaporation, air humidity, winds and precipitation, in combination with a Lagrangian framework that can map water vapor trajectories and explore multi-dimensional feedbacks. We estimate the reduction in precipitation in the direction of drought propagation that is caused by the upwind soil moisture drought, and isolate this effect from the influence of potential evaporation and circulation changes. By doing so, the downwind lack of precipitation caused by upwind soil drought via water vapor deficits, and hence the impact of drought self-propagation, is determined. We show that droughts occurring in dryland regions are particularly prone to self-propagate, as evaporation there tends to respond strongly to enhanced soil stress and precipitation is frequently convective. This kind of knowledge may be used to improve climate and forecast models and can be exploited to develop geo-engineering mitigation strategies to help prevent drought events from aggravating during their early stages.</p>


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